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Very recently, a new type of two-dimensional layered material MoSi2N4 has been fabricated, which is semiconducting with weak interlayer interaction, high strength, and excellent stability. We systematically investigate theoretically the…

材料科学 · 物理学 2021-02-24 Hongxia Zhong , Wenqi Xiong , Pengfei Lv , Jin Yu , Shengjun Yuan

Stacking two-dimensional (2D) van der Waals materials with different interlayer atomic registry in a heterobilayer causes the formation of a long-range periodic superlattice that may bestow the heterostructure with exotic properties such as…

Interlayer rotation and stacking were recently demonstrated as effective strategies for tuning physical properties of various two-dimensional materials. The latter strategy was mostly realized in hetero-structures with continuously varied…

In search of an improved strategy to form low resistance contacts to MoS2 and related semiconducting transition metal dichalcogenides, we use ab initio density functional electronic structure calculations in order to determine the…

介观与纳米尺度物理 · 物理学 2019-05-03 Zhibin Gao , Zhixian Zhou , David Tomanek

Employing density functional theory-based methods, we investigate monolayer and bilayer structures of hexagonal SnS$_{2}$, which is recently synthesized monolayer metal dichalcogenide. Comparison of 1H and 1T phases of monolayer SnS$_{2}$…

介观与纳米尺度物理 · 物理学 2016-03-14 C. Bacaksiz , S. Cahangirov , A. Rubio , R. T. Senger , F. M. Peeters , H. Sahin

Bilayer (BL) molybdenum disulfide (MoS$_2$) is one of the most important electronic structures not only in valleytronics but also in realizing twistronic systems on the basis of the topological mosaics in Moir\'e superlattices. In this…

材料科学 · 物理学 2023-04-17 Xingjia Cheng , Wen Xu , Hua Wen , Jing Zhang , Heng Zhang , Haowen Li , Qingqing Chen

The creation of moir\'e superlattices in twisted bilayers of two-dimensional crystals has been utilised to engineer quantum material properties in graphene and transition metal dichalcogenide (TMD) semiconductors. Here, we examine the…

介观与纳米尺度物理 · 物理学 2024-05-27 J. G. McHugh , V. V. Enaldiev , V. I. Fal'ko

The emergence of transition metal dichalcogenides (TMDs) as 2D electronic materials has stimulated proposals of novel electronic and photonic devices based on TMD heterostructures. Here we report the determination of band offsets in TMD…

We introduce a generalizable, physics informed strategy for generating training data that enables a machine learning force field accurate over a broad range of twist angles and stacking layer numbers in moire systems. Applying this to…

材料科学 · 物理学 2025-11-26 Yueyao Fan , Xiao-Wei Zhang , Yusen Ye , Xiaoyu Liu , Chong Wang , Kaijie Yang , Di Xiao , Ting Cao

Transition metal dichalcogenides (TMDs) are a branch of two-dimensional materials which in addition to having an easy-to-exfoliate layered structure, also host semiconducting, metallic, superconducting, and topological properties in various…

超导电性 · 物理学 2023-01-25 Suvodeep Paul , Saswata Talukdar , Ravi Shankar Singh , Surajit Saha

Twistronic van der Waals heterostrutures offer exciting opportunities for engineering optoelectronic properties of nanomaterials. Here, we use multiscale modeling to study trapping of charge carriers and excitons by ferroelectric…

介观与纳米尺度物理 · 物理学 2021-03-23 V. V. Enaldiev , F. Ferreira , S. J. Magorrian , V. I. Fal'ko

Moir\'{e} interference effects have profound impact on the optoelectronic properties of vertical van der Waals structures. Here we establish secondary electron imaging in a scanning electron microscope as a powerful technique for…

介观与纳米尺度物理 · 物理学 2023-06-27 Anna Rupp , Jonas Göser , Zhijie Li , Ismail Bilgin , Anvar Baimuratov , Alexander Högele

Twisted bilayer (t-BL) transition metal dichalcogenides (TMDCs) attracted considerable attention in recent years due to their distinctive electronic properties, which arise due to the moire superlattices that lead to the emergence of flat…

The electronic structure of semiconducting 2D materials such as transition metal dichalcogenides (TMDs) is known to be tunable by its environment, from simple external fields applied with electrical contacts up to complex van der Waals…

Motivated by the recent experimental realization of twisted transition metal dichalcogenide bilayers, we study a simplified model driven by different forms of monochromatic light. As a concrete and representative example we use parameters…

介观与纳米尺度物理 · 物理学 2021-02-01 Michael Vogl , Martin Rodriguez-Vega , Benedetta Flebus , Allan H. MacDonald , Gregory A. Fiete

We study in-plane lateral heterostructures of commensurate transition-metal dichalcogenides, such as MoS$_{2}$-WS$_{2}$ and MoSe$_{2}$-WSe$_{2}$, and find interfacial and edge states that are highly localized to these regions of the…

介观与纳米尺度物理 · 物理学 2019-01-04 Oscar Ávalos-Ovando , Diego Mastrogiuseppe , Sergio E. Ulloa

In bilayers of two-dimensional (2D) semiconductors with stacking arrangements which lack inversion symmetry charge transfer between the layers due to layer-asymmetric interband hybridisation can generate a potential difference between the…

介观与纳米尺度物理 · 物理学 2021-07-01 F. Ferreira , V. V. Enaldiev , V. I. Fal'ko , S. J. Magorrian

Twisted van der Waals bilayers provide an ideal platform to study the electron correlation in solids. Of particular interest is the 30 degree twisted bilayer honeycomb lattice system, which possesses an incommensurate moire pattern and…

材料科学 · 物理学 2021-03-02 Yu-Hao Shen , Wen-Yi Tong , He Hu , Jun-Ding Zheng , Chun-Gang Duan

Moir\'e superlattices serve as a playground for emerging phenomena, such as localization of band states, superconductivity, and localization of excitons. These superlattices are large and are often modeled in the zero angle limit, which…

材料科学 · 物理学 2022-06-01 Christopher Linderälv , Joakim Hagel , Samuel Brem , Ermin Malic , Paul Erhart

Optical and electrical properties of two-dimensional transition metal dichalcogenides (TMDCs) grown by chemical vapor deposition (CVD) are strongly determined by their microstructure. Consequently, the visualization of spatial structural…