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The use of semiconductor nanocrystals in scalable quantum technologies requires characterization of the exciton coherence dynamics in an \emph{ensemble} of electronically isolated crystals in which system-bath interactions are nevertheless…

We have studied emission properties of high-density excitons in single-walled carbon nanotubes through nonlinear photoluminescence excitation spectroscopy. As the excitation intensity was increased, all emission peaks arising from different…

介观与纳米尺度物理 · 物理学 2009-11-13 Y. Murakami , J. Kono

We systematically study the coupling of longitudinal modes (shells) in a carbon nanotube quantum dot. Inelastic cotunneling spectroscopy is used to probe the excitation spectrum in parallel, perpendicular and rotating magnetic fields. The…

介观与纳米尺度物理 · 物理学 2019-01-23 M. C. Hels , T. S. Jespersen , J. Nygård , K. Grove-Rasmussen

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…

化学物理 · 物理学 2020-11-18 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

Self-assembled supramolecular aggregates are excellent candidates for the design of efficient excitation transport devices. Both artificially prepared and natural photosynthetic aggregates in plants and bacteria present an important degree…

量子物理 · 物理学 2017-09-04 Alejandro D. Somoza , Ke-Wei Sun , Rafael A. Molina , Yang Zhao

The interplay of the non-equivalent corners in the Brillouin zone of transition metal dichalcogenides have been investigated extensively. While experimental and theoretical works contributed to a detailed understanding of the relaxation of…

介观与纳米尺度物理 · 物理学 2023-10-13 Malte Selig , Dominik Christiansen , Manuel Katzer , Mariana V. Ballottin , Peter C. M. Christianen , Andreas Knorr

Intense few-to-sub-femtosecond soft x-ray pulses can produce neutral, two-site excited double-core-hole states by promoting two core electrons to the same unoccupied molecular orbital. We theoretically investigate double nitrogen K-edge…

化学物理 · 物理学 2023-06-28 Adam E. A. Fouda , Dimitris Koulentianos , Linda Young , Gilles Doumy , Phay J. Ho

Transient extreme ultraviolet (XUV) spectroscopy probes core level transitions to unoccupied valence and conduction band states. Uncertainty remains to what degree the core-hole created by the XUV transition modifies the measurement of…

In this work, we have simulated the processes of broadening the first exciton band in optical absorption spectra (OA) for InP/ZnS ensembles of colloidal quantum dots (QDs). A phenomenological model has been proposed that takes into account…

材料科学 · 物理学 2019-08-05 Sergey S. Savchenko , Ilya A. Weinstein

The excitonic occupancy state of a single, nanowire-based, heterostructure quantum dot is dynamically programmed by a surface acoustic wave. The quantum dot is formed by an interface or thickness fluctuation of a GaAs QW embedded in a…

We use a configuration interaction approach within the envelope function approximation to study the nature of the excitonic resonance in nano-hybrids, composite nanoparticles (NPs) combining a semiconducting and a metallic segment in…

介观与纳米尺度物理 · 物理学 2011-07-25 Juan I. Climente , Jose L. Movilla , Guido Goldoni , Josep Planelles

We use the macroscopic quantum electrodynamics approach suitable for absorbing and dispersing media to study the properties and role of collective surface excitations --- excitons and plasmons --- in single-wall and double-wall carbon…

介观与纳米尺度物理 · 物理学 2017-08-14 I. V. Bondarev , L. M. Woods , A. Popescu

We study the band-edge exciton fine structure and in particular its bright-dark splitting in colloidal semiconductor nanocrystals by four different optical methods based on fluorescence line narrowing and time-resolved measurements at…

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

Current-induced self-sustained magnetization oscillations in spin-torque nano-oscillators (STNOs) are promising candidates for ultra-agile microwave sources or detectors. While usually STNOs behave as a monochrome source, we report here…

介观与纳米尺度物理 · 物理学 2022-10-19 A. Hamadeh , D. Slobodianiuk , R. Moukhader , G. Melkov , V. Borynskyi , M. Mohseni , G. Finocchio , V. Lomakin , R. Verba , G. de Loubens , P. Pirro , O. Klein

We studied the nonlinear time-resolved luminescence signals due to multiexciton recombination processes in single-walled carbon nanotubes (SWNTs) using femtosecond excitation correlation (FEC) spectroscopy. From theoretical analysis of the…

材料科学 · 物理学 2015-05-13 Yuhei Miyauchi , Kazunari Matsuda , Yoshihiko Kanemitsu

The measurement and manipulation of the coherent dynamics of excitonic states constitute a forefront research challenge in semiconductor optics and in quantum coherence-based protocols for optoelectronic technologies. Layered semiconductors…

Scanning probe microscopy (SPM) has been extensively applied to probe interfacial water in many interdisciplinary fields but the disturbance of the probes on the hydrogen-bonding structure of water has remained an intractable problem. Here…