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How does nonequilibrium activity modify the approach to a glass? This is an important question, since many experiments reveal the near-glassy nature of the cell interior, remodelled by activity. However, different simulations of dense…

软凝聚态物质 · 物理学 2018-08-28 Saroj Kumar Nandi , Rituparno Mandal , Pranab Jyoti Bhuyan , Chandan Dasgupta , Madan Rao , Nir. S. Gov

Dense active matter, in the fluid or amorphous-solid form, has generated intense interest as a model for the dynamics inside living cells and multicellular systems. An extension of the random first-order transition theory (RFOT) to include…

软凝聚态物质 · 物理学 2021-02-16 Rituparno Mandal , Saroj Kumar Nandi , Chandan Dasgupta , Peter Sollich , Nir S. Gov

Activity-driven glassy dynamics, while ubiquitous in collective cell migration, intracellular transport, dynamics in bacterial and ant colonies, etc., also extend the scope and extent of the as-yet mysterious physics of glass transition.…

软凝聚态物质 · 物理学 2023-05-11 Kallol Paul , Anoop Mutneja , Saroj Kumar Nandi , Smarajit Karmakar

Activity-mediated unjamming of a confluent glassy system is crucial for several biological processes, such as embryogenesis and cancer metastasis. During these processes, the cells progressively change their junction properties,…

软凝聚态物质 · 物理学 2025-05-13 Souvik Sadhukhan , Chandan Dasgupta , Saroj Kumar Nandi

Active glasses refer to a class of driven non-equilibrium systems that share remarkably similar dynamical behavior as conventional glass-formers in equilibrium. Glass-like dynamical characteristics have been observed in various biological…

软凝聚态物质 · 物理学 2024-12-24 Subhodeep Dey , Smarajit Karmakar

The steep increase of the relaxation time of glass forming liquids upon cooling is traditionally ascribed to an impending entropy crisis: since the system has "nowhere to go", dynamics must come to a halt. This classic argument, due to Adam…

无序系统与神经网络 · 物理学 2024-02-23 Jean-Philippe Bouchaud

We analyze the ways in which the random first order phase transition (RFOT) of the glass transition differs from the well-studied regular first order and second order (or continuous) phase transitions. Just as is the case in the latter two…

统计力学 · 物理学 2024-09-23 T. R. Kirkpatrick , D. Thirumalai

The dramatic slowdown of glass-forming liquids has been variously linked to increasing dynamic and static correlation lengths. Yet, empirical evidence is insufficient to decide among competing theories. The random first order theory (RFOT)…

无序系统与神经网络 · 物理学 2010-02-25 C. Cammarota , A. Cavagna , G. Gradenigo , T. S. Grigera , P. Verrocchio

The Random First Order Transition (RFOT) theory of glasses provides a unified framework for explaining the observed correlations of the kinetic and thermodynamic behaviors of glass-forming liquids having a wide variety of chemical…

软凝聚态物质 · 物理学 2025-07-29 M. H. Brown , P. G. Wolynes

The routine transformation of a liquid, as it is cooled rapidly, resulting in glass formation, is remarkably complex. A theoretical explanation of the dynamics associated with this process has remained one of the major unsolved problems in…

无序系统与神经网络 · 物理学 2014-12-17 T. R. Kirkpatrick , D. Thirumalai

We compute the temperature-dependent barrier for alpha-relaxations in several liquids, without adjustable parameters, using experimentally determined elastic, structural, and calorimetric data. We employ the random first order…

无序系统与神经网络 · 物理学 2013-10-17 Pyotr Rabochiy , Peter G. Wolynes , Vassiliy Lubchenko

The random first-order transition (RFOT) theory of the structural glass transition is reviewed in a pedagogical fashion. The rigidity that emerges in crystals and glassy liquids is of the same fundamental origin. In both cases, it…

无序系统与神经网络 · 物理学 2015-11-20 Vassiliy Lubchenko

We develop a real space renormalisation group analysis of disordered models of glasses, in particular of the spin models at the origin of the Random First Order Transition theory. We find three fixed points respectively associated to the…

无序系统与神经网络 · 物理学 2017-07-05 Maria Chiara Angelini , Giulio Biroli

A unified treatment of structural relaxation in a deeply supercooled glassy liquid is developed which extends the existing mode coupling theory (MCT) by incorporating the effects of activated events by using the concepts from the random…

无序系统与神经网络 · 物理学 2007-05-23 Sarika Maitra Bhattacharyya , Biman Bagchi , Peter G. Wolynes

Extensive computer simulations are performed for a few model glass-forming liquids in both two and three dimensions to study their dynamics when a randomly chosen fraction of particles are frozen in their equilibrium positions. For all the…

统计力学 · 物理学 2016-08-03 Saurish Chakrabarty , Rajsekhar Das , Smarajit Karmakar , Chandan Dasgupta

According to the Random First Order Transition (RFOT) theory of glasses, the barriers for activated dynamics in supercooled liquids vanish as the temperature of a viscous liquid approaches the dynamical transition temperature from below.…

无序系统与神经网络 · 物理学 2009-11-10 Vassiliy Lubchenko , Peter G. Wolynes

The aim of this paper is to summarise the basic arguments and the intuition bolstering the RFOT picture for glasses, based on a finite dimensional extension of mean-field models with an exponentially large number of metastable states. We…

无序系统与神经网络 · 物理学 2009-12-15 G. Biroli , J. P. Bouchaud

Dynamics near the surface of glasses is generally much faster than in the bulk. Neglecting static perturbations of structure at the surface, we use random first order transition theory to show the free energy barrier for activated motion…

软凝聚态物质 · 物理学 2009-11-13 Jacob D. Stevenson , Peter G. Wolynes

The possible role of growing static order in the dynamical slowing down towards the glass transition has recently attracted considerable attention. On the basis of random first-order transition (RFOT) theory, a new method to measure the…

软凝聚态物质 · 物理学 2016-02-17 John Russo , Hajime Tanaka

We use Brownian dynamics simulations of a binary mixture of highly charged spherical colloidal particles to illustrate many of the implications of the Random First Order Transition (RFOT) theory (PRA 40 1045 (1989)), which is the only…

统计力学 · 物理学 2015-06-12 Hongsuk Kang , T. R. Kirkpatrick , D. Thirumalai
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