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相关论文: RPA vs. exact shell-model correlation energies

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The ground state equilibrium properties of copper-gold alloys have been explored with the state of art random phase approximation (RPA). Our estimated lattice constants agree with the experiment within a mean absolute percentage error…

材料科学 · 物理学 2019-07-31 Niraj K. Nepal , Santosh Adhikari , Jefferson E. Bates , Adrienn Ruzsinszky

The ground-state correlation energy calculated in the random-phase approximation (RPA) is known to be identical to that calculated using a subset of terms appearing in coupled-cluster theory with double excitations. In particular, this…

化学物理 · 物理学 2019-04-16 Timothy C. Berkelbach

A fast method is developed for calculating the Random-Phase-Approximation (RPA) correlation energy for density functional theory. The correlation energy is given by a trace over a projected RPA response matrix and the trace is taken by a…

化学物理 · 物理学 2013-01-01 Daniel Neuhauser , Eran Rabani , Roi Baer

The random phase approximation (RPA) is attracting renewed interest as a universal and accurate method for first-principles total energy calculations. The RPA naturally accounts for long-range dispersive forces without compromising accuracy…

材料科学 · 物理学 2013-03-04 Thomas Olsen , Kristian S. Thygesen

We present a real-space method for computing the random phase approximation (RPA) correlation energy within Kohn-Sham density functional theory, leveraging the low-rank nature of the frequency-dependent density response operator. In…

计算物理 · 物理学 2025-04-03 Boqin Zhang , Shikhar Shah , John E. Pask , Edmond Chow , Phanish Suryanarayana

We determine the correlation energy of BN, SiO$_2$ and ice polymorphs employing a recently developed RPAx (random phase approximation with exchange) approach. The RPAx provides larger and more accurate polarizabilities as compared to the…

材料科学 · 物理学 2021-09-22 Maria Hellgren , Lucas Baguet

Recently the damping of the collective charge (and spin) modes of interacting fermions in one spatial dimension was studied. It results from the nonlinear correction to the energy dispersion in the vicinity of the Fermi points. To…

强关联电子 · 物理学 2009-11-13 K. Schönhammer

The RPA long range correlations are known to play a significant role in understanding the depletion of single particle-hole states observed in (e, e') and (e, e'p) measurements. Here the Random Phase Approximation (RPA) theory, implemented…

核理论 · 物理学 2009-11-11 M. Dupuis , S. Karataglidis , E. Bauge , J. P. Delaroche , D. Gogny

We report an improved implementation for evaluating the analytical gradients of the random phase approximation (RPA) electron-correlation energy based on atomic orbitals and the localized resolution of identity scheme. The more efficient…

材料科学 · 物理学 2024-04-17 Muhammad N. Tahir , Honghui Shang , Jia Li , Xinguo Ren

We use the random phase approximation (RPA) method with the singles correlation energy contributions to calculate lattice energies of ten molecular solids. While RPA gives too weak binding, underestimating the reference data by $13.7$\% on…

化学物理 · 物理学 2016-09-21 Jiří Klimeš

We study an extended Lipkin-Meshkov-Glick model that permits a transition to a deformed phase with a broken continuous symmetry. Unlike simpler models, one sees a persistent zero-frequency Goldstone mode past the transition point into the…

核理论 · 物理学 2009-10-31 K. Hagino , G. F. Bertsch

Several approximations are tested by calculating the ground-state energy and the energy of the first excited $0^{+}$ state using an exactly solvable model with two symmetric levels interacting via a pairing force. They are the BCS…

核理论 · 物理学 2009-09-29 Nguyen Dinh Dang

We explore several random phase approximation (RPA) correlation energy variants within the adiabatic-connection fluctuation-dissipation theorem approach. These variants differ in the way the exchange interactions are treated. One of these…

化学物理 · 物理学 2014-04-08 János G. Angyán , Ru-Fen Liu , Julien Toulouse , Georg Jansen

We assess the performance of a recently proposed renormalized adiabatic local density approximation (rALDA) for \textit{ab initio} calculations of electronic correlation energies in solids and molecules. The method is an extension of the…

材料科学 · 物理学 2014-05-30 Thomas Olsen , Kristian S. Thygesen

Random Phase Approximation (RPA) is the theory most commonly used to describe the excitations of many-body systems. In this article, the secular equations of the theory are obtained by using three different approaches: the equation of…

核理论 · 物理学 2023-03-14 Giampaolo Co'

Using the adiabatic connection, we formulate the free energy in terms of the correlation function of a fictitious system, $h_{\lambda}({\bf r},{\bf r}')$, where $\lambda$ determines the interaction strength. To obtain $h_{\lambda}({\bf…

统计力学 · 物理学 2016-06-15 Derek Frydel , Manman Ma

In recent work, generalized gradient approximations (GGA's) have been constructed from the energy density of the Airy gas for exchange but not for correlation. We report the random phase approximation (RPA) conventional correlation energy…

材料科学 · 物理学 2009-06-30 Lucian A. Constantin , Adrienn Ruzsinszky , John P. Perdew

By coupling a doorway state to a see of random background states, we develop the theory of doorway states in the framework of the random-phase approximation (RPA). Because of the symmetry of the RPA equations, that theory is radically…

核理论 · 物理学 2015-06-22 A. De Pace , A. Molinari , H. A. Weidenmueller

The Relativistic Random Phase Approximation (RRPA) is derived from the Time-dependent Relativistic Mean Field (TD RMF) theory in the limit of small amplitude oscillations. In the no-sea approximation of the RMF theory, the RRPA…

核理论 · 物理学 2009-11-07 P. Ring , Zhong-yu Ma , Nguyen Van Giai , D. Vretenar , A. Wandelt , Li-gang Cao

We explore different variants of the random phase approximation (RPA) to the correlation energy derived from closed-shell ring-diagram approximations to coupled cluster doubles theory. We implement these variants in range-separated…

化学物理 · 物理学 2011-09-01 Julien Toulouse , Wuming Zhu , Andreas Savin , Georg Jansen , János G. Angyán