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Exciton-phonon coupling limits the homogeneous emission linewidth of nanocrystals. Hence, a full understanding of it is crucial. In this work, we statistically investigate exciton-phonon coupling by performing single-particle spectroscopy…

An overview on photon echo spectroscopy under resonant excitation of the exciton complexes in semiconductor nanostructures is presented. The use of four-wave-mixing technique with the pulsed excitation and heterodyne detection allowed us to…

介观与纳米尺度物理 · 物理学 2018-08-29 S. V. Poltavtsev , I. A. Yugova , I. A. Akimov D. R. Yakovlev , M. Bayer

The surprising recent observation of highly emissive triplet-states in lead halide perovskites accounts for their orders-of-magnitude brighter optical signals and high quantum efficiencies compared to other semiconductors. This makes them…

The properties of nucleus-acoustic (NA) solitary waves (SWs) and double layers (DLs) in a four-component magnetized degenerate quantum plasma system (containing non-degenerate inertial light nuclei, both non-relativistically and…

等离子体物理 · 物理学 2017-07-19 B. Hosen. M. G. Shah , M. R. Hossen , A. A. Mamun

In this work, Pt-Ti core-shell nanoparticles (NP) of 2 nm to 3 nm in size and 30000 u \pm 1500 u as specified single particle mass, deposited on flat silicon substrates by means of a mass-selected cluster beam source, were used for the…

Excitons in 2D material bubbles-nanoscale deformations in atomically thin materials, typically exhibiting a dome-like shape-are confined by the strain effect, exhibiting extraordinary emission properties, such as single photon generation,…

Exciton condensation, characterized by uniform phase coherence across macroscopic length scales, has enabled the discovery of a variety of excitonic states, greatly enriching our understanding of correlated many-body physics. More exotic…

强关联电子 · 物理学 2026-03-31 Deguang Wu , Yiran Xue , Baigeng Wang , Rui Wang , D. Y. Xing

The lack of available table-top extreme ultraviolet (XUV) sources with high enough fluxes and coherence properties have limited the availability of nonlinear XUV and x-ray spectroscopies to free electron lasers (FEL). Here, we demonstrate…

Understanding and controlling microscopic dynamics across spatial and temporal scales has driven major progress in science and technology over the past several decades. While ultrafast laser-based techniques have enabled probing nanoscale…

Hybrid plasmonic devices involve a nanostructured metal supporting localized surface plasmons to amplify light-matter interaction, and a non-plasmonic material to functionalize charge excitations. Application-relevant epitaxial…

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

化学物理 · 物理学 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

Through molecular dynamics simulations considering thermal vibration of surface atoms, ionic behaviors in concentrated NaCl solutions confined between discretely charged silicon surfaces have been investigated. The electric double layer…

化学物理 · 物理学 2017-04-06 Yinghua Qiu , Jian Ma , Yunfei Chen

Few-layer tungsten diselenide (WSe2) is investigated using circularly polarized Raman spectroscopy with up to eight excitation energies. The main E2g1 and A1g modes near 250 cm-1 appear as a single peak in the Raman spectrum taken without…

介观与纳米尺度物理 · 物理学 2019-06-11 Sanghun Kim , Kangwon Kim , Jae-Ung Lee , Hyeonsik Cheong

Excitons are bosonic quasiparticles with a variety of applications in optoelectronics, photosyn thesis, and dissipationless informatics, and their lifetime can become sufficiently long to form a quantum condensate. While exciton…

We perform two-dimensional coherent spectroscopy on CdSe/CdZnS core/shell colloidal quantum dots at cryogenic temperatures. In the two-dimensonal spectra, sidebands due to electronic coupling with CdSe lattice LO-phonon modes are observed…

材料科学 · 物理学 2019-08-16 A. Liu , D. B. Almeida , W. K. Bae , L. A. Padilha , S. T. Cundiff

We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe…

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

原子物理 · 物理学 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

We present a detailed investigation of the near-field optical response of core-shell nanoparticles using Fourier-demodulated full-wave simulations, revealing significant modifications to established contrast mechanisms in scattering-type…

We conduct systematic studies of the optical characteristics of plasmonic nanoparticles that exhibit C2v symmetry. We analyze three distinct geometric configurations: an L-type shape, a crescent, and a split-ring resonator. Optical…

光学 · 物理学 2024-05-24 Michael R. Clark , Syed A. Shah , Andrei Piryatinski , Maxim Sukharev

F\"orster Resonant Energy Transfer (FRET)-mediated exciton diffusion through artificial nanoscale building block assemblies could be used as a new optoelectronic design element to transport energy. However, so far nanocrystal (NC) systems…