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We describe a new approach based on semiclassical molecular dynamics that allows to simulate infrared absorption or emission spectra of molecular systems with inclusion of anharmonic intensities. This is achieved from semiclassical power…

化学物理 · 物理学 2018-11-12 Marco Micciarelli , Riccardo Conte , Jaime Suarez , Michele Ceotto

Quantum theory of self-phase and cross-phase modulation of ultrashort light pulses in the Kerr medium is developed with taking into account the response time of an electronic nonlinearity. The correspondent algebra of time-dependent…

量子物理 · 物理学 2007-05-23 F. Popescu , A. S. Chirkin

We made use of supersymmetric (SUSY) quantum mechanics to find a condition under which the Stark effect problem for a polar and polarizable closed-shell diatomic molecule subject to collinear electrostatic and nonresonant radiative fields…

化学物理 · 物理学 2011-06-24 Mikhail Lemeshko , Mustafa Mustafa , Sabre Kais , Bretislav Friedrich

We revisited the electronic structure parameters used to interpret the hyperfine structure of neutral polonium. We used a computational scheme that treats relativistic and high-order electronic correlation effects within the coupled cluster…

原子物理 · 物理学 2024-03-08 Leonid V. Skripnikov , Anatoly E. Barzakh

This paper discusses temporally continuous and discrete forms of the speed-limited particle-in-cell (SLPIC) method first treated by Werner et al. [Phys. Plasmas 25, 123512 (2018)]. The dispersion relation for a 1D1V electrostatic plasma…

等离子体物理 · 物理学 2021-08-31 Thomas G. Jenkins , Gregory R. Werner , John R. Cary

We use an optical centrifuge to excite coherent rotational wave packets in N$_2$O, CS$_2$ and OCS molecules with rotational quantum numbers reaching up to J=465, 690 and 1186, respectively. Time-resolved rotational spectroscopy at such…

化学物理 · 物理学 2017-10-25 A. A. Milner , A. Korobenko , J. W. Hepburn , V. Milner

Nonlinear plasma oscillations in an arbitrary mass ratio cold plasma have been studied using 1-D particle-in-cell simulation. In contrast to earlier work for infinitely massive ion plasmas it has been found that the oscillations phase mix…

等离子体物理 · 物理学 2009-11-06 Sudip Sen Gupta , Predhiman K. Kaw

The response of a MoRe-based superconducting resonator operating near 5 K to pulsed infrared irradiation is investigated, and the underlying physical mechanisms are analyzed. The device exhibits a pronounced nonlinear response dominated by…

A zeptosecond multi--MeV laser pulse may either excite a "plasma" of strongly interacting nucleons or a collective mode. We derive the conditions on laser energy and photon number such that either of these scenarios is realized. We use the…

核理论 · 物理学 2011-05-26 Hans A. Weidenmueller

The real and imaginary parts of the susceptibility are fundamentally associated with the molecular dispersion and absorption, respectively. Measurement of the molecular dispersion has given insight into underlying molecular dynamics such as…

化学物理 · 物理学 2019-01-15 Rachel Glenn

In this paper we develop a method capable of modeling the space-time focusing of nondiffracting pulses. The new pulses can possess arbitrary peak velocities and, in addition to being resistant to diffraction, can have their peak intensities…

光学 · 物理学 2016-10-19 Michel Zamboni-Rached , Ioannis M. Besieris

An understanding of pulsar timing noise offers the potential to improve the timing precision of a large number of pulsars as well as facilitating our understanding of pulsar magnetospheres. For some sources, timing noise is attributable to…

高能天体物理现象 · 物理学 2018-02-07 B. Shaw , B. W. Stappers , P. Weltevrede

In this work, we present analytical solution of Schr\"odinger equation of confined pseudoharmonic potential in presence of a moving boundary condition, for an arbitrary angular momentum state. It turns out that an important quantity to…

量子物理 · 物理学 2025-06-27 Akash Halder , Amlan K. Roy , Debraj Nath

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

原子物理 · 物理学 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

We review some of the few available nonadiabatic calculations of dipole moments. We show that those carried out in a laboratory-fixed set of coordinate axes are bound to fail and discuss the more reasonable ones in a molecule-fixed…

化学物理 · 物理学 2009-09-07 Francisco M. Fernández , Julián Echave

Laser-induced molecular alignment is well understood within the framework of the Born-Oppenheimer (BO) approximation Without the BO approximation, however, the concept of molecular structure is lost, making alignment hard to define…

化学物理 · 物理学 2022-09-16 Ludwik Adamowicz , Simen Kvaal , Caroline Lasser , Thomas Bondo Pedersen

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

化学物理 · 物理学 2018-02-28 E. Gershnabel , I. Sh. Averbukh

We study a nonlinear Schr\"odinger equation which arises as an effective single particle model in X-ray Free Electron Lasers (XFEL). This equation appears as a first-principles model for the beam-matter interactions that would take place in…

We consider deflection of rotating symmetric molecules by inhomogeneous optical and static electric fields, compare results with the case of linear molecules, and find new singularities in the distribution of the scattering angle.…

化学物理 · 物理学 2015-05-28 Erez Gershnabel , Ilya Sh. Averbukh

Atomic and molecular electric dipole moments are calculated within the minimal supersymmetric standard model. Present experiments already provide strong bounds on the combination of phases responsible for the dipole moments of the neutron…

高能物理 - 唯象学 · 物理学 2010-11-01 Willy Fischler , Sonia Paban , Scott Thomas
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