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We develop a fully quantum mechanical methodology to describe the static properties and the dynamics of a single anharmonic vibrational mode interacting with a quantized infrared cavity field in the strong and ultrastrong coupling regimes.…

化学物理 · 物理学 2020-06-22 Johan F. Triana , Federico J. Hernández , Felipe Herrera

Molecular rotation spectra, generated by the coupling of the molecular electric-dipole moments to an external time-dependent electric field, are discussed in a few particular conditions which can be of some experimental interest. First, the…

其他凝聚态物理 · 物理学 2015-12-15 M. Apostol , L. C. Cune

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

原子物理 · 物理学 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe…

量子物理 · 物理学 2013-05-29 Szczepan Chelkowski , André D. Bandrauk

A theoretical framework is presented for the computation of rovibrational polaritonic states of a molecule in a lossless infrared (IR) microcavity. In the proposed approach the quantum treatment of the rotational and vibrational motion of…

化学物理 · 物理学 2023-10-30 Tamás Szidarovszky

We propose an accurate and efficient method to compute vibrational spectra of molecules, based on exact diagonalization of an algebraically calculated matrix based on powers of Morse coordinate. The present work focuses on the 1D potential…

化学物理 · 物理学 2009-11-13 Andrea Bordoni , Nicola Manini

We formulate a theory of nonequilibrium quantum solvation in which parameters of the solvent are explicitly depending on time. We assume in a simplest approach a spherical molecular Onsager cavity with a time-dependent radius. We analyze…

化学物理 · 物理学 2018-05-23 Henning Kirchberg , Peter Nalbach , Michael Thorwart

Molecular vibrational transitions are prime candidates for model-independent searches for variation of the proton-to-electron mass ratio. Searches for present-day variation achieve highest sensitivity with deep molecular potentials. We…

原子物理 · 物理学 2016-11-15 D. Hanneke , R. A. Carollo , D. A. Lane

We give a study of some molecular vibration potentials by solving the D-dimensional Schrodinger equation using the asymptotic iteration method (AIM). The eigenvalue values obtained by the AIM are found to agree with analytic solutions. The…

数学物理 · 物理学 2012-05-07 D. Agboola

When ions move through solids, they interact with the solid's constituent atoms and cause them to vibrate around their equilibrium points. This vibration, in turn, modifies the potential landscape through which the mobile ions travel.…

材料科学 · 物理学 2024-07-03 A. Rodin , B. A. Olsen , A. Ustyuzhanin , A. Maevskiy , K. Noori

Short intense laser pulses are routinely used to induce rotational wave packet dynamics of molecules. Ro-vibrational wave packet dynamics has been explored comparatively infrequently, focusing predominantly on extremely light and rigid…

量子气体 · 物理学 2024-11-12 D. Blume , Q. Guan , J. Kruse , M. Kunitski , R. Doerner

Following excitation by a strong ultra-short laser pulse, molecules develop coordinated rotational motion, exhibiting transient alignment along the direction of the laser electric field, followed by periodic full and fractional revivals…

量子物理 · 物理学 2007-05-23 Sharly Fleischer , Ilya. Sh. Averbukh , Yehiam Prior

The impulsive limit (the "sudden approximation") has been widely employed to describe the interaction between molecules and short, far-off-resonant laser pulses. This approximation assumes that the timescale of the laser--molecule…

化学物理 · 物理学 2023-08-14 Volker Karle , Mikhail Lemeshko

We present an efficient method for modeling the single and double ionization dynamics of the H$_2$ molecule in ultrashort intense laser fields. This method is based on a semi-analytical approach to calculate the time-dependent single and…

量子物理 · 物理学 2025-11-04 Jean-Nicolas Vigneau , Thanh-Tung Nguyen Dang , Eric Charron

Theoretical investigations are presented, and their results are discussed, of the laser acceleration of a single electron by a chirped pulse. Fields of the pulse are modeled by simple plane-wave oscillations and a $\cos^2$ envelope. The…

加速器物理 · 物理学 2015-06-22 Najeh M. Jisrawi , Benjamin J. Galow , Yousef I. Salamin

We demonstrate how dynamic Stark control (DSC) can be achieved on molecular photodissociation in the dipole limit, using single-cycle (FWHM) laser pulses in the terahertz (THz) regime. As the laser-molecule interaction follows the…

化学物理 · 物理学 2020-03-25 A. Tóth , A. Csehi , G. J. Halász , Á. Vibók

Theoretical description of oscillations of electron liquid in large metallic nanospheres (with radius of few tens nm) is formulated within random-phase-approximation semiclassical scheme. Spectrum of plasmons is determined including both…

介观与纳米尺度物理 · 物理学 2015-05-14 W. Jacak , J. Krasnyj , J. Jacak , R. Gonczarek , A. Chepok , L. Jacak , D. Z. Hu , D. Schaadt

We discuss the influence of periodic orbits on the dissociation of a model diatomic molecule driven by a strong bichromatic laser fields. Through the stability of periodic orbits we analyze the dissociation probability when parameters like…

混沌动力学 · 物理学 2009-11-13 S. Huang , C. Chandre , T. Uzer

We study the pair-production process in the presence of two counterpropagating linearly polarized short laser pulses. By means of a nonperturbative technique, we take into account the full coordinate dependence of the external field going…

高能物理 - 唯象学 · 物理学 2017-11-10 I. A. Aleksandrov , G. Plunien , V. M. Shabaev

This is the second article in which we study the rotating Morse potential model for diatomic molecules using the tridiagonal J-matrix approach. Here, we improve further the accuracy of computing the bound states and resonance energies for…

化学物理 · 物理学 2008-10-14 I. Nasser , M. S. Abdelmonem , H. Bahlouli , A. D. Alhaidari