English

Spatial correlations in glass-forming liquids across the mode-coupling crossover

Disordered Systems and Neural Networks 2013-07-04 v1

Abstract

We discuss a novel approach, the point-to-set correlation functions, that allows to determine relevant static and dynamic length scales in glass-forming liquids. We find that static length scales increase monotonically when the temperature is lowered, whereas the measured dynamic length scale shows a maximum around the critical temperature of mode-coupling theory. We show that a similar non-monotonicity is found in the temperature evolution of certain finite size effects in the relaxation dynamics. These two independent sets of results demonstrate the existence of a change in the transport mechanism when the glass-former is cooled from moderately to deeply supercooled states across the mode-coupling crossover and clarify the status of the theoretical calculations done at the mean field level.

Keywords

Cite

@article{arxiv.1203.4423,
  title  = {Spatial correlations in glass-forming liquids across the mode-coupling crossover},
  author = {Walter Kob and Sandalo Roldan-Vargas and Ludovic Berthier},
  journal= {arXiv preprint arXiv:1203.4423},
  year   = {2013}
}

Comments

10 pages

R2 v1 2026-06-21T20:37:04.103Z