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We give a detailed account of an $\it{ab}$ $\it{initio}$ spectral approach for the calculation of energy spectra of two active electron atoms in a system of hyperspherical coordinates. In this system of coordinates, the Hamiltonian has the…

The two-electron self-energy contribution to the ground state energy of heliumlike ions is calculated both for a point nucleus and an extended nucleus in a wide interval of Z. All the two-electron contributions are compiled to obtain most…

原子物理 · 物理学 2009-10-30 V. A. Yerokhin , A. N. Artemyev , V. M. Shabaev

The correlation energies of various atoms in their excited-states are estimated by modelling the Coulomb hole following the previous work by Chakravorty and Clementi. The parameter in the model is fixed by making the corresponding Coulomb…

化学物理 · 物理学 2014-09-23 M. Hemanadhan , Manoj K. Harbola

We study the ground-state correlation energy $E_{\rm c}$ of two electrons of opposite spin confined within a $D$-dimensional ball ($D \ge 2$) of radius $R$. In the high-density regime, we report accurate results for the exact and restricted…

其他凝聚态物理 · 物理学 2010-08-17 Pierre-François Loos , Peter M. W. Gill

We have simultaneously measured angular distributions and electronic energy loss of helium ions and protons directly transmitted through self-supporting, single-crystalline silicon foils. We have compared the energy loss along channelled…

材料科学 · 物理学 2020-03-11 Svenja Lohmann , Daniel Primetzhofer

The present work studies aspects of the electronic correlation in confined H$^{-}$, He and Li$^+$ atoms in their ground states using the informational entropies. In this way, different variational wavefunctions are employed in order of…

原子物理 · 物理学 2021-06-10 Wallas S. Nascimento , Marcos M. de Almeida , Frederico V. Prudente

We study the correlation energy, the effective anisotropy parameter, and quantum fluctuations of the pseudospin magnetization in bilayer quantum Hall systems at total filling factor nu=1 by means of exact diagonalizations of the Hamiltonian…

介观与纳米尺度物理 · 物理学 2009-11-07 John Schliemann

We investigate the effect of dynamic electron correlation on high-harmonic generation in helium atoms using intense visible light (\lambda=390nm). Two complementary approaches are used which account for correlation in an approximate manner:…

量子物理 · 物理学 2009-05-21 G. A. McKenna , R. Nepstad , J. F. McCann , D. Dundas

We present a fully {\it ab initio}, non-perturbative, time-dependent approach to describe single and double ionization of helium by proton and antiproton impact. A flexible and accurate finite-element discrete-variable-representation is…

原子物理 · 物理学 2016-11-17 Xiaoxu Guan , Klaus Bartschat

A rapid and relatively simple scheme of calculation is elaborated and applied to cosmological recombination of helium. Employing the nonrelativistic Coulomb Green's function, a wavefunction of a colliding electron is represented in an…

宇宙学与河外天体物理 · 物理学 2022-09-13 Tamaz Kereselidze , Zaal Machavariani , Irakli Noselidze

An alternative multipole expansion of the correlation term is derived. Modified spherical Bessel type functions which simplify as a summation of multiple orders of basic trigonometric functions are generated from this new method. We use…

量子物理 · 物理学 2017-04-10 Eric Ouma Jobunga

We explore ground-state entanglement properties of helium atom confined at the center of an impenetrable spherical cavity of varying radius by using explicitly correlated Hylleraas-type basis set. Results for the dependencies of the von…

量子物理 · 物理学 2017-07-17 Przemyslaw Koscik , Jayanta K. Saha

Iglesias et al. (2002) showed that the Rayleigh scattering from helium atoms decreases by collective effects in the atmospheres of cool white dwarf stars. Their study is here extended to consider an accurate evaluation of the atomic…

太阳与恒星天体物理 · 物理学 2017-10-25 René D. Rohrmann

We present an efficient \textit{ab initio} method for calculating the electronic structure and total energy of strongly correlated electron systems. The method extends the traditional Gutzwiller approximation for one-particle operators to…

强关联电子 · 物理学 2014-07-01 Y. X. Yao , J. Liu , C. Liu , W. C. Lu , C. Z. Wang , K. M. Ho

The independent atom ansatz of density functional theory yields an accurate analytical expression for dynamic correlation energy in the H$_{2}$ molecule: $E_{c} = 0.5(1 - \sqrt{2})(ab|ba)$ for the atom-additive self-consistent density $\rho…

化学物理 · 物理学 2024-05-28 Alanna 'Lanie' Leung , Alexander V. Mironenko

The technique of quantum electrodynamics (QED) calculations of energy levels in the helium atom is reviewed. The calculations start with the solution of the Schr\"odinger equation and account for relativistic and QED effects by perturbation…

原子物理 · 物理学 2021-07-14 Vladimir A. Yerokhin , Vojtech Patkos , Krzysztof Pachucki

The non-relativistic interacting electron gas in an external field of positively charged massive cores is dealt with in the scheme of second quantization. Ladder operators that change between stationary states of contiguous energy…

量子物理 · 物理学 2025-02-27 Miguel Lagos

In quantum chemistry calculations, the correlation energy is defined as the difference between the Hartree-Fock limit energy and the exact solution of the nonrelativistic Schrodinger equation. With this definition, the electron correlation…

量子物理 · 物理学 2009-11-11 Zhen Huang , Sabre Kais

Extensive variational computations are reported for the ground state energy of the non-relativistic two-electron atom. Several different sets of basis functions were systematically explored, starting with the original scheme of Hylleraas.…

原子物理 · 物理学 2009-11-07 Charles Schwartz

We review our recent progress in the determination of the high-density correlation energy $\Ec$ in two-electron systems. Several two-electron systems are considered, such as the well known helium-like ions (helium), and the Hooke's law atom…

化学物理 · 物理学 2011-01-14 Pierre-François Loos , Peter M. W. Gill