Linking dynamical heterogeneity to static amorphous order
Abstract
Glass-forming liquids grow dramatically sluggish upon cooling. This slowdown has long been thought to be accompanied by a growing correlation length. Characteristic dynamical and static length scales, however, have been observed to grow at different rates, which perplexes the relationship between the two and with the slowdown. Here, we show the existence of a direct link between dynamical sluggishness and static point-to-set correlations, holding at the local level as we probe different environments within a liquid. This link, which is stronger and more general than that observed with locally preferred structures, suggests the existence of an intimate relationship between structure and dynamics in a broader range of glass-forming liquids than previously thought.
Keywords
Cite
@article{arxiv.1309.5085,
title = {Linking dynamical heterogeneity to static amorphous order},
author = {Patrick Charbonneau and Ethan Dyer and Jaehoon Lee and Sho Yaida},
journal= {arXiv preprint arXiv:1309.5085},
year = {2016}
}
Comments
8 pages, 3 figures; v4: one cavity data point (T=0.51, R=3.2) added. Data relevant to this work can be accessed at http://dx.doi.org/10.7924/G8VD6WC5