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We analyze static properties of a strongly confined semiflexible polymer, i.e. either trapped in a closed space or compressed by external forces, in an athermal solvent. Like a flexible polymer case, we can resort to an analogy with the…

软凝聚态物质 · 物理学 2009-11-13 Takahiro Sakaue

Phase diagram of the ground states of DNA in a bad solvent is studied for a semi-flexible polymer model with a generalized local elastic bending potential characterized by a nonlinearity parameter $x$ and effective self-attraction promoting…

生物大分子 · 定量生物学 2016-01-28 Trinh X. Hoang , Hoa Lan Trinh , Achille Giacometti , Rudolf Podgornik , Jayanth R. Banavar , Amos Maritan

The dynamics of loop formation by linear polymer chains has been a topic of several theoretical/experimental studies. Formation of loops and their opening are key processes in many important biological processes. Loop formation in flexible…

软凝聚态物质 · 物理学 2015-05-14 K. P. Santo , K. L. Sebastian

A theoretical study of toroidal membranes with various degrees of intrinsic orientational order is presented at mean-field level. The study uses a simple Ginzburg-Landau style free energy functional, which gives rise to a rich variety of…

凝聚态物理 · 物理学 2009-10-22 R. M. L. Evans

We have studied the transition in shape of two dimensional polyampholytes using Monte Carlo simulation. We observe that polymers with randomly charged monomers get into a globular shape at lower temperatures, provided that their total…

凝聚态物理 · 物理学 2007-05-23 M. R. Ejtehadi , S. Rouhani

A coarse grained model for flexible polymers end-grafted to repulsive spherical nanoparticles is studied for various chain lengths and grafting densities under good solvent conditions, by Molecular Dynamics methods and density functional…

软凝聚态物质 · 物理学 2015-05-18 Federica Lo Verso , Sergei A. Egorov , Andrey Milchev , Kurt Binder

We have studied structure formation in a confined block copolymer melt by means of dynamic density functional theory (DDFT). The confinement is two-dimensional, and the confined geometry is that of a cylindrical nanopore. Although the…

软凝聚态物质 · 物理学 2009-11-13 G. J. A. Sevink , A. V. Zvelindovsky

Biomolecules are often very long with a definite chirality. DNA, xanthan and poly-gamma-benzyl-glutamate (PBLG) can all form columnar crystalline phases. The chirality, however, competes with the tendency for crystalline order. For chiral…

凝聚态物理 · 物理学 2009-10-28 Randall D. Kamien , David R. Nelson

The percentage and sequence of AT and GC base pairs and charges on the DNA backbone contribute significantly to the stiffness of DNA. This elastic property of DNA also changes with small interacting ligands. The single-molecule force…

软凝聚态物质 · 物理学 2017-02-02 Anurag Singh , Amar Nath Gupta

Borophene is a two-dimensional material made out of boron atoms only. It exhibits polymorphism and different allotropes can be studied in terms of a rigid electronic structure, where only the occupation of the states change with the respect…

材料科学 · 物理学 2025-09-24 Alam Osorio , Lucia Reining , Francesco Sottile

In the paper we investigate statistical and topological properties of fractional Brownian polymer chains, equipped with the short-range volume interactions. The attention is paid to statistical properties of collapsed conformations with the…

软凝聚态物质 · 物理学 2021-06-09 A. M. Astakhov , V. A. Avetisov , S. K. Nechaev , K. E. Polovnikov

Monte Carlo simulations are used to study the conformational behavior of a semiflexible polymer confined to cylindrical and conical channels. The channels are sufficiently narrow that the conditions for the Odijk regime are marginally…

软凝聚态物质 · 物理学 2020-12-02 James M. Polson , Cameron G. Hastie

The structure of flexible polymers endgrafted in cylindrical pores of diameter D is studied as a function of chain length N and grafting density \sigma, assuming good solvent conditions. A phenomenological scaling theory, describing the…

软凝聚态物质 · 物理学 2009-11-11 D. I. Dimitrov , A. Milchev , K. Binder

We extend the Rouse model of polymer dynamics to situations of non-stationary chain growth. For a dragged polymer chain of length $N(t) = t^\alpha$, we find two transitions in conformational dynamics. At $\alpha= 1/2$, the propagation of…

软凝聚态物质 · 物理学 2016-07-25 Ali Malek , Reiner Kree

Here, we provide an overview of theoretical approaches to semiflexible polymers and their networks. Such semiflexible polymers have large bending rigidities that can compete with the entropic tendency of a chain to crumple up into a random…

软凝聚态物质 · 物理学 2016-05-25 Chase P. Broedersz , Fred. C. MacKintosh

We have studied the thermodynamics of isolated homopolymer chains of varying stiffness using a lattice model. A complex phase behaviour is found; phases include chain-folded `crystalline' structures, the disordered globule and the coil. It…

软凝聚态物质 · 物理学 2008-02-03 Jonathan Doye , Richard Sear , Daan Frenkel

In the hexagonal columnar phase of chiral polymers a bias towards cholesteric twist competes with braiding along an average direction. When the chirality is strong, topological defects proliferate, leading to either a tilt grain boundary…

软凝聚态物质 · 物理学 2007-05-23 Randall D. Kamien

Polymer chains immersed in different solvent molecules exhibit diverse properties due to multiple spatiotemporal scales and complex interactions. Using molecular dynamics simulations, we study the conformational and static properties of…

软凝聚态物质 · 物理学 2024-07-08 Hong-Yao Li , Bokai Zhang , Zhi-Yong Wang

We study the dynamics of a single chain polymer confined to a two dimensional cell. We introduce a kinetically constrained lattice gas model that preserves the connectivity of the chain, and we use this kinetically constrained model to…

统计力学 · 物理学 2011-11-09 Armin Rahmani , Claudio Castelnovo , Jeremy Schmit , Claudio Chamon

Entangled states are ubiquitous amongst fibrous materials, whether naturally occurring (keratin, collagen, DNA) or synthetic (nanotube assemblies, elastane). A key mechanical characteristic of these systems is their ability to reorganise in…