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To understand the interaction between nitrogen dopants and native point defects in graphene, we have studied the energetic stability of N-doped graphene with vacancies and Stone-Wales (SW) defect by performing the density functional theory…

介观与纳米尺度物理 · 物理学 2012-05-03 Zhufeng Hou , Xianlong Wang , Takashi Ikeda , Kiyoyuki Terakura , Masaharu Oshima , Masa-aki Kakimoto , Seizo Miyata

Sulfur and nitrogen dual doped graphene have been extensively investigated in the field of oxygen reduction reaction, supercapacitors and batteries, but their magnetic and absorption performance have not been explored. Besides, the effects…

应用物理 · 物理学 2020-03-24 L. Quan , H. T. Lu , F. X. Qin , D. Estevez , Y. F. Wang , Y. H. Li , Y. Tian , H. Wang , H. X. Peng

Mechanically exfoliated graphene layers deposited on SiO2 substrate were irradiated with Ar+ ions in order to experimentally study the effect of atomic scale defects and disorder on the low-energy electronic structure of graphene. The…

介观与纳米尺度物理 · 物理学 2009-01-21 Levente Tapaszto , Gergely Dobrik , Peter Nemes-Incze , Gabor Vertesy , Philippe Lambin , Laszlo P Biro

Graphene has emerged as an electronic material that is promising for device applications and for studying two-dimensional electron gases with relativistic dispersion near two Dirac points. Nonetheless, deviations from Dirac-like…

材料科学 · 物理学 2009-07-23 M. L. Teague , A. P. Lai , J. Velasco , C. R. Hughes , A. D. Beyer , M. W. Bockrath , C. N. Lau , N. -C. Yeh

Although defects on graphene can degrade electron transport and its ability for use as a protection layer, they can also be helpful to tailor the local properties or activate new sites for particular adsorbates. Here, carbon vacancy defects…

材料科学 · 物理学 2018-05-23 Tianbai Li , Jory A. Yarmoff

Combining scanning tunneling microscopy and angle-resolved photoemission spectroscopy, we demonstrate how to tune the doping of epitaxial graphene from p to n by exploiting the structural changes that occur spontaneously on the Ge surface…

To minimize parasitic doping effects caused by uncontrolled material adsorption, graphene is often investigated under vacuum. Here we report an entirely unexpected phenomenon occurring in vacuum systems, namely strong n-doping of graphene…

介观与纳米尺度物理 · 物理学 2013-11-11 Christophe Caillier , Dong-Keun Ki , Yuliya Lisunova , Iaroslav Gaponenko , Patrycja Paruch , Alberto F. Morpurgo

While doping and defects are often considered detrimental to material performance, at the nanoscale, modifications are needed to create novel properties beneficial for device applications. In this work, we focus on optimizing graphene as a…

应用物理 · 物理学 2025-05-21 Raju Kumar Yadav , Prince Philip , Boddepalli SanthiBhushan

The electronic transport of monolayer graphene devices is studied before and after \emph{in situ} deposition of a sub-monolayer coating of osmium adatoms. Unexpectedly, and unlike all other metallic adatoms studied to date, osmium adatoms…

介观与纳米尺度物理 · 物理学 2019-12-11 Jamie A. Elias , Erik A. Henriksen

We performed density functional theory calculations on heterostructures of single layers of hexagonal BN and MoS$_2$ to assess the effect of doping in the BN sheet and of interstitial Na atoms on the electronic properties of the adjacent…

介观与纳米尺度物理 · 物理学 2015-06-19 Roland Gillen , John Robertson , Janina Maultzsch

The effect of oxygen adsorption on the local structure and electronic properties of monolayer graphene grown on SiC(0001) has been studied by means of Low Energy Electron Microscopy (LEEM), microprobe Low Energy Electron Diffraction…

材料科学 · 物理学 2015-06-05 C. Mathieu , B. Lalmi , T. O. Mentes , E. Pallecchi , A. Locatelli , S. Latil , R. Belkhou , A. Ouerghi

Hydrogenated graphene, graphane, is studied on oxygen-terminated silicon dioxide substrate using ab initio calculations. A structure with hydrogenation only on one side of the graphene layer is found stable and its hydrogen configurations…

介观与纳米尺度物理 · 物理学 2011-07-13 M. Ijäs , P. Havu , A. Harju , P. Pasanen

Bottom-up fabrication of graphene antidot lattices (GALs) has previously yielded atomically precise structures with sub-nanometer periodicity. Focusing on this type of experimentally realized GAL, we perform density functional theory…

介观与纳米尺度物理 · 物理学 2016-07-28 Søren J. Brun , Vitor M. Pereira , Thomas G. Pedersen

It has been shown that graphene doping is sufficient to lead to an improvement in the critical current density - field performance (Jc(B)), with little change in the transition temperature in MgB2. At 3.7 at% graphene doping of MgB2 an…

超导电性 · 物理学 2015-05-18 X. Xu , S. X. Dou , X. L. Wang , J. H. Kim , J. A. Stride , M. Choucair , W. K. Yeoh , R. K. Zheng , S. P. Ringer

Graphene, a two-dimensional (2D) promising emergent photocatalyst consisting of earth-abundant elements. This study evaluated the potential of graphene oxide (GO) towards photocatalytic degradation of a novel organic dye, Methylene Blue…

Nitrogen-doped graphene was recently synthesized and was reported to be a catalyst for hydrogen dissociative adsorption under a perpendicular applied electric field (F). In this work, the diffusion of H atoms on N-doped graphene, in the…

材料科学 · 物理学 2012-02-15 Z. M. Ao , A. D. Hernández-Nieves , F. M. Peeters , S. Li

It has been shown that the first C layer on the SiC(0001)(2{\times}2)C surface already exhibits graphene-like electronic structure, with linear pi bands near the Dirac point. Indeed, the (2{\times}2)C reconstruction, with a Si adatom and C…

介观与纳米尺度物理 · 物理学 2015-05-27 F. Hiebel , P. Mallet , J. -Y. Veuillen , L. Magaud

Heavily doping graphene by intercalation can raise its Fermi level near an extended van Hove singularity, potentially inducing correlated electronic phases. Intercalation also modifies the band structure: dopants may hybridize with carbon…

Graphene on noble-metal nanostructures constitutes an attractive nanocomposite with possible applications in sensors or energy conversion. In this work we study the properties of hybrid graphene/gold nanoparticle structures by Raman…

介观与纳米尺度物理 · 物理学 2018-06-14 András Pálinkás , Péter Kun , Antal A. Koós , Zoltán Osváth

In order to realize applications of hydrogen-adsorbed graphene, a main issue is how to control hydrogen adsorption/desorption at room temperature. In this study, we demonstrate the possibility to tune hydrogen adsorption on graphene by…

介观与纳米尺度物理 · 物理学 2019-05-07 Yuya Murata , Arrigo Calzolari , Stefan Heun