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The glass transition can simply be viewed as the point at which the viscosity of a structurally disordered liquid reaches 10^{13} Poise [1]. This definition is operational but it sidesteps fundamental controversies about the glass: Is the…

统计力学 · 物理学 2017-05-10 Ludger Santen , Werner Krauth

The glass transition refers to the non-equilibrium process by which an equilibrium liquid is transformed to a non-equilibrium disordered solid, or vice versa. Associated response functions, such as heat capacities, are markedly different on…

软凝聚态物质 · 物理学 2013-03-26 Aaron S. Keys , Juan P. Garrahan , David Chandler

In this work we numerically investigate a new method for the characterization of growing length scales associated with spatially heterogeneous dynamics of glass-forming liquids. This approach, motivated by the formulation of the…

无序系统与神经网络 · 物理学 2013-10-28 Kang Kim , Shinji Saito , Kunimasa Miyazaki , Giulio Biroli , David R. Reichman

We discuss recent advances in developing a mode-coupling theory of the glass transition (MCT) of two-dimensional systems of active Brownian particles (ABP). We specifically discuss the case of a single ABP tracer in a glass-forming passive…

软凝聚态物质 · 物理学 2020-12-15 Julian Reichert , Leon Granz , Thomas Voigtmann

We discuss a novel approach, the point-to-set correlation functions, that allows to determine relevant static and dynamic length scales in glass-forming liquids. We find that static length scales increase monotonically when the temperature…

无序系统与神经网络 · 物理学 2013-07-04 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

We use event driven simulations to analyze glassy dynamics as a function of density and energy dissipation in a two-dimensional bidisperse granular fluid under stationary conditions. Clear signatures of a glass transition are identified,…

统计力学 · 物理学 2011-10-05 Iraj Gholami , Andrea Fiege , Annette Zippelius

The nature of the glass transition is theoretically understood in the mean-field limit of infinite spatial dimensions, but the problem remains totally open in physical dimensions. Nontrivial finite-dimensional fluctuations are hard to…

统计力学 · 物理学 2019-04-05 Ludovic Berthier , Patrick Charbonneau , Andrea Ninarello , Misaki Ozawa , Sho Yaida

We propose a model to study symmetric binary fluids, based in the mesoscopic molecular simulation technique known as multiparticle collision, where space and state variables are continuous while time is discrete. We include a repulsion rule…

适应与自组织系统 · 物理学 2016-06-22 C. Echeverria , K. Tucci , O. Alvarez-Llamoza , E. E. Orozco-Guillén , M. Morales , M. G. Cosenza

We study the glass and jamming transition of finite-dimensional models of simple liquids: hard- spheres, harmonic spheres and more generally bounded pair potentials that modelize frictionless spheres in interaction. At finite temperature,…

无序系统与神经网络 · 物理学 2013-07-16 Hugo Jacquin

The Random First Order Transition (RFOT) theory of glasses provides a unified framework for explaining the observed correlations of the kinetic and thermodynamic behaviors of glass-forming liquids having a wide variety of chemical…

软凝聚态物质 · 物理学 2025-07-29 M. H. Brown , P. G. Wolynes

An equilibrated model glass-forming liquid is studied by mapping successive configurations produced by molecular dynamics simulation onto a time series of inherent structures (local minima in the potential energy). Using this ``inherent…

软凝聚态物质 · 物理学 2012-03-27 Thomas B. Schroeder , Srikanth Sastry , Jeppe C. Dyre , Sharon C. Glotzer

The viscosity of glass-forming liquids increases by many orders of magnitude if their temperature is lowered by a mere factor of 2-3 [1,2]. Recent studies suggest that this widespread phenomenon is accompanied by spatially heterogeneous…

无序系统与神经网络 · 物理学 2015-05-28 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

We use replica exchange Monte-Carlo simulations to measure the equilibrium equation of state of the disordered fluid state for a binary hard sphere mixture up to very large densities where standard Monte-Carlo simulations do not easily…

统计力学 · 物理学 2011-02-04 Gerardo Odriozola , Ludovic Berthier

The Multiparticle Collision Dynamics technique (MPC) for hydrodynamics simulations is generalized to binary fluid mixtures and multiphase flows, by coupling the particle-based fluid dynamics to a Ginzburg-Landau free-energy functional for…

软凝聚态物质 · 物理学 2024-06-03 Thomas Eisenstecken , Raphael Hornung , Roland G. Winkler , Gerhard Gompper

A simplified nonlinear memory function is proposed in the ideal time-convolutionless mode-coupling theory equation to study the dynamics of glass-forming liquids. The numerical solutions are then compared with the simulation results…

统计力学 · 物理学 2020-01-22 Michio Tokuyama

Dynamical heterogeneities -- strong fluctuations near the glass transition -- are believed to be crucial to explain much of the glass transition phenomenology. One possible hypothesis for their origin is that they emerge from soft…

软凝聚态物质 · 物理学 2012-01-10 Karina E. Avila , Horacio E. Castillo , Azita Parsaeian

A microscopic approach is presented for calculating general properties of interacting Brownian particles under steady shearing. We start from exact expressions for shear-dependent steady-state averages, such as correlation and structure…

软凝聚态物质 · 物理学 2009-07-02 Matthias Fuchs , Michael E. Cates

In this paper we investigate, both analytically and numerically, the emergence of a kinetic glass transition in two different model systems: a uniformly heated granular gas and a molecular fluid with nonlinear drag. Despite the profound…

软凝聚态物质 · 物理学 2024-04-25 A. Patrón , B. Sánchez-Rey , A. Prados

The only available quantitative description of the slowing down of the dynamics upon approaching the glass transition has been, so far, the mode-coupling theory, developed in the 80's by G\"otze and collaborators. The standard derivation of…

统计力学 · 物理学 2012-06-11 Hugo Jacquin , Frédéric Van Wijland

We derive a mode-coupling theory (MCT) to describe the dynamics of tracer particles in dense systems of active Brownian particles (ABPs) in two spatial dimensions. The ABP undergo translational and rotational Brownian dynamics, and are…

软凝聚态物质 · 物理学 2021-11-03 Julian Reichert , Suvendu Mandal , Thomas Voigtmann