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Accurate determination of the exciton binding energy and reduced effective mass in halide perovskites is of utmost importance for the selective design of optoelectronic devices. Although these properties are currently determined by several…

We study the linear optical absorption of bulk semiconductors in the presence of a homogeneous constant (dc) electric field with an approach suitable for including excitonic effects while working with many-band models. The absorption…

介观与纳米尺度物理 · 物理学 2015-06-19 Federico Duque-Gomez , J. E. Sipe

Lead iodide perovskites have attracted considerable interest in the upcoming photovoltaic technologies and optoelectronic devices. Therefore, an accurate theoretical description of the electronic and optical properties especially to…

材料科学 · 物理学 2022-01-20 Pooja Basera , Arunima Singh , Deepika Gill , Saswata Bhattacharya

A major obstacle for computing optical spectra of solids is the lack of reliable approximations for capturing excitonic effects within time-dependent density-functional theory. We show that the trustful prediction of strongly bound…

Electronic states of the hybrid perovskite enable their promising applications as distinctive optoelectronic materials. The understanding of their electronic structures and charge characters remains highly controversial. The electronic…

Direct-gap materials hold promises for excitonic insulator. In contrast to indirect-gap materials, here the difficulty to distinguish from a Peierls charge density wave is circumvented. However, direct-gap materials still suffer from the…

材料科学 · 物理学 2018-08-29 Zeyu Jiang , Yuanchang Li , Shengbai Zhang , Wenhui Duan

The energy band structure of excitons is studied in periodic potentials produced by the short-range interaction between the exciton and electrons of Wigner or Moir\'{e} lattices. Treating the exciton as a point-like dipole that interacts…

材料科学 · 物理学 2023-08-16 Dinh Van Tuan , Hanan Dery

The exciton absorption coefficient is determined analytically for a semiconductor superlattice in crossed electric and magnetic fields, for the magnetic field being parallel and the electric field being perpendicular to the superlattice…

介观与纳米尺度物理 · 物理学 2019-03-27 B. S. Monozon , V. G. Bezchastnov , P. Schmelcher

Owing to both electronic and dielectric confinement effects, two-dimensional organic-inorganic hybrid perovskites sustain strongly bound excitons at room temperature. Here, we demonstrate that there are non-negligible contributions to the…

The magnetic field dependence of photoabsorption provides direct insights into the band structure of semiconductors. It is perhaps surprising that there is a large discrepancy between electron, hole, and reduced mass reported in the recent…

介观与纳米尺度物理 · 物理学 2025-01-22 Jack N. Engdahl , Harley D. Scammell , Dmitry K. Efimkin , Oleg P. Sushkov

We present an \textit{ab initio} method to calculate phonon-assisted absorption and emission spectra in the presence of strong excitonic effects. We apply the method to bulk hexagonal BN which has an indirect band gap and is known for its…

We compare first-principle band gaps and optical absorption spectra of single- and double-layer fluorographene with bulk graphite fluoride. The electronic properties are calculated using the many-body GW approximation and the optical…

材料科学 · 物理学 2014-10-24 František Karlický , Michal Otyepka

We calculate the binding energy, transition energies, oscillator strength, and absorption coefficient of indirect excitons in transition metal dichalcogenide (TMDC) double layers separated by an integer number of hexagonal boron nitride…

介观与纳米尺度物理 · 物理学 2018-09-19 Matthew N. Brunetti , Oleg L. Berman , Roman Ya. Kezerashvili

Polaronic effects involving stabilization of localized charge character by structural deformations and polarizations have attracted considerable investigations in soft lattice lead halide perovskites. However, the concept of polaron…

Perovskites have attracted much attention due to their remarkable optical properties. While it is well established that excitons dominate their optical response, the impact of higher excitonic states and formation of phonon sidebands in…

The exciton binding energy ($E_b$) is a key parameter that governs the physics of many optoelectronic devices. At their best, trustworthy and precise measurements of $E_b$ challenge theoreticians to refine models, are a driving force in…

材料科学 · 物理学 2023-06-27 Kameron R. Hansen , John S. Colton , Luisa Whittaker-Brooks

Excitons, bound electron-hole pairs, are responsible for strong optical resonances near the bandgap in low-dimensional materials and wide-bandgap insulators. Although current ab initio methods can accurately determine exciton energies and…

介观与纳米尺度物理 · 物理学 2026-05-12 Muralidhar Nalabothula , Davide Sangalli , Fulvio Paleari , Sven Reichardt , Ludger Wirtz

Antiperovskite derivatives have emerged as promising candidates for optoelectronic applications. However, due to the significant computational cost, their excitonic and polaronic properties remain underexplored despite being critical for…

材料科学 · 物理学 2025-10-23 Ayan Chakravorty , Surajit Adhikari , Priya Johari

Shift current transient are obtained for near band gap excitation of bulk GaAs by numerical solutions of the semiconductor Bloch equations in a basis obtained from a 14 band k.p model of the band structure. This approach provides a…

介观与纳米尺度物理 · 物理学 2017-11-08 Reinold Podzimski , Huynh Thanh Duc , Torsten Meier

Wannier-Mott excitons in a semiconductor layered superlattice (SL) of period much smaller than the 2D exciton Bohr radius in the presence of a longitudinal external dc electric field directed parallel to the SL axis are investigated…

介观与纳米尺度物理 · 物理学 2017-01-04 B. S. Monozon , P. Schmelcher
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