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In strained heteroepitaxy, two-dimensional (2D) layers can exhibit a critical thickness at which three-dimensional (3D) islands self-assemble, relieving misfit strain at the cost of an increased surface area. Here we show that such a…

Surface energies play a dominant role in the self-assembly of three dimensional (3D) nanostructures. In this letter, we show that using surfactants to modify surface energies can provide a means to externally control nanostructure…

介观与纳米尺度物理 · 物理学 2017-07-24 Ryan B. Lewis , Pierre Corfdir , Jesús Herranz , Hanno Küpers , Uwe Jahn , Oliver Brandt , Lutz Geelhaar

Quantum dot (QD) growth on high ($c_{3v}$) symmetry GaAs{111} surfaces holds promise for efficient entangled photon sources. Unfortunately, homoepitaxy on GaAs{111} surfaces suffers from surface roughness/defects and InAs deposition does…

材料科学 · 物理学 2023-11-14 Ahmed M. Hassanen , Jesus Herranz , Lutz Geelhaar , Ryan B. Lewis

The size distribution of self-assembled InAs quantum dots grown on (001) InP under the Stranski-Krastanow growth mode is controlled using selective area/chemical beam epitaxy, which allows the formation of quantum dots at specific…

介观与纳米尺度物理 · 物理学 2007-05-23 J. Lefebvre , P. J. Poole , J. Fraser , G. C. Aers , D. Chithrani , R. L. Williams

The evolution of InAs quantum dots grown on InP substrates by metal-organic vapour phase epitaxy is studied as a function of InAs coverage. Under specific growth conditions, the onset of the two- to three-dimensional transition is seen to…

材料科学 · 物理学 2007-05-23 Bhavtosh Bansal , M. R. Gokhale , Arnab Bhattacharya , B. M. Arora

Self-assembled InAs quantum dots (QDs) grown on GaAs(001) surface by molecular beam epitaxy under continuous and growth-interruption modes exhibit two families of QDs, quasi-3D (Q3D) and 3D QDs, whose volume density evolution is…

材料科学 · 物理学 2009-11-13 A. Balzarotti

We studied the size distribution and its scaling behavior of self-assembled InAlAs/AlGaAs quantum dots (QDs) grown on GaAs with the Stranski-Krastanov (SK) mode by molecular beam epitaxy (MBE), at both 480{\deg}C and 510{\deg}C, as a…

材料科学 · 物理学 2015-06-05 X. M. Lu , M. Koyama , Y. Izumi , Y. Nakata , S. Adachi , S. Muto

Bismuth (Bi) atomic layers are known as 2D topological materials with variety of the electronic structures and topological orders depending on the number of stacking layers. Recently, it is reported that few layers of Bi grown on…

材料科学 · 物理学 2023-01-02 Yoshiyuki Ohtsubo , Takuto Nakamura , Shin-ichi Kimura

Emerging applications of self-assembled semiconductor quantum dot (QD)-based nonclassical light sources emitting in the telecom C-band (1530 to 1565 nm) present challenges in terms of controlled synthesis of their low-density ensembles,…

The equilibrium shapes of InAs quantum dots (i.e., dislocation-free, strained islands with sizes >= 10,000 atoms) grown on a GaAs (001) substrate are studied using a hybrid approach which combines density functional theory (DFT)…

材料科学 · 物理学 2009-10-31 N. Moll , M. Scheffler , E. Pehlke

We report on a new approach for positioning of self-assembled InAs quantum dots on (110) GaAs with nanometer precision. By combining self-assembly of quantum dots with molecular beam epitaxy on in-situ cleaved surfaces (cleaved-edge…

介观与纳米尺度物理 · 物理学 2007-05-23 J. Bauer , D. Schuh , E. Uccelli , R. Schulz , A. Kress , F. Hofbauer , J. J. Finley , G. Abstreiter

We analyze the shape and position of heteroepitaxial InAs islands on the top face of cylindrical GaAs(111)A nanopillars experimentally and theoretically. Catalyst-free molecular beam epitaxial growth of InAs at low temperatures on GaAs…

材料科学 · 物理学 2020-01-14 T. Riedl , V. S. Kunnathully , A. Trapp , T. Langer , D. Reuter , J. K. N. Lindner

The formation of dislocation-free three-dimensional islands during the heteroepitaxial growth of lattice-mismatched materials has been observed experimentally for several material systems. The equilibrium shape of the islands is governed by…

材料科学 · 物理学 2008-02-03 E. Pehlke , N. Moll , M. Scheffler

The two- to three-dimensional growth transition in the InAs/GaAs(001) heterostructure has been investigated by atomic force microscopy. The kinetics of the density of three dimensional quantum dots evidences two transition thresholds at…

材料科学 · 物理学 2009-11-11 F. Arciprete , E. Placidi , V. Sessi , M. Fanfoni , F. Patella , A. Balzarotti

The thermodynamics of the Stranski-Krastanov mode of epitaxial growth and the effect of the sign of the lattice misfit are discussed. The Stranski-Krastanov mode of growth represents a sequence of layer-by-layer or Frank-van der Merwe…

材料科学 · 物理学 2017-11-10 J. E. Prieto , I. Markov

We report the growth of self-assembled Bi2Se3 quantum dots (QDs) by molecular beam epitaxy on GaAs substrates using the droplet epitaxy technique. The QD formation occurs after anneal of Bismuth droplets under Selenium flux.…

材料科学 · 物理学 2020-05-22 Marcel S. Claro , Abhinandan Gangopadhyay , David J. Smith , Maria C. Tamargo

We have revisited the epitaxial growth modes of Fe on W(110) and Mo(110), and propose an overview or our contribution to the field. We show that the Stranski-Krastanov growth mode, recognized for a long time in these systems, is in fact…

We investigate the optical properties of InAs quantum dots grown by molecular beam epitaxy on GaAs(110) using Bi as a surfactant. The quantum dots are synthesized on planar GaAs(110) substrates as well as on the {110} sidewall facets of…

介观与纳米尺度物理 · 物理学 2017-08-02 Pierre Corfdir , Ryan B. Lewis , Lutz Geelhaar , Oliver Brandt

Tailoring electronic and optical properties of self-assembled InAs quantum dots (QDs) is a critical limit for the design of several QD-based optoelectronic devices operating in the telecom frequency range. We describe how a fine control of…

介观与纳米尺度物理 · 物理学 2015-06-18 Vittorianna Tasco , Muhammad Usman , Milena De Giorgi , Adriana Passaseo

Quantum dots have promising properties for optoelectronic applications. They can be grown free of dislocations in highly mismatched epitaxy in the coherent Stranski-Krastanov mode. In this chapter, some thermodynamic aspects related to the…

材料科学 · 物理学 2007-05-23 J. E. Prieto , E. Korutcheva , I. Markov
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