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相关论文: RPA vs. exact shell-model correlation energies

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We calculate the ground-state expectation value of scalar observables in the matrix formulation of the random phase approximation (RPA). Our expression, derived using the quasiboson approximation, is a straightforward generalization of the…

核理论 · 物理学 2009-11-07 Calvin W. Johnson , Ionel Stetcu

The self-consistent random phase approximation (RPA) based on a correlated realistic nucleon-nucleon interaction is used to evaluate correlation energies in closed-shell nuclei beyond the Hartree-Fock level. The relevance of contributions…

核理论 · 物理学 2007-05-23 C. Barbieri , N. Paar , R. Roth , P. Papakonstantinou

The random phase approximation (RPA) to the correlation energy is extended to fractional occupations and its performance examined for exact conditions on fractional charges and fractional spins. RPA satisfies the constancy condition for…

其他凝聚态物理 · 物理学 2009-03-26 Paula Mori-Sánchez , Aron J. Cohen , Weitao Yang

The random phase approximation (RPA) for the electron correlation energy, combined with the exact-exchange energy, represents the state-of-the-art exchange-correlation functional within density-functional theory (DFT). However, the standard…

其他凝聚态物理 · 物理学 2015-05-20 Xinguo Ren , Patrick Rinke , Alexandre Tkatchenko , Matthias Scheffler

The random phase approximation (RPA) for the correlation energy functional of density functional theory has recently attracted renewed interest. Formulated in terms of the Kohn-Sham (KS) orbitals and eigenvalues, it promises to resolve some…

其他凝聚态物理 · 物理学 2009-11-13 Hong Jiang , Eberhard Engel

While the no-core shell model is a state-of-the-art microscopic approach to low-energy nuclear structure, its intense computational requirements lead us to consider time-honored approximations such as the Hartree-Fock (HF) approximation and…

核理论 · 物理学 2007-05-23 Calvin W. Johnson , Ionel Stetcu

We study the correlation energy associated with the pair fluctuations in BCS theory. We use a schematic two-level pairing model and discuss the behavior of the correlation energy across shell closures, including the even-odd differences. It…

核理论 · 物理学 2009-11-06 K. Hagino , G. F. Bertsch

The random-phase approximation (RPA) as an approach for computing the electronic correlation energy is reviewed. After a brief account of its basic concept and historical development, the paper is devoted to the theoretical formulations of…

材料科学 · 物理学 2017-07-26 Xinguo Ren , Patrick Rinke , Christian Joas , Matthias Scheffler

The matrix equations of the random-phase approximation (RPA) are derived for the point-coupling Lagrangian of the relativistic mean-field (RMF) model. Fully consistent RMF plus (quasiparticle) RPA illustrative calculations of the isoscalar…

核理论 · 物理学 2009-11-11 T. Niksic , D. Vretenar , P. Ring

The hole-state random phase approximation (hRPA) and the particle-state random phase approximation (pRPA) for systems like odd $A$ nuclei are discussed. These hRPA and pRPA are formulated based on the Hartree-Fock ground state. An extension…

核理论 · 物理学 2015-06-12 Mitsuru Tohyama , Peter Schuck

The random-phase approximation to the ground state correlation energy (RPA) in combination with exact exchange (EX) has brought Kohn-Sham (KS) density functional theory one step closer towards a universal, "general purpose first principles…

The Hartree-Fock approximation to the many-fermion problem can break exact symmetries, and in some cases by changing a parameter in the interaction one can drive the Hartree-Fock minimum from a symmetry-breaking state to a…

核理论 · 物理学 2009-09-11 Calvin W. Johnson , Ionel Stetcu

We present a method to approximate post-Hartree-Fock correlation energies by using approximate natural orbitals obtained by the random phase approximation (RPA). We demonstrate the method by applying it to the helium atom, the hydrogen and…

化学物理 · 物理学 2021-03-22 Benjamin Ramberger , Zoran Sukurma , Tobias Schäfer , Georg Kresse

We present an analytic proof demonstrating the equivalence between the Random Phase Approximation (RPA) to the ground state correlation energy and a ring-diagram simplification of the Coupled Cluster Doubles (CCD) equations. In the CCD…

其他凝聚态物理 · 物理学 2009-11-13 Gustavo E. Scuseria , Thomas M. Henderson , Danny C. Sorensen

The random phase approximation (RPA) is exact for the exchange energy of a many-electron ground state, but RPA makes the correlation energy too negative by about 0.5 eV/electron. That large short-range error, which tends to cancel out of…

计算物理 · 物理学 2020-06-24 Tim Gould , Adrienn Ruzsinszky , John P. Perdew

Self-consistent correlation potentials for H$_2$ and LiH for various inter-atomic separations are obtained within the random phase approximation (RPA) of density functional theory. The RPA correlation potential shows a peak at the bond…

化学物理 · 物理学 2015-05-30 M. Hellgren , D. R. Rohr , E. K. U. Gross

The Random Phase Approximation (RPA) for total energies has previously been shown to provide a qualitatively correct description of static correlation in molecular systems, where density functional theory (DFT) with local functionals are…

材料科学 · 物理学 2017-09-27 Thomas Olsen

The effects of the correlations in the ground state of $^{16}$O on the octupole and dipole excitations are studied using the extended random phase approximation (ERPA) derived from the time-dependent density-matrix theory. It is found that…

核理论 · 物理学 2015-06-15 Mitsuru Tohyama

In this article, we revisit the question of the validity of Hartree-Fock and random-phase approximations. We show that there is a connection between the two and while the RPA as it is known in much of the physics literature is of limited…

强关联电子 · 物理学 2007-05-23 Girish S. Setlur , Yia-Chung Chang

The random phase approximation (RPA) has received a considerable interest in the field of modeling systems where noncovalent interactions are important. Its advantages over widely used density functional theory (DFT) approximations are the…

化学物理 · 物理学 2019-12-04 Marcin Modrzejewski , Sirous Yourdkhani , Jiri Klimes
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