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The Dirac equation for H$_2^+$ is solved numerically using an iterative method proposed by Kutzelnigg [Z. Phys. 11, 15 (1989]. The four-component wavefunction is expanded in a newly introduced kinetically balanced exponential basis set. The…

原子物理 · 物理学 2022-06-15 Hugo D. Nogueira , Vladimir I. Korobov , Jean-Philippe Karr

A new approach to finite basis sets for the Dirac equation is developed. It solves the problem of spurious states and, as a result, improves the convergence properties of basis set calculations. The efficiency of the method is demonstrated…

原子物理 · 物理学 2009-11-10 V. M. Shabaev , I. I. Tupitsyn , V. A. Yerokhin , G. Plunien , G. Soff

We present a high-precision solution of Dirac equation by numerically solving the minmax two-center Dirac equation with the finite element method (FEM). The minmax FEM provide a highly accurate benchmark result for systems with light or…

量子物理 · 物理学 2024-11-22 Ossama Kullie

A two-dimensional, fully numerical approach to the solution of four-component Dirac-Fock equation using the moderately long Hermitian basis of B-splines is applied to H, H2+ and H2 in a strong magnetic field. The geometric parameters,…

天体物理学 · 物理学 2007-05-23 G. B. Deineka

Dual kinetic balance (DKB) technique was previously developed to eliminate spurious states in the finite-basis-set-based solution of the Dirac equation in central fields. In the present paper, it is extended to the Dirac equation for…

原子物理 · 物理学 2014-02-14 E. B. Rozenbaum , D. A. Glazov , V. M. Shabaev , K. E. Sosnova , D. A. Telnov

We present a precise fully relativistic numerical solution of the two-center Coulomb problem. The special case of unit nuclear charges is relevant for the accurate description of the ${\rm H}_2^+$ molecular ion and its isotopologues,…

量子物理 · 物理学 2022-05-11 O. Kullie , S. Schiller

The electronic spectra of light one-electron quasi-molecular compounds H-H$^+$, He$^+$-He$^2+$ and He$^+$-H$^+$ are analyzed. To this end, the two-center Dirac equation is solved by the dual-kinetically balanced finite-basis-set method for…

原子物理 · 物理学 2025-09-11 D. Solovyev , A. Anikin , A. Danilov , D. Glazov , A. Kotov

A procedure is described for the precise nonrelativistic evaluation of the dipole polarizabilities of H_2^+ and D_2^+ that avoids any approximation based on the size of the electron mass relative to the nucleus mass. The procedure is…

原子物理 · 物理学 2007-05-23 J. M. Taylor , A. Dalgarno , J. F. Babb

The dual-kinetic-balance (DKB) finite basis set method for solving the Dirac equation for hydrogen-like ions [V. M. Shabaev et al., Phys. Rev. Lett. 93, 130405 (2004)] is extended to problems with a non-local spherically-symmetric…

原子物理 · 物理学 2011-07-13 Kyle Beloy , Andrei Derevianko

The time-dependent Dirac equation can be solved exactly for ionization induced by ultrarelativistic heavy ion collisions. Ionization calculations are carried out in such a framework for a number of representative ion-ion pairs. For each…

原子物理 · 物理学 2009-10-31 Anthony J. Baltz

A non-perturbative approach to the solution of the time-dependent, two-center Dirac equation is presented with a special emphasis on the proper treatment of the potential of the nuclei. In order to account for the full multipole expansion…

原子物理 · 物理学 2012-11-14 S. R. McConnell , A. N. Artemyev , M. Mai , A. Surzhykov

We calculate the bound-electron $g$ factor for a wide range of rovibrational states of the molecular hydrogen ions H$_2^+$ and HD$^+$. Relativistic and QED corrections of orders up to $\alpha^5$ are taken into account. All contributions are…

原子物理 · 物理学 2025-08-07 Ossama Kullie , Hugo D. Nogueira , Jean-Philippe Karr

We use the Dirac equation to study the mass spectrum of mesons with heavy-light quark combinations. First we study the Dirac equation with spherically symmetry and funnel potential, and apply them on the hydrogen-like atom problem to check…

高能物理 - 唯象学 · 物理学 2011-11-24 B. Pan

The rigorous two-center approach based on the dual-kinetically balanced finite-basis-set expansion is applied to one-electron, heteronuclear diatomic Bi-Au, U-Pb, and Cf-U quasimolecules. The obtained $1\sigma$ ground-state energies are…

The static and dynamic electric multipolar polarizabilities and second hyperpolarizabilities of the H$_2^+$, D$_2^+$, and HD$^+$ molecular ions in the ground and first excited states are calculated nonrelativistically using explicitly…

原子物理 · 物理学 2014-09-23 Li-Yan Tang , Zong-Chao Yan , Ting-Yun Shi , James F. Babb

Two numerical methods are used to evaluate the relativistic spectrum of the two-centre Coulomb problem (for the $H_{2}^{+}$ and $Th_{2}^{179+}$ diatomic molecules) in the fixed nuclei approximation by solving the single particle…

化学物理 · 物理学 2012-10-01 F. Fillion-Gourdeau , E. Lorin , A. D. Bandrauk

General transformation expressions of the second-order non-adiabatic Hamiltonian of the atomic nuclei, including the kinetic-energy correction terms, are derived upon the change from laboratory-fixed Cartesian coordinates to general…

化学物理 · 物理学 2018-12-05 Edit Mátyus

In this work, we propose an efficient and accurate computational method to evaluate the many-potential $\alpha\left(Z\alpha\right)^{n\ge3}$ vacuum polarization density of hydrogen-like atoms within the finite-basis approximation of the…

原子物理 · 物理学 2023-07-26 Maen Salman , Trond Saue

Accurate predictions for hydrogen molecular levels require the treatment of electrons and nuclei on an equal footing. While nonrelativistic theory has been effectively formulated this way, calculation of relativistic and quantum…

化学物理 · 物理学 2024-01-24 Krzysztof Pachucki , Jacek Komasa

The possible use of high-resolution rovibrational spectroscopy of the hydrogen molecular ions H + 2 and HD + for an independent determination of several fundamental constants is analyzed. While these molecules had been proposed for…

原子物理 · 物理学 2017-02-20 J. -Ph Karr , L Hilico , Jeroen Koelemeij , Vladimir Korobov
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