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Transport in molecular electronic devices is different from that in semiconductor mesoscopic devices in two important aspects: (1) the effect of the electronic structure and (2) the effect of the interface to the external contact. A…

介观与纳米尺度物理 · 物理学 2009-11-07 Yongqiang Xue , Supriyo Datta , Mark A. Ratner

Devices for nano- and molecular size electronics are currently a focus of research aimed at an efficient current rectification and switching. A few generic molecular scale devices are reviewed here on the basis of first-principles and model…

软凝聚态物质 · 物理学 2015-06-25 A. M. Bratkovsky

Solvation effect might have a tremendous influence on chemical reactions. However, precise quantum chemistry calculations are most often done either in vacuum neglecting the role of the solvent or using continuum solvent model ignoring its…

化学物理 · 物理学 2020-07-14 Guillaume Jeanmairet , Maximilien Levesque , Daniel Borgis

We study the kinetics of the distribution function for charged particles of hard momentum in scalar QED. The goal is to understand the effects of infrared divergences associated with the exchange of quasistatic magnetic photons in the…

高能物理 - 唯象学 · 物理学 2016-08-25 D. Boyanovsky , H. J. de Vega

Electrophoresis is a motion of charged dispersed particles relative to a fluid in a uniform electric field. The effect is widely used to separate macromolecules, to assemble colloidal structures, to transport particles in nano- and…

软凝聚态物质 · 物理学 2011-01-21 Oleg D. Lavrentovich , Israel Lazo , Oleg P. Pishnyak

We analyze the interplay between vibrational and electronic degrees of freedom in charge transport across a molecular single-electron transistor. We focus on the wide class of molecules which possess quasi-degenerate vibrational…

软凝聚态物质 · 物理学 2007-05-23 Andrea Donarini , Milena Grifoni , Klaus Richter

The one-dimensional kinetic equation with integral of collisions type BGK (Bhatnagar, Gross and Krook) and frequency of collisions affine depending on the module of molecular velocity is constructed. Laws of preservation of number of…

数学物理 · 物理学 2014-03-11 A. L. Bugrimov , A. V. Latyshev , A. A. Yushkanov

We investigated a mechanism of rectification in di-block oligomer diode molecules that have recently been synthesized and showed a pronounced asymmetry in the measured I-V spectrum. The observed rectification effect is due to the resonant…

其他凝聚态物理 · 物理学 2009-11-11 I. I. Oleynik , M. A. Kozhushner , V. S. Posvyanskii , L. Yu

Ocean turbulence plays a key role in shaping large-scale circulation, heat uptake, and biogeochemical processes. The kinetic energy (KE) wavenumber spectrum is a fundamental diagnostic, quantifying how KE is distributed across spatial…

大气与海洋物理 · 物理学 2026-05-12 Ayantika Bhattacharjee , Spencer Jones , Dhruv Balwada , Shane Elipot , Manuel Gutierrez-Villanueva

We study current rectification effect in an asymmetric molecule HOOC-C$_6$H$_4$-(CH$_2$)$_n$ sandwiched between two Aluminum electrodes using an {\sl ab initio} nonequilibrium Green function method. The conductance of the system decreases…

介观与纳米尺度物理 · 物理学 2009-11-11 Yan-hong Zhou , Xiao-hong Zheng , Ying Xu , Zhao Yang Zeng

The second-order nonlinear responses of inviscid chiral fluids near local equilibrium are investigated by applying the chiral kinetic theory (CKT) incorporating side-jump effects. It is shown that the local equilibrium distribution function…

高能物理 - 理论 · 物理学 2019-04-09 Yoshimasa Hidaka , Shi Pu , Di-Lun Yang

Within the frame of quantum dissipation theory, we develop a new hierarchical equations of motion theory, combined with the small polaron transformation. We fully investigate the electron transport of a single attractive impurity system…

介观与纳米尺度物理 · 物理学 2013-06-04 Feng Jiang , Shikuan Wang , Hang Xie , Yonghong Yan , YiJing Yan

We derive from a microscopic Hamiltonian a set of stochastic equations of motion for a system of spinless charged particles in an electromagnetic (EM) field based on a consistent application of a dimensionful 1/c expansion of quantum…

量子物理 · 物理学 2012-06-05 C. H. Fleming , P. R. Johnson , B. L. Hu

Transport of ions in molecular-scale confined spaces is central to all aspects of life and technology: into a crack, it may break steel within days; through a membrane separator, it determines the efficiency of electrochemical energy…

软凝聚态物质 · 物理学 2021-04-05 H. -W. Cheng , J. Dziadkowiec , V. Wieser , A. M. Imre , M. Valtiner

This tutorial article presents a "bottom-up" view of electrical resistance starting from something really small, like a molecule, and then discussing the issues that arises as we move to bigger conductors. Remarkably, no serious quantum…

介观与纳米尺度物理 · 物理学 2007-05-23 Supriyo Datta

The performances of lubricated systems widely used in natural, biological, and artificial settings are traditionally dictated by their load bearing capacities. Here we unveil that, by exploiting a unique coupling between interfacial…

流体动力学 · 物理学 2022-07-26 Siddhartha Mukherjee , Jayabrata Dhar , Sunando DasGupta , Suman Chakraborty

We describe a quantum electromechanical system(QEMS) comprising a single quantum dot harmonically bound between two electrodes and facilitating a tunneling current between them. An example of such a system is a fullerene molecule between…

介观与纳米尺度物理 · 物理学 2007-05-23 D. Wahyu Utami , Hsi-Sheng Goan , G. J. Milburn

A possible model for quantum kinematics of a test particle in a curved space-time is proposed. Every reasonable neighbourhood V_e of a curved space-time can be equipped with a nonassociative binary operation called the geodesic…

高能物理 - 理论 · 物理学 2011-04-15 P. Kuusk , J. Ord

A simple experimentally accessible realization of current rectification by molecules (molecular films) bridging metal electrodes is described. It is based on the spatial asymmetry of the molecule and requires only one resonant conducting…

软凝聚态物质 · 物理学 2009-11-07 P. E. Kornilovitch , A. M. Bratkovsky , R. S. Williams

Rectified transport of active ellipsoidal particles is numerically investigated in a two-dimensional asymmetric potential. The out-of-equilibrium condition for the active particle is an intrinsic property, which can break thermodynamical…

软凝聚态物质 · 物理学 2015-05-12 Bao-quan Ai , Jian-chun Wu