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Heterobilayers consisting of MoSe$_2$ and WSe$_2$ monolayers can host optically bright interlayer excitons with intriguing properties such as ultralong lifetimes and pronounced circular polarization of their photoluminescence due to valley…

In monolayer transition metal dichalcogenide semiconductors, valley coherence degrades rapidly due to a combination of fast scattering and inter-valley exchange interaction. This leads to a sub-picosecond valley coherence time, making…

介观与纳米尺度物理 · 物理学 2023-07-21 Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Monolayer transition metal dichalcogenides have attracted great attentions for potential applications in valleytronics. However, the valley polarization degree is usually not high because of the intervalley scattering. Here, we demonstrate…

材料科学 · 物理学 2023-02-23 Jianchen Dang , Mingwei Yang , Xin Xie , Zhen Yang , Danjie Dai , Zhanchun Zuo , Can Wang , Kuijuan Jin , Xiulai Xu

We have investigated the steady-sate valley polarization and valley coherence of encapsulated MoS2 monolayer as a function of the temperature and the power density with a continuous wave laser excitation. Both valley polarization and…

材料科学 · 物理学 2021-11-01 Fabian Cadiz , Stefan Gerl , Takashi Taniguchi , Kenji Watanabe

We report on scattering induced valley polarization enhancement in monolayer molybdenum disulfide. With thermally activated and charge doping introduced scattering, our sample exhibits seven? and twelve-folds of improvements respectively.…

光学 · 物理学 2021-10-13 Yueh-Chun Wu , Takashi Taniguchi , Kenji Watanabe , Jun Yan

Two-dimensional transition metal dichalcogenide (TMD) semiconductors provide a unique possibility to access the electronic valley degree of freedom using polarized light, opening the way to valley information transfer between distant…

The thermal, mechanical, and electronic performance of atomically thin semiconductors is governed by their low-energy phonons, yet the impact of atomic-scale disorder on these modes remains poorly understood. Here, we report the first…

材料科学 · 物理学 2026-01-22 Aleksandar Radic , Boyao Liu , Akshay Rao , Sam Lambrick

Moir\'e superlattices created by stacking atomic layers of transition metal dichalcogenide semiconductors have emerged as a class of fascinating artificial photonic and electronic materials. An appealing attribute of these structures is the…

介观与纳米尺度物理 · 物理学 2025-03-11 Yueh-Chun Wu , Matthew DeCapua , ZhongChen Xu , Takashi Taniguchi , Kenji Watanabe , YouGuo Shi , Jun Yan

A monolayer of $MoS_{2}$ has a non-centrosymmetric crystal structure, with spin polarized bands. It is a two valley semiconductor with direct gap falling in the visible range of the electromagnetic spectrum. Its optical properties are of…

介观与纳米尺度物理 · 物理学 2023-06-09 Zhou Li , J. P. Carbotte

We present helium atom micro-diffraction as an ideal technique for characterization of 2D materials due to its ultimate surface sensitivity combined with sub-micron spatial resolution. Thermal energy neutral helium scatters from the valence…

In atomically thin two-dimensional semiconductors such as transition metal dichalcogenides (TMDs), controlling the density and type of defects promises to be an effective approach for engineering light-matter interactions. We demonstrate…

介观与纳米尺度物理 · 物理学 2018-08-15 Galan Moody , Kha Tran , Xiaobo Lu , Travis Autry , James M. Fraser , Richard P. Mirin , Li Yang , Xiaoqin Li , Kevin L. Silverman

The band structure of transition metal dichalcogenides (TMDCs) with valence band edges at different locations in the momentum space could be harnessed to build devices that operate relying on the valley degree of freedom. To realize such…

介观与纳米尺度物理 · 物理学 2016-09-06 Oriol Lopez Sanchez , Dmitry Ovchinnikov , Shikhar Misra , Adrien Allain , Andras Kis

In the strong light-matter coupling regime realized e.g. by integrating semiconductors into optical microcavities, polaritons as new hybrid light-matter quasi-particles are formed. The corresponding change in the dispersion relation has a…

材料科学 · 物理学 2022-09-08 Beatriz Ferreira , Roberto Rosati , Ermin Malic

We investigate with polarized microphotoluminescence the optical pumping of the valley degree of freedom in charge-tunable MoS2 monolayers encapsulated with hexagonal boron nitride at cryogenic temperatures. We report a large steady state…

介观与纳米尺度物理 · 物理学 2021-10-15 Sangjun Park , Steve Arscott , Takashi Taniguchi , Kenji Watanabe , Fausto Sirotti , Fabian Cadiz

The strong light matter interaction and the valley selective optical selection rules make monolayer (ML) MoS2 an exciting 2D material for fundamental physics and optoelectronics applications. But so far optical transition linewidths even at…

Coherence is a crucial requirement to realize quantum manipulation through light-matter interactions. Here we report the observation of anomalously robust valley polarization and valley coherence in bilayer WS2. The polarization of the…

介观与纳米尺度物理 · 物理学 2023-07-21 Bairen Zhu , Hualing Zeng , Junfeng Dai , Zhirui Gong , Xiaodong Cui

We predict the existence and study properties of the valley Hall edge solitons in a composite photonic graphene with a domain wall between two honeycomb lattices with broken inversion symmetry. Inversion symmetry in our system is broken due…

Spin-orbit coupling is a fundamental mechanism that connects the spin of a charge carrier with its momentum. Likewise, in the optical domain, a synthetic spin-orbit coupling is accessible, for instance, by engineering optical anisotropies…

The valley degree of freedom of electrons in solids has been proposed as a new type of information carriers beyond the electronic charge and spin. Recent experimental demonstrations of the optical orientation of the valley polarization and…

介观与纳米尺度物理 · 物理学 2017-07-14 Jieun Lee , Kin Fai Mak , Jie Shan

Valley, as a new degree of freedom for electrons, has drawn considerable attention due to its significant potential for encoding and storing information. Lifting the energy degeneracy to achieve valley polarization is necessary for…

材料科学 · 物理学 2020-03-11 Pei Zhaos , Yandong Ma , Hao Wang , Baibiao Huang , Liangzhi Kou , Ying Dai