相关论文: Instabilities govern the low-frequency vibrational…
Amorphous solids are dynamically inhomogeneous due to in lack of translational symmetry and hence exhibit vibrational properties different from crystalline solids with anomalous low frequency vibrational density of states (VDOS) and related…
We show through simulations of amorphous solids prepared in open boundary conditions that they possess significantly fewer low-frequency vibrational modes compared to their periodic boundary counterparts. Specifically, using measurements of…
Recently, progress has been made in the understanding of anomalous vibrational excitations in amorphous solids. In the lowest-frequency region, the vibrational spectrum follows a non-Debye quartic law, which persists up to zero frequency…
Interpreting the vibrational properties of amorphous solids beyond Debye's theory is challenging due to the presence of inhomogeneity on the mesoscopic scale. In this work, we model this inhomogeneity by real-space fluctuating elasticity…
Atomic vibrations play a vital role in the functions of various physical, chemical, and biological systems. The vibrational properties and the specific heat of crystalline bulk materials are well described by Debye theory, which…
The vibrational density of states $D(\omega)$ of solids controls their thermal and transport properties. In crystals, the low-frequency modes are extended phonons distributed in frequency according to Debye's law, $D(\omega) \propto…
A theory of vibrational excitations based on power-law spatial correlations in the elastic constants (or equivalently in the internal stress) is derived, in order to determine the vibrational density of states $D(\omega)$ of disordered…
The low-frequency vibrational and low-temperature thermal properties of amorphous solids are markedly different from those of crystalline solids. This situation is counter-intuitive because any solid material is expected to behave as a…
Amorphous solids tend to present an abundance of soft elastic modes, which diminish their transport properties, generate heterogeneities in their elastic response, and affect non-linear processes like thermal activation of plasticity. This…
Mechanical deformation of amorphous solids can be described as consisting of an elastic part in which the stress increases linearly with strain, up to a yield point at which the solid either fractures or starts deforming plastically. It is…
We study energy minimized configurations of amorphous solids with a simple shear degree of freedom. We show that the low-frequency regime of the vibrational density of states of structural glass formers is crucially sensitive to the…
The low-frequency vibrations of glasses are markedly different from those of crystals. These vibrations have recently been categorized into two types: spatially extended vibrations, whose vibrational density of states (vDOS) follows a…
The vibrational spectra of solids, both ordered and amorphous, in the low-energy regime, control the thermal and transport properties of materials, from heat capacity to heat conduction, electron-phonon couplings, conventional…
We consider the contribution to the density of vibrational states and the distribution of energy barrier heights of incipient instabilities in a glass modeled by a jammed packing of spheres. On approaching an instability, the frequency of a…
Glasses possess more low-frequency vibrational modes than predicted by Debye theory. These excess modes are crucial for the understanding the low temperature thermal and mechanical properties of glasses, which differ from those of…
Much of the discussion in the literature of the low frequency part of the density of states of amorphous solids was dominated for years by comparing measured or simulated density of states to the classical Debye model. Since this model is…
We build a minimal, mean-field, model of plasticity of amorphous solids, based upon a phenomenology of dissipative events derived, in a preceding paper [A. Lemaitre, C. Caroli, arXiv:0705.0823] from extensive molecular simulations. It…
Quasi-localised modes appear in the vibrational spectrum of amorphous solids at low-frequency. Though never formalised, these modes are believed to have a close relationship with other important local excitations, including shear…
Glasses have a large excess of low-frequency vibrational modes in comparison with crystalline solids. We show that such a feature is a necessary consequence of the geometry generic to weakly connected solids. In particular, we analyze the…
Recent research has made significant progress in understanding the non-phonon vibrational states present in amorphous materials. It has been established that their vibrational density of states follows non-Debye scaling laws. Here, we show…