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The ac nonlinear dielectric response $\chi_3(\omega,T)$ of glycerol was measured close to its glass transition temperature $T_g$ to investigate the prediction that supercooled liquids respond in an increasingly non-linear way as the…

软凝聚态物质 · 物理学 2015-05-18 C. Crauste-Thibierge , C. Brun , F. Ladieu , D. L'Hote , G. Biroli , J-P. Bouchaud

Advances in high-precision dielectric spectroscopy has enabled access to non-linear susceptibilities of polar molecular liquids. The observed non-monotonic behavior has been claimed to provide strong support for theories of dynamic arrest…

软凝聚态物质 · 物理学 2021-07-07 Thomas Speck

It is commonly accepted that shear waves do not propagate in a liquid medium. The shear wave energy is supposed to dissipate nearly instantaneously. This statement originates from the difficulty to access static shear stress in macroscopic…

介观与纳米尺度物理 · 物理学 2021-07-28 Eni Kume , Alessio Zaccone , Laurence Noirez

The temperature evolution of the broadband $10^{-6}$-$10^{10}$ Hz dielectric susceptibility of the paradigmatic glass formers glycerol, propylene carbonate, and fluoro-aniline is analyzed assuming a three-step relaxation due to the…

无序系统与神经网络 · 物理学 2007-05-23 Catalin Gainaru , Alexander Brodin , Vladimir Novikov , Ernst A. Rössler

We study theoretically the non-linear response properties of glass formers. We establish several general results which, together with the assumption of Time-Temperature Superposition, lead to a relation between the non-linear response and…

统计力学 · 物理学 2009-12-19 Marco Tarzia , Giulio Biroli , Jean-Philippe Bouchaud , Alexandre Lefèvre

We performed parallel measurements of heat effects and shear modulus relaxation for glassy Te$_{75}$Ge$_{15}$Ga$_{10}$ taken as a representative of practically important non-metallic glasses with covalent bonding. It is shown that the heat…

无序系统与神经网络 · 物理学 2026-05-27 G. V. Afonin , R. A. Konchakov , D. A. Chareev , S. A. Badmaeva , R. S. Khmyrov , A. N. Vasiliev , N. P. Kobelev , V. A. Khonik

The dielectric response of supercooled liquids is phenomenologically modeled by a set of Asymmetric Double Wells (ADW), where each ADW contains a dynamical heterogeneity of $N_{corr}$ molecules. We find that the linear macroscopic…

软凝聚态物质 · 物理学 2012-03-08 François Ladieu , Coralie Brun , Denis L'Hôte

We present a high sensitivity method allowing the measurement of the non linear dielectric susceptibility of an insulating material at finite frequency. It has been developped for the study of dynamic heterogeneities in supercooled liquids…

材料科学 · 物理学 2009-11-17 C. Thibierge , D. L'Hote , F. Ladieu , R. Tourbot

We review the works devoted to third and fifth harmonic susceptibilities in glasses, namely $\chi$ (3) 3 and $\chi$ (5) 5. We explain why these nonlinear responses are especially well adapted to test whether or not some amorphous…

软凝聚态物质 · 物理学 2020-01-29 Samuel Albert , M. Michl , P. Lunkenheimer , A. Loidl , P. Déjardin , F. Ladieu

Dielectric study over a broadband was carried out from 10 to 70 K on ceramic Gd1-xYxMnO3 (x= 0.2, 0.3, and 0.4). For all the compositions, a prominent sharp peak about ~18K was observed in the temperature dependence of both {\epsilon}'(T)…

材料科学 · 物理学 2017-06-28 R. M. Sarguna , V. Sridahran , A. M. Awasthi , N. Subramanian

Experimental measurements of the specific heat in glass-forming systems reveal anomalies in the temperature dependence of the specific heat, including the so called "specific heat peak" in the vicinity of the glass transition. The aim of…

统计力学 · 物理学 2009-11-13 H. G. E. Hentschel , Valery Ilyin , Itamar Procaccia , Nurith Schupper

We have investigated the effect that dissipation may have on the cavitation process in normal liquid $^3$He. Our results indicate that a rather small dissipation decreases sizeably the quantum-to-thermal crossover temperature $T^*$ for…

凝聚态物理 · 物理学 2009-10-31 Dora M. Jezek , Marti Pi , Manuel Barranco

Magnetic dc susceptibility between 1.5 and 800 K, ac susceptibility and magnetization, thermodynamic properties, temperature dependence of radio and audio-wave dielectric constants and conductivity, contact-free dielectric constants at…

The frequency-dependent dielectric constant, shear and adiabatic bulk moduli, longitudinal thermal expansion coefficient, and longitudinal specific heat have been measured for two van der Waals glass-forming liquids,…

软凝聚态物质 · 物理学 2012-02-28 Bo Jakobsen , Tina Hecksher , Kristine Niss , Tage Christensen , Niels Boye Olsen , Jeppe C. Dyre

A theory of weakly-nonlinear low-temperature relaxational absorption of acoustic and electromagnetic waves in dielectric and metallic glasses is developed. Basing upon the model of two-level tunneling systems we show that the nonlinear…

无序系统与神经网络 · 物理学 2009-10-30 M. Kirkengen , Yu. M. Galperin

We search for a Gardner transition in glassy glycerol, a standard molecular glass, measuring the third harmonics cubic susceptibility $\chi_3^{(3)}$ from slightly below the usual glass transition temperature down to $10K$. According to the…

无序系统与神经网络 · 物理学 2021-01-20 Samuel Albert , Giulio Biroli , François Ladieu , Roland Tourbot , Pierfrancesco Urbani

Dielectric relaxation and thermal expansion spectroscopy were made for thin polystyrene films in order to measure the temperature $T_{\alpha}$ corresponding to the peak in the loss component of susceptibility due to the $\alpha$-process and…

软凝聚态物质 · 物理学 2007-05-23 Koji Fukao , Yoshihisa Miyamoto

The thermo-mechanical effect in superfluid helium is used to create an initial chemical potential difference, $\Delta \mu_0$, across a solid $^4$He sample. This $\Delta \mu_0$ causes a flow of helium atoms from one reservoir filled with…

其他凝聚态物理 · 物理学 2015-06-22 Ye. Vekhov , R. B. Hallock

Experimental measurements of nonlinear dielectric response in glassformers like supercooled glycerol or propylene carbonate have been interpreted as providing evidence for a growing thermodynamic length scale when lowering temperature. A…

无序系统与神经网络 · 物理学 2026-01-08 Eric Bertin , François Ladieu

We revisit the issue of the leading nonanalytic corrections to the temperature dependence of the specific heat coefficient, $\gamma (T)=C(T)/T,$ for a system of interacting fermions in three dimensions. We show that the leading temperature…

强关联电子 · 物理学 2009-02-06 A. V. Chubukov , D. L. Maslov , A. J. Millis
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