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相关论文: Analytic Evaluation of two-electron Atomic Integra…

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Some typical kinetic energy integrals which arise in the application of extended Hylleraas-configuration interaction (E-Hy-CI) function in the framework of Rayleigh-Ritz method of variation, have been evaluated analytically for two-electron…

原子物理 · 物理学 2018-02-01 B Padhy

An improved algorithm to evaluate the nonrelativistic three-electron Hylleraas-Configuration Interaction (Hy-CI) kinetic energy integrals over Slater orbitals and the Hamiltonian in Hylleraas coordinates is shown. The resulting analytical…

原子物理 · 物理学 2016-01-29 Maria Belen Ruiz

In this paper we consider calculation of two-centre exchange integrals over Slater-type orbitals (STOs). We apply the Neumann expansion of the Coulomb interaction potential and consider calculation of all basic quantities which appear in…

量子物理 · 物理学 2016-11-04 Michał Lesiuk , Robert Moszynski

In this paper, which constitutes the first part of the series, we consider calculation of two-centre Coulomb and hybrid integrals over Slater-type orbitals (STOs). General formulae for these integrals are derived with no restrictions on the…

量子物理 · 物理学 2015-01-09 Michał Lesiuk , Robert Moszynski

We present a general methodology to evaluate matrix elements of the effective core potentials (ECPs) within one-electron basis set of Slater-type orbitals (STOs). The scheme is based on translation of individual STO distributions in the…

化学物理 · 物理学 2017-05-17 Michal Lesiuk , Aleksandra M. Tucholska , Robert Moszynski

In this work we propose a novel composite method for accurate calculation of the energies of many-electron atoms. The dominant contribution to the energy (pair energies) are calculated by using explicitly correlated factorisable coupled…

原子物理 · 物理学 2018-12-12 Michal Przybytek , Michal Lesiuk

Hylleraas-Configuration Interaction (Hy-CI) calculations on the ground $1^1$S state of helium atom are presented using s-, p-, d-, and f-Slater orbitals of both real and complex form. Techniques of construction of adapted configurations,…

原子物理 · 物理学 2016-01-29 Maria Belen Ruiz

In this study, using the analytical and recurrence relations suggested by the authors in previous works, the new efficient and reliable program procedure for the overlap integrals over Slater type orbitals (STOs) is presented. The proposed…

化学物理 · 物理学 2015-05-13 I. I. Guseinov , B. A. Mamedov

Various properties of the general two-center two-electron integral over the explicitly correlated exponential function are analyzed for the potential use in high precision calculations for diatomic molecules. A compact one dimensional…

化学物理 · 物理学 2015-06-11 Krzysztof Pachucki

Extensive variational computations are reported for the ground state energy of the non-relativistic two-electron atom. Several different sets of basis functions were systematically explored, starting with the original scheme of Hylleraas.…

原子物理 · 物理学 2009-11-07 Charles Schwartz

New sets of functions with arbitrary large finite cardinality are constructed for two-electron atoms. Functions from these sets exactly satisfy the Kato's cusp conditions. The new functions are special linear combinations of Hylleraas-…

原子物理 · 物理学 2020-01-08 A. T. Kruppa , J. Kovács , I. Hornyak

We give a detailed account of an $\it{ab}$ $\it{initio}$ spectral approach for the calculation of energy spectra of two active electron atoms in a system of hyperspherical coordinates. In this system of coordinates, the Hamiltonian has the…

The total energies of twenty eight bound S-, P-, D-, F-, G-, H-, and I-states in the three-electron systems Li atom and Be+ ion, respectively, are determined with the use of the Configuration Interaction (CI) with Slater orbitals and L-S…

原子物理 · 物理学 2013-08-09 Maria Belen Ruiz , Johannes T. Margraf , Alexei M. Frolov

A closed form expression for the three-electron Hylleraas integral involving the inverse quadratic power of one inter-particle coordinate is obtained, and recursion relations are derived for positive powers of other coordinates. This result…

原子物理 · 物理学 2009-11-11 K. Pachucki , M. Puchalski

A simple method is outlined for analytic evaluation of the basic 2-electron atomic integral with integrand containing products of atomic s-type Slater orbitals and exponentially correlated function of the form $r_{ij}…

原子物理 · 物理学 2016-09-02 Bholanath Padhy

We derive direct single-stage numerical evaluation of the electronic overlap integral between arbitrary atomic orbitals (including STOs). Integration is over cartesian co-ordinates, and replaces previous sums over 'special' functions. The…

化学物理 · 物理学 2016-04-21 Michael J Caola

We present analytical formulas for the calculation of the two-center two-electron integrals in the basis of Slater geminals and products of Slater orbitals. Our derivation starts with establishing a inhomogeneous fourth-order ordinary…

量子物理 · 物理学 2012-12-07 Michał Lesiuk , Robert Moszynski

In this paper methods for calculations of multi-center integrals of squared Coulomb potentials and Slater-type orbitals (STO) are derived. These integrals are necessary for accurate lower bounds to energy levels of molecular systems. All…

化学物理 · 物理学 2022-02-10 Sohei Ashida

For general two-electron two-centre integrals over Slater-type orbitals (STOs), the use of the Neumann expansion for the Coulomb interaction potential yields infinite series in terms of few basic functions. In many important cases the…

量子物理 · 物理学 2017-02-08 Michal Lesiuk

The method of evaluation outlined in a previous work has been utilized here to evaluate certain other three- electron and four- electron atomic integrals involving s Slater-type orbitals and exponential correlation with unlinked $r_{ij}$'s.…

原子物理 · 物理学 2017-01-23 B Padhy
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