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DNAs charge transfer and self-assembly characteristics have made it a hallmark of molecular electronics for the past two decades. A fast and efficient charge transfer mechanism with programmable properties using DNA nanostructures is…

材料科学 · 物理学 2023-07-05 Busra Demir , Hashem Mohammad , M. P. Anantram , Ersin Emre Oren

Various charge migration mechanisms in the DNA are studied within the framework of the Peyrard-Bishop-Holstein model which has been widely used to address charge dynamics in this macromolecule. To analyze these mechanisms we consider…

生物物理 · 物理学 2022-09-14 R. P. A. Lima , A. V. Malyshev

In solution, DNA is a highly charged macromolecule which bears a unit of negative charge on each phosphate of its sugar-phosphate backbone. Although partially compensated by counterions adsorbed at or condensed near it, DNA still produces a…

软凝聚态物质 · 物理学 2024-03-11 Jonathan G. Hedley , Kush Coshic , Aleksei Aksimentiev , Alexei A. Kornyshev

Charge transfer in a DNA duplex chain is studied by constructing a system with virtual electrodes connected at the ends of each DNA strand. The systeym is described by the tight-binding model and its transport is analyzed by the transfer…

介观与纳米尺度物理 · 物理学 2009-11-11 X. F. Wang , Tapash Chakraborty

Charge migration along DNA molecules has attracted scientific interest for over half a century. Reports on possible high rates of charge transfer between donor and acceptor through the DNA, obtained in the last decade from solution…

材料科学 · 物理学 2009-11-10 Danny Porath , Gianaurelio Cuniberti , Rosa Di Felice

We consider voltage-driving DNA translocation through a nanopore in the present study. By assuming the DNA is coaxial with the cylindrical nanopore, a hydrodynamic model for determining effective force on a single DNA molecule in a nanopore…

软凝聚态物质 · 物理学 2013-06-19 Wen-Yue Tang , Guo-Hui Hu

A versatile approach to modeling the conformations and energetics of DNA loops is presented. The model is based on the classical theory of elasticity, modified to describe the intrinsic twist and curvature of DNA, the DNA bending…

生物物理 · 物理学 2007-05-23 Alexander Balaeff , L. Mahadevan , Klaus Schulten

Long range charge transfer experiments in DNA oligomers and the subsequently measured -- and very diverse -- transport response of DNA wires in solid state experiments exemplifies the need for a thorough theoretical understanding of charge…

基因组学 · 定量生物学 2015-05-13 G. Cuniberti , E. Macia , A. Rodriguez , R. A. Römer

The electrical properties of DNA molecules are investigated by charge injection and electric force microscopy experiments. Prior to injection, DNA molecules exhibit a weak positively charged state. We probe the electrical behaviour of DNA…

材料科学 · 物理学 2009-11-10 Thomas Heim , Thierry Melin , Dominique Deresmes , Dominique Vuillaume

A statistical model of homopolymer DNA, coupling internal base pair states (unbroken or broken) and external thermal chain fluctuations, is exactly solved using transfer kernel techniques. The dependence on temperature and DNA length of the…

软凝聚态物质 · 物理学 2007-08-29 J. Palmeri , M. Manghi , N. Destainville

We discuss various measures of net charge (conserved quantities) fluctuations proposed for the identification of critical phenomena in heavy ion collisions. We show the dynamical component of fluctuations of the net charge can be expressed…

核实验 · 物理学 2009-11-07 C. Pruneau , S. Gavin , S. Voloshin

We investigate diffusion-limited reactions between a diffusing particle and a target site on a semiflexible polymer, a key factor determining the kinetics of DNA-protein binding and polymerization of cytoskeletal filaments. Our theory…

软凝聚态物质 · 物理学 2010-12-08 Yann von Hansen , Roland R. Netz , Michael Hinczewski

The temperature dependence of DNA flexibility is studied in the presence of stretching and unzipping forces. Two classes of models are considered. In one case the origin of elasticity is entropic due to the polymeric correlations, and in…

软凝聚态物质 · 物理学 2016-06-27 Tanmoy Pal , Somendra M. Bhattacharjee

In this short note, a correction is made to the recently proposed solution [1] to a 1D biased diffusion model for linear DNA translocation and a new analysis will be given to the data in [1]. It was pointed out [2] by us recently that this…

软凝聚态物质 · 物理学 2013-08-23 Daniel Y. Ling , X. S. Ling

A class of nucleosome remodeling motors translocate nucleosomes, to which they are attached, toward the middle of DNA chain in the presence of ATP during in vitro experiments. Such a biological activity is likely based on a physical…

生物物理 · 物理学 2016-05-23 Kuni H. Iwasa , Ana Maria Florescu

We investigate quantum transport characteristics of a ladder model, which effectively mimics the topology of a double-stranded DNA molecule. We consider the interaction of tunneling charges with a selected internal vibrational degree of…

软凝聚态物质 · 物理学 2007-05-23 R. Gutierrez , S. Mohapatra , H. Cohen , D. Porath , G. Cuniberti

The lack of molecular-level understanding for the electronic excitation response of DNA to charged particle radiation, such as high-energy protons, remains a fundamental scientific bottleneck in advancing proton and other ion beam cancer…

软凝聚态物质 · 物理学 2023-03-17 Christopher Shepard , Dillon Yost , Yosuke Kanai

Grafting linkers with open ends of complementary single-stranded DNA makes a flexible tool to tune interactions between colloids,which facilitates the design of complex self-assembly structures. Recently, it has been proposed to coat…

软凝聚态物质 · 物理学 2018-01-31 Hao Hu , Pablo Sampedro Ruiz , Ran Ni

We present a low-temperature experimental test of the fluctuation theorem for electron transport through a double quantum dot. The rare entropy-consuming system trajectories are detected in the form of single charges flowing against the…

介观与纳米尺度物理 · 物理学 2012-01-20 B. Küng , C. Rössler , M. Beck , M. Marthaler , D. S. Golubev , Y. Utsumi , T. Ihn , K. Ensslin

The role of thermal pressure fluctuations in the ejection of tightly packaged DNA from protein capsid shells is discussed in a model calculation. At equilibrium before ejection we assume the DNA is folded many times into a bundle of…

介观与纳米尺度物理 · 物理学 2010-09-20 Michael J. Harrison