相关论文: Time evolution in the Morse potential using supers…
For non-zero $\ell$ values, we present an analytical solution of the radial Schr\"{o}dinger equation for the rotating Morse potential using the Pekeris approximation within the framework of the Asymptotic Iteration Method. The bound state…
Motivated by the huge need of data for non-equilibrium plasma modeling, a theoretical investigation of dissociative electron attachment to the NO molecule is performed. The calculations presented here are based on the…
We have investigated non-dipole effects in the interaction of a hydrogen atom with elliptically polarized laser pulses of intensity 10$^{14}$ W/cm$^2$ with about 8 fs duration. The study was performed within the framework of a hybrid…
We show here that due to non-adiabatic couplings in decaying systems applying the same time-dependent protocol in the forward and reverse direction to the same mixed initial state leads to different final pure states. In particular, in…
The dependence of the radiative emission and the non-radiative (energy transfer to the metal) relaxation rates of a molecule near a small metal particle on the molecule-to-particle distance and on the molecular orientation is calculated…
We have developed experimental methods for the generation of chirped laser pulses of controlled frequency evolution in the nanosecond pulse length range for coherent atomic interaction studies. The pulses are sliced from the radiation of a…
We have developed and experimentally demonstrated an improved electrostatic deflector for the spatial separation of molecules according to their dipole-moment-to-mass ratio. The device features a very open structure that allows for…
We present some approaches to the computation of ultra-fast laser pulses capable of selectively breaking molecular bonds. The calculations are based on a mixed quantum-classical description: The electrons are treated quantum mechanically…
The dynamics of molecular electron excitation and ionisation is studied in real-time for ultra-short IR laser pulses of intensity I>10^{13} W/cm^{2}. The multi-electron molecule is modeled by a system of two active electrons moving in a…
Dissipative solitons are fundamental wave-pulses that preserve their form in the presence of periodic loss and gain. The canonical realization of dissipative solitons is Kerr-lens mode locking in lasers, which delicately balance nonlinear…
The computation of vibrational spectra of diatomic molecules through the exact diagonalization of algebraically determined matrixes based on powers of Morse coordinates is made substantially more efficient by choosing a properly adapted…
We present a theoretical study of the impact of an electrostatic field combined with nonresonant linearly polarized laser pulses on the rotational dynamics of a thermal ensemble of linear molecules. We solve the time-dependent Schr\"odinger…
We discuss the mechanism by which the inclusion of multielectron polarization improves the solution of the time-dependent Schr\"{o}dinger equation (TDSE) for the oriented CO molecule in a strong external laser pulse within the…
Orientation states of two coupled polar molecules controlled by laser pulses are studied theoretically. By varying the period of a series of periodically applied laser pulse, transition from regular to chaotic behavior may occur. Schmidt…
The vibrational relaxation of NO molecules scattering from an Au(111) surface has served as the focus of efforts to understand nonadiabatic energy transfer at metal-molecule interfaces. Experimental measurements and previous theoretical…
We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…
An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…
We have theoretically investigated the molecular orientation by a asymmetric potential created by the superposition of two-color laser fields. The time-dependent Schrodinger equation is solved numerically for different field parameters. We…
With a specific choice of laser parameters resulting into a so-called exceptional point in the wavelength-intensity plane, it is possible to produce the coalescence of two Floquet resonances describing the photodissociation of the molecule…
A coherent control scheme for the population distribution in the vibrational states of nonpolar molecules is proposed. Our theoretical analysis and results of numerical simulations for the interaction of the hydrogen molecular ion in its…