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Confined acoustic and optical phonons in Si nanoclusters embedded in sapphire, synthesized using ion-beam implantation are investigated using Raman spectroscopy. The l = 0 and l = 2 confined acoustic phonons, found at low Raman shift, are…

材料科学 · 物理学 2008-09-10 Satyaprakash Sahoo , S. Dhara , S. Mahadevan , A. K. Arora

A modified phonon confinement model considering the size distribution, an improved phonon dispersion curve and a confinement function is developed for the calculation of size dependent Raman spectra of the silicon (Si) nanocrystals. The…

介观与纳米尺度物理 · 物理学 2015-05-13 Sanjeev K. Gupta , Prafulla K. Jha

A comparative analysis of two Raman line-shape functions has been carried out to validate the true representation of experimentally observed Raman scattering data for semiconducting nanomaterials. A modified form of already existing phonon…

Strong light-matter coupling gives rise to polaritons -- quasiparticles that combine both photonic and material characteristics. Here, we show that polar nanocrystals exhibit structure- and environment-dependent Raman scattering, enabled by…

In the present paper, we utilize the coupled-oscillator model describing the hybridization of optical phonons in touching and/or overlapping particles in order to study the Raman spectra of nanoparticles organized into various types of…

介观与纳米尺度物理 · 物理学 2023-12-01 S. V. Koniakhin , O. I. Utesov , A. G. Yashenkin

Intermediate frequency range (511 - 514 cm-1) Si phonons in Si-SiO2 nanocomposites are shown to have contribution from both core1 and surface/interface1 Si phonons, where, ratio of contribution of the two depends on the size of a Si…

介观与纳米尺度物理 · 物理学 2015-03-13 Ekta Rani , Alka Ingale , A. Chaturvedi , M. P. Joshi , L. M. Kukreja

We present Raman spectroscopy of the polycrystalline Si and Ge films deposited by molecular beam deposition on a dielectric substrate. The Raman study has been made using lasers with different wavelengths. Structural properties of the…

A comparison of experimentally observed Raman scattering data with Raman line-shapes, generated theoretically using phonon confinement model, has been carried out to understand the sensitivity of different Raman spectral parameters on…

介观与纳米尺度物理 · 物理学 2020-03-20 Neeshu K. M. , Chanchal Rani , Ritika Kaushik , Manushree Tanwar , Ashisha Kumar , Rajesh Kumar

Raman spectra from silicon nanostructures, recorded using excitation laser power density of 1.0 kW/cm^2, is employed here to reveal the dominance of thermal effects at temperatures higher than the room temperature. Room temperature Raman…

介观与纳米尺度物理 · 物理学 2012-01-25 Rajesh Kumar , Vivek Kumar , A. K. Shukla

Raman spectroscopy of crystalline/molecular systems is well backed with quantum chemical calculations and group theory, making it a unique characterization tool. For the "intermediate" case of nanoscale systems, however, the use of Raman…

化学物理 · 物理学 2017-04-07 Vitaly I. Korepanov , Hiro-o Hamaguchi

Phonons-quantized vibrational modes in crystalline structures-govern phenomena ranging from thermal and mechanical transport to quantum mechanics. In recent years, a new class of artificial materials called phononic crystals has emerged,…

介观与纳米尺度物理 · 物理学 2024-12-03 Michele Diego , Roman Anufriev , Ryoto Yanagisawa , Masahiro Nomura

We study the effect of confinement on the phonon properties of ultra-narrow silicon nanowires of side sizes of 1-10nm . We use the modified valence force field method to compute the phononic dispersion, and extract the density of states,…

介观与纳米尺度物理 · 物理学 2013-04-05 Hossein Karamitaheri , Neophytos Neophytou , Mohsen Karami Taheri , Rahim Faez , Hans Kosina

We have measured polarized spectra of Raman scattering, infrared and optical transmission of NaV_2O_5 single crystals above the temperature of the spin-Peierls transition Tsp=35 K. Some of the far-infrared (FIR) phonon lines are strongly…

强关联电子 · 物理学 2009-10-30 S. A. Golubchik , M. Isobe , A. N. Ivlev , B. N. Mavrin , M. N. Popova , A. B. Sushkov , Yu. Ueda , A. N. Vasil'ev

A theoretical study describing the coherence properties of near-field Raman scattering in two- and one-dimensional systems is presented. The model is applied to the Raman modes of pristine graphene and graphene edges. Our analysis is based…

介观与纳米尺度物理 · 物理学 2014-03-31 Luiz Gustavo Cançado , Ryan Beams , Ado Jorio , Lukas Novotny

Phonons diffraction and interference patterns are observed at the atomic scale, using molecular dynamics simulations in systems containing crystalline silicon and nanometric obstacles as voids or amorphous-inclusions. The diffraction…

We calculate low-frequency Raman scattering from the confined acoustic phonon modes of CdS1-xSex nanoparticles embedded in borosilicate glass. The calculation of the Raman scattering by acoustic phonons in nanoparticles has been performed…

介观与纳米尺度物理 · 物理学 2009-04-16 Sanjeev K. Gupta , Prafulla K. Jha , Satyaprakash Sahoo , A. K. Arora , Y. M. Azhniuk

Together with their fingerprint modes, molecules carry coherent vibrations of all their atoms (phonons). Phonon spectra extend from $\sim$20 to more than $10^{4}\,\mu$m, depending on molecular size. These spectra are discrete but large…

星系天体物理 · 物理学 2015-05-20 Renaud Papoular

Raman scattering from the acoustic phonons confied in si nanocrystals is investigated by a microscopic lattice-dynamical calculation. Polarized and depolarized spectra are found to be rather different, indicated from different acoustic…

软凝聚态物质 · 物理学 2009-10-31 J. Zi , K. Zhang , x. Xie

Extending the idea of optical microcavities to sound waves, we propose a {\it phonon cavity} consisting of two semiconductor superlattices enclosing a spacer with thickness determined by the acoustic wavelength at the center of the first…

凝聚态物理 · 物理学 2009-11-07 M. Trigo , A. Bruchhausen , A. Fainstein , B. Jusserand , V. Thierry-Mieg

We used Raman scattering for study the phonon modes of self-organized Ge/Si quantum dots, grown by a molecular-beam epitaxy method. It is revealed, that Ge-Ge and Si-Ge vibrational modes considerably intensify at excitation of exciton…

介观与纳米尺度物理 · 物理学 2011-05-17 I. V. Kucherenko , V. S. Vinogradov , N. N. Melnik , L. V. Arapkina , V. A. Chapnin , K. V. Chizh , V. A. Yuryev
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