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With the global transition towards cleaner energy and sustainable processes, the demand for efficient catalysts, especially for the oxygen reduction reaction, has gained attention from the scientific community. This research work…

Graphene is, in principle, a promising material for consideration as component (support, active site) of electrocatalytic materials, particularly with respect to reduction of oxygen, an electrode reaction of importance to low-temperature…

Graphite is one of the most chemically inert materials. Its elementary constituent, monolayer graphene, is generally expected to inherit most of the parent material's properties including chemical inertness. Here we show that, unlike…

Application of graphene-type materials in electrocatalysis is a topic of growing scientific and technological interest. A tremendous amount of research has been carried out in the field of oxygen electroreduction, particularly with respect…

The chemical production of graphene as well as its controlled wet- chemical modification is a challenge for synthetic chemists and the characterization of reaction products requires sophisticated analytic methods. In this review we first…

化学物理 · 物理学 2018-05-09 Siegfried Eigler , Andreas Hirsch

Catalysts for oxygen reduction and evolution reactions are at the heart of key renewable energy technologies including fuel cells and water splitting. Despite tremendous efforts, developing oxygen electrode catalysts with high activity at…

材料科学 · 物理学 2011-08-12 Yongye Liang , Yanguang Li , Hailiang Wang , Jigang Zhou , Jian Wang , Tom Regier , Hongjie Dai

Here we describe a computational study undertaken in an effort to elucidate the reaction mechanisms behind the experimentally observed oxidations and hydrations catalyzed by graphene oxide (GO). Using the oxidation of benzyl alcohol to…

材料科学 · 物理学 2012-11-13 Danil W. Boukhvalov , Daniel R. Dreyer , Christopher W. Bielawski , Young-Woo Son

One of the most important developments in condensed matter physics in recent years has been the discovery and characterization of graphene. A two-dimensional layer of Carbon arranged in a hexagonal lattice, graphene exhibits many…

高能物理 - 格点 · 物理学 2015-09-23 Christopher Winterowd , Carleton DeTar , Savvas Zafeiropoulos

Methanol occupies a central role in chemical synthesis and is considered an ideal candidate for cleaner fuel storage and transportation. It can be catalyzed from water and volatile organic compounds such as carbon dioxide, thereby offering…

化学物理 · 物理学 2018-09-18 William Foster , Juan A. Aguilar , Halim Kusumaatmaja , Kislon Voïtchovsky

Based on first principles density functional theory calculations we explored energetics of oxygen reduction reaction over pristine and nitrogen-doped graphene with different amounts of nitrogen doping. The process of oxygen reduction…

材料科学 · 物理学 2012-05-04 Danil W. Boukhvalov , Young-Woo Son

Graphene and related two-dimensional materials are promising candidates for atomically thin, flexible, and transparent optoelectronics. In particular, the strong light-matter interaction in graphene has allowed for the development of…

While freestanding clean graphene is essential for various applications, existing technologies for removing the polymer layer after transfer of graphene to the desired substrate still leave significant contaminations behind. We discovered a…

材料科学 · 物理学 2015-06-11 Jean-Nicolas Longchamp , Conrad Escher , Hans-Werner Fink

Formic acid is a promising liquid hydrogen carrier, but its catalytic decomposition requires both high activity and selectivity toward dehydrogenation. Here, we investigated the catalytic activity and selectivity of formic acid…

材料科学 · 物理学 2025-09-10 Kazuma Sato , Norihito Sakaguchi , Yuji Kunisada

Graphene outstanding properties created a huge interest in the condensed matter community and unprecedented fundings at the international scale in the hope of application developments. Recently, there have been several reports of incomplete…

材料科学 · 物理学 2016-04-20 L. Delfour , A. Davydova , E. Despiau-Pujo , G. Cunge , D. B. Graves , L. Magaud

Interfacing graphene with solid-state devices and maintaining it free of contamination is a crucial step towards a functioning device, be it a semiconductor structure or any other device for technological applications. We take advantage of…

介观与纳米尺度物理 · 物理学 2014-08-27 Jean-Nicolas Longchamp , Conrad Escher , Hans-Werner Fink

Graphene oxide (GO), the functionalized graphene with oxygenated groups (mainly epoxy and hydroxyl), has attracted resurgent interests in the past decade owing to its large surface area, superior physical and chemical properties, and easy…

材料科学 · 物理学 2020-01-14 Xiaoming Huang , Lizhao Liu , Si Zhou , Jijun Zhao

Here we present an overview of recent fundamental studies on the nature of the interaction between individual metal atoms and metal clusters and the conjugated surfaces of graphene and carbon nanotube with a particular focus on the…

材料科学 · 物理学 2014-09-19 Santanu Sarkar , Robert Cort Haddon

Graphene is the physical realization of many fundamental concepts and phenomena in solid state-physics, but in the long list of graphene remarkable properties, a fundamental block is missing: superconductivity. Making graphene…

超导电性 · 物理学 2011-05-20 Gianni Profeta , Matteo Calandra , Francesco Mauri

Graphene oxide (GO) is an important intermediate to prepare graphene and it is also a versatile material with various applications. However, despite its importance, the detailed structure of GO is still unclear. For example, previous…

材料科学 · 物理学 2011-08-08 Ning Lu , Zhenyu Li , Jinlong Yang

Graphene Oxide and reduced Graphene Oxide are intriguing materials for photonics and electronic devices both for intrinsic characteristics and as precursors for the synthesis of graphene. Whatever the application and the engineering…

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