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Monolayers of semiconducting transition metal dichalcogenides are two-dimensional direct-gap systems which host tightly-bound excitons with an internal degree of freedom corresponding to the valley of the constituting carriers. Strong…

Single layers of transition metal dichalcogenides are two-dimensional direct bandgap semiconductors with degenerate, but inequivalent, `valleys' in the electronic structure that can be selectively excited by polarized light. Coherent…

The band structure of transition metal dichalcogenides (TMDCs) with valence band edges at different locations in the momentum space could be harnessed to build devices that operate relying on the valley degree of freedom. To realize such…

介观与纳米尺度物理 · 物理学 2016-09-06 Oriol Lopez Sanchez , Dmitry Ovchinnikov , Shikhar Misra , Adrien Allain , Andras Kis

Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a…

介观与纳米尺度物理 · 物理学 2015-06-22 Grant Aivazian , Zhirui Gong , Aaron M Jones , Rui-Lin Chu , Jiaqiang Yan , David G Mandrus , Chuanwei Zhang , David Cobden , Wang Yao , Xiaodong Xu

Modern electronic devices heavily rely on the accurate control of charge and spin of electrons. The emergence of controllable valley degree of freedom brings new possibilities and presents a promising prospect towards valleytronics.…

A monolayer of a transition metal dichalcogenide (TMD) such as WSe$_2$ is a two-dimensional (2D) direct band-gap valley-semiconductor having an effective Honeycomb lattice structure with broken inversion symmetry. The inequivalent valleys…

介观与纳米尺度物理 · 物理学 2015-06-22 Ajit Srivastava , Meinrad Sidler , Adrien V. Allain , Dominik S. Lembke , Andras Kis , Atac Imamoglu

Interlayer valley excitons in bilayer MoS2 feature concurrently large oscillator strength and long lifetime, and hence represent an advantageous scenario for valleytronic applications. However, control of valley pseudospin of interlayer…

Preserving a high degree of valley polarization of excitons in photo-excited transition-metal dichalcogenide monolayers (TMD-MLs) is desirable for the valley-based photonic applications, but widely recognized as a hard task hindered by the…

介观与纳米尺度物理 · 物理学 2020-10-13 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

Monolayer semiconducting transition metal dichalcogenides possess broken inversion symmetry and strong spin-orbit coupling, which leads to unique spin-valley locking effect. In 2H stacked pristine multilayers, the spin-valley locking yields…

介观与纳米尺度物理 · 物理学 2023-06-07 Yinong Zhang , Chengxin Xiao , Dmitry Ovchinnikov , Jiayi Zhu , Xi Wang , Takashi Taniguchi , Kenji Watanabe , Jiaqiang Yan , Wang Yao , Xiaodong Xu

Monolayer group-VIB transition metal dichalcogenides have recently emerged as a new class of semiconductors in the two-dimensional limit. The attractive properties include: the visible range direct band gap ideal for exploring…

介观与纳米尺度物理 · 物理学 2015-07-30 Hongyi Yu , Xiaodong Cui , Xiaodong Xu , Wang Yao

The valley degree of freedom in atomically thin transition-metal dichalcogenides provides a natural binary index for information processing. Exciton-polaritons formed under strong light-matter coupling offer a promising route to overcome…

介观与纳米尺度物理 · 物理学 2026-01-23 Xingzhou Chen , Yuanjun Guan , Areg Ghazaryan , Shiran Sun , Lingxiao Yu , Ruitao Lv , Artem Volosniev , Zheng Sun , Jian Wu

Excitons, composite electron-hole quasiparticles, are known to play an important role in optoelectronic phenomena in many semiconducting materials. Recent experiments and theory indicate that the band-gap optics of the newly discovered…

介观与纳米尺度物理 · 物理学 2015-09-02 Yuri N. Gartstein , Xiao Li , Chuanwei Zhang

We investigate with polarized microphotoluminescence the optical pumping of the valley degree of freedom in charge-tunable MoS2 monolayers encapsulated with hexagonal boron nitride at cryogenic temperatures. We report a large steady state…

介观与纳米尺度物理 · 物理学 2021-10-15 Sangjun Park , Steve Arscott , Takashi Taniguchi , Kenji Watanabe , Fausto Sirotti , Fabian Cadiz

The emerging field of valleytronics aims to exploit the valley pseudospin of electrons residing near Bloch band extrema as an information carrier. Recent experiments demonstrating optical generation and manipulation of exciton valley…

介观与纳米尺度物理 · 物理学 2017-05-24 Kai Hao , Lixiang Xu , Fengcheng Wu , Philipp Nagler , Kha Tran , Xin Ma , Christian Schüller , Tobias Korn , Allan H. MacDonald , Galan Moody , Xiaoqin Li

Increasing the speed limits of conventional electronics requires innovative approaches to manipulate other quantum properties of electrons besides their charge. An alternative approach utilizes the valley degree of freedom in…

介观与纳米尺度物理 · 物理学 2023-03-29 A. O. Slobodeniuk , P. Koutenský , M. Bartoš , F. Trojánek , P. Malý , T. Novotný , M. Kozák

In monolayer Transition Metal Dichalcogenides (TMDs) the valence and conduction bands are spin split because of the strong spin-orbit interaction. In tungsten-based TMDs the spin-ordering of the conduction band is such that the so-called…

Due to degeneracies arising from crystal symmetries, it is possible for electron states at band edges ("valleys") to have additional spin-like quantum numbers. An important question is whether coherent manipulation can be performed on such…

Strong spin-orbit coupling and inversion symmetry breaking in transition metal dichalcogenide monolayers yield the intriguing effects of valley-dependent optical selection rules. As such, it is possible to substantially polarize valley…

Zeeman effect induced by the magnetic field introduces a splitting between the two valleys at K$^+$ and K$^-$ points of the Brillouin zone in monolayer semiconducting transition metal dichalcogenides. In consequence, the photoluminescence…

介观与纳米尺度物理 · 物理学 2020-12-30 Tomasz Smoleński , Tomasz Kazimierczuk , Mateusz Goryca , Karol Nogajewski , Marek Potemski , Piotr Kossacki

Photonic bound states in the continuum (BICs) have emerged as a versatile tool for enhancing light-matter interactions by strongly confining light fields. Chiral BICs are photonic resonances with a high degree of circular polarisation,…