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Solving the time-dependent Schr\"odinger equation (TDSE) is pivotal for modeling non-adiabatic electron dynamics, a key process in ultrafast spectroscopy and laser-matter interactions. However, exact solutions to the TDSE remain…

化学物理 · 物理学 2025-12-29 Bizi Huang , Weizhong Fu , Ji Chen

We derive a new time-dependent Schr\"odinger equation(TDSE) for quantum models with non-hermitian Hamiltonian. Within our theory, the TDSE is symmetric in the two Hilbert spaces spanned by the left and the right eigenstates, respectively.…

量子物理 · 物理学 2017-02-24 Ye Xiong , Peiqing Tong

In this work we present the theoretical framework for the solution of the time-dependent Schr\"{o}dinger equation (TDSE) of atomic and molecular systems under strong electromagnetic fields with the configuration space of the electron's…

原子物理 · 物理学 2009-11-13 L. A. A. Nikolopoulos , J. S. Parker , K. T. Taylor

We show that the time-dependent Schr\"odinger equation (TDSE) is the phenomenological dynamical law of evolution unraveled in the classical limit from a timeless formulation in terms of probability amplitudes conditioned by the values of…

量子物理 · 物理学 2015-06-04 Julio César Arce

The time-dependent Schrodinger equation (TDSE) is usually treated in real space in the textbook. However, it makes the numerical simulations of strong-field processes difficult due to the wide dispersion and fast oscillation of the electron…

原子物理 · 物理学 2020-01-20 Yan Xu , Xue-Bin Bian

A global solution of the Schr\"odinger equation for explicitly time-dependent Hamiltonians is derived by integrating the non-linear differential equation associated with the time-dependent wave operator. A fast iterative solution method is…

量子物理 · 物理学 2015-05-18 Arnaud Leclerc , Georges Jolicard

We present a wave-function based method to solve the time-dependent many-electron Schr\"odinger equation (TDSE) with special emphasis on strong-field ionization phenomena. The theory builds on the configuration-interaction (CI) approach…

量子物理 · 物理学 2014-12-11 Sebastian Bauch , Lasse Kragh Sørensen , Lars Bojer Madsen

Understanding the real-time evolution of many-electron quantum systems is essential for studying dynamical properties in condensed matter, quantum chemistry, and complex materials, yet it poses a significant theoretical and computational…

强关联电子 · 物理学 2024-11-07 Jannes Nys , Gabriel Pescia , Alessandro Sinibaldi , Giuseppe Carleo

We present a stochastic method for solving the time-dependent Schr\"odinger equation, generalizing a ground-state full configuration interaction Quantum Monte Carlo method. By performing the time-integration in the complex plane close to…

强关联电子 · 物理学 2018-08-08 Kai Guther , Werner Dobrautz , Olle Gunnarsson , Ali Alavi

The Finite-Difference Time-Domain (FDTD) method is a well-known technique for the analysis of quantum devices. It solves a discretized Schrodinger equation in an explicitly iterative process. However, the method requires the spatial grid…

量子物理 · 物理学 2012-12-05 Frederick Ira Moxley , Weizhong Dai

A method of solving the time-dependent Schr\"odinger equation is presented, in which a finite region of space is treated explicitly, with the boundary conditions for matching the wave-functions on to the rest of the system replaced by an…

材料科学 · 物理学 2009-11-13 J. E. Inglesfield

A detailed exposition of highly efficient and accurate method for the propagation of the time-dependent Schr\"odinger equation is presented. The method is readily generalized to solve an arbitrary set of ODE's. The propagation is based on a…

量子物理 · 物理学 2017-05-12 Ido Schaefer , Hillel Tal-Ezer , Ronnie Kosloff

Quantum theory has been remarkably successful in providing an understanding of physical systems at foundational scales. Solving the Schr\"odinger equation provides full knowledge of all dynamical quantities of the physical system. However…

量子物理 · 物理学 2020-11-24 Cesar Lema , Anna Choromanska

The linear Schr\"odinger equation with piecewise constant potential in one spatial dimension is a well-studied textbook problem. It is one of only a few solvable models in quantum mechanics and shares many qualitative features with…

偏微分方程分析 · 数学 2018-07-02 Natalie E Sheils , Bernard Deconinck

We describe the time-dependent restricted-active-space self-consistent-field (TD-RASSCF) method for a system of interacting bosons. We provide the theory of the method and discuss its numerical implementation. The method provides a general…

量子物理 · 物理学 2017-04-28 Camille Lévêque , Lars Bojer Madsen

The time-dependent Schrodinger equation is solved for two model problems for a non-Hermitian quantum system.A simple matrix model system is used to examine two critical problems for these systems: complex and non-observable energies and…

量子物理 · 物理学 2024-12-11 Brian L Burrows

We address the problem of identifying the (nonstationary) quantum systems that admit supersymmetric dynamical invariants. In particular, we give a general expression for the bosonic and fermionic partner Hamiltonians. Due to the…

量子物理 · 物理学 2009-11-07 Ali Mostafazadeh

We describe a parallel algorithm for solving the time-independent 3d Schrodinger equation using the finite difference time domain (FDTD) method. We introduce an optimized parallelization scheme that reduces communication overhead between…

量子物理 · 物理学 2014-11-18 Michael Strickland , David Yager-Elorriaga

We approximate the solution for the time dependent Schr\"odinger equation (TDSE) in two steps. We first use a pseudo-spectral collocation method that uses samples of functions on rank-1 or rank-r lattice points with unitary Fourier…

数值分析 · 数学 2020-07-01 Yuya Suzuki , Gowri Suryanarayana , Dirk Nuyens

A strategy is developed for writing the time-dependent Schr\"{o}dinger Equation (TDSE), and more generally the Dyson Series, as a convolution equation using recursive Fourier transforms, thereby decoupling the second-order integral from the…

量子物理 · 物理学 2024-06-27 Sky Nelson-Isaacs
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