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We investigate Ge mixing at the Si(001) surface and characterize the $2\times N$ Si(001) reconstruction by means of hybrid quantum and molecular mechanics calculations (QM/MM). Avoiding fake elastic dampening, this scheme allows to…

材料科学 · 物理学 2014-10-15 Laurent Karim Béland , Eduardo Machado-Charry , Pascal Pochet , Normand Mousseau

Dimer vacancy (DV) defect complexes in the Si(001)2x1 surface were investigated using high-resolution scanning tunneling microscopy and first principles calculations. We find that under low bias filled-state tunneling conditions, isolated…

The atomic structure, energy of formation, and electronic states of vacancies in H-passivated Ge nanocrystals are studied by density functional theory (DFT) methods. The competition between quantum self-purification and the free surface…

材料科学 · 物理学 2015-05-19 Kenneth Bayus , O. Paz , S. P. Beckman

The structure and properties of vacancies in a 2 nm Si nano-crystal are studied using a real space density functional theory/pseudopotential method. It is observed that a vacancy's electronic properties and energy of formation are directly…

材料科学 · 物理学 2007-10-11 S. P. Beckman , James R. Chelikowsky

We characterized the formation of vacancies at a surface slab model and contrasted the results with the bulk of lead-halide perovskites using cubic and tetragonal CsPbI$_3$ as representative structures. The defect-free CsI-terminated (100)…

材料科学 · 物理学 2024-04-26 Oleg Rubel , Xavier Rocquefelte

We have performed total-energy density-functional calculations using first-principles pseudopotentials to determine the atomic and electronic structure of neutral surface and subsurface vacancies at the GaP(110) surface. The cation as well…

材料科学 · 物理学 2009-10-30 G. Schwarz , A. Kley , J. Neugebauer , M. Scheffler

The initial stages of growth of Ge and Si on the Ge(001) surface are studied and compared to growth on the Si(001) surface. Metastable rows of diluted ad-dimers exist on both surfaces as intermediate stages of epitaxial growth.…

材料科学 · 物理学 2007-05-23 G. Brocks , J. H. Snoeijer , P. J. Kelly , H. J. W. Zandvliet , Bene Poelsema

The scattering potential of the defects on Ge(001) surfaces is investigated by first-principles methods. The standing wave in the spatial map of the local density of states obtained by wave function matching is compared to the image of the…

材料科学 · 物理学 2024-01-09 Tomoya Ono

Experimental observations of heteroepitaxial growth of Ge on Si(001) show a (2xn) reconstruction for sub-monolayer coverages, with dimer rows crossed by missing-dimer trenches. We present first-principles density-functional calculations…

材料科学 · 物理学 2009-11-07 J. Oviedo , D. R. Bowler , M. J. Gillan

First-principles calculations are used to calculate the strain dependencies of the binding and diffusion-activation energies for Ge adatoms on both Si(001) and Ge(001) surfaces. Our calculations reveal that the binding and activation…

统计力学 · 物理学 2009-11-10 A. van de Walle , M. Asta , P. W. Voorhees

Hydrogen segregation to vacancies in the surface and subsurface layers of (111) and (100) surfaces of Pd is studied in the density functional theory (DFT) approach. Adsorption energies and configurations of various clusters of H atoms at…

材料科学 · 物理学 2020-06-24 A. V. Subashiev , H. H. Nee

In this paper we examine the electronic and geometrical structure of impurity-vacancy complexes in Si and Ge. Already Watkins suggested that in Si the pairing of Sn with the vacancy produces a complex with the Sn-atom at the bond center and…

材料科学 · 物理学 2016-08-31 H. Hoehler , N. Atodiresei , K. Schroeder , R. Zeller , P. H. Dederichs

Multi-crystalline silicon is widely used for producing low-cost and high-efficiency solar cells. During crystal growth and device fabrication, silicon solar cells contain grain boundaries (GBs) which are preferential segregation sites for…

材料科学 · 物理学 2020-11-24 Rita Maji , Eleonora Luppi , Nathalie Capron , Elena Degoli

We report differences in adsorption and reaction energetics for ethylene on Si(001) with respect to different dangling bond configurations induced by hydrogen precoverage as obtained via density functional theory calculations. This can help…

化学物理 · 物理学 2016-12-06 Josua Pecher , Gerson Mette , Michael Dürr , Ralf Tonner

The coupling energies between the buckled dimers of the Si(001) surface were determined through analysis of the anisotropic critical behavior of its order-disorder phase transition. Spot profiles in high-resolution low-energy electron…

Grain boundaries (GBs) are defects originating in multi-crystalline silicon during crystal growth for device Si solar cell fabrication. The presence of GBs changes the coordination of Si, making it advantageous for charge carriers to…

材料科学 · 物理学 2022-01-20 Rita Maji , Julia Contreras-García , Nathalie Capron , Elena Degoli , Eleonora Luppi

The stability and formation mechanism of the defects relevant to silicon and carbon vacancies at the 4H-SiC(000$\bar{1}$)/SiO$_2$ interface after wet oxidation are investigated by first-principles calculation based on the density functional…

材料科学 · 物理学 2024-01-09 Mukai Tsunasaki , Tomoya Ono , Mitsuharu Uemoto

Renewed focus on the P-Si system due to its potential application in quantum computing and self-directed growth of molecular wires, has led us to study structural changes induced by P upon placement on Si(001)-$p(2\times 1)$. Using…

材料科学 · 物理学 2009-11-11 Prasenjit Sen , Bikash C Gupta , Inder P. Batra

The formation of framework vacancies in Si- and Ge-based type-I clathrates is studied as function of filling the cages with K and Ba atoms using density-functional theory. Our analysis reveals the relevance of structural disorder, geometric…

The basic properties of point defects (atomic geometry, the position of charge-transfer levels, and formation energies) on the (110) surface of GaAs, GaP, and InP have been calculated employing density-functional theory. Based on these…

材料科学 · 物理学 2007-05-23 G. Schwarz , J. Neugebauer , M. Scheffler
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