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Computational feasibility of turbulent reacting flows hinges on the reduction of large chemical kinetics systems to smaller more manageable reaction sets. Recently, several sophisticated reduction techniques have been developed but they…

化学物理 · 物理学 2012-02-17 Sharath Girimaji , Ashraf Ibrahim

Quasi steady state assumptions are often used to simplify complex systems of ordinary differential equations in modelling of biochemical processes. The simplified system is designed to have the same qualitative properties as the original…

动力系统 · 数学 2013-12-11 Tomáš Vejchodský

We discuss parameter dependent polynomial ordinary differential equations that model chemical reaction networks. By classical quasi-steady state (QSS) reduction we understand the following familiar heuristic: Set the rate of change for…

经典分析与常微分方程 · 数学 2022-09-20 Alexandra Goeke , Sebastian Walcher , Eva Zerz

In this paper we derive several quasi steady-state approximations (QSSAs) to the stochastic reaction network describing the Michaelis-Menten enzyme kinetics. We show how the different assumptions about chemical species abundance and…

分子网络 · 定量生物学 2017-11-09 Hye-Won Kang , Wasiur R. KhudaBukhsh , Heinz Koeppl , Grzegorz A. Rempała

There are many mathematical models of biochemical cell signaling pathways that contain a large number of elements (species and reactions). This is sometimes a big issue for identifying critical model elements and describing the model…

分子网络 · 定量生物学 2021-09-15 Hemn Mohammed Rasool , Sarbaz H. A. Khoshnaw

The quasi-steady-state assumption (QSSA) is an approximation that is widely used in chemistry and chemical engineering to simplify reaction mechanisms. The key step in the method requires a solution by radicals of a system of multivariate…

动力系统 · 数学 2025-05-16 Ophelia Adams

Stochastic models for biochemical reaction networks are widely used to explore their complex dynamics but face significant challenges, including difficulties in determining rate constants and high computational costs. To address these…

分子网络 · 定量生物学 2025-03-04 Yun Min Song , Kangmin Lee , Jae Kyoung Kim

Quasi-steady state (QSS) reduction is a commonly used method to lower the dimension of a differential equation model of a chemical reaction network. From a mathematical perspective, QSS reduction is generally interpreted as a special type…

动力系统 · 数学 2019-08-30 Elisenda Feliu , Christian Lax , Sebastian Walcher , Carsten Wiuf

Efficient analysis and simulation of multiscale stochastic systems of chemical kinetics is an ongoing area for research, and is the source of many theoretical and computational challenges. In this paper, we present a significant improvement…

数值分析 · 数学 2016-09-21 Simon Cotter

Partial equilibrium approximation (PEA) and quasi-steady-state approximation (QSSA) are two classical methods for reducing complex macroscopic chemical reactions into simple computable ones. Previous studies mainly focus on the accuracy of…

化学物理 · 物理学 2023-08-15 Liangrong Peng , Liu Hong

In biochemical networks, reactions often occur on disparate timescales and can be characterized as either "fast" or "slow." The quasi-steady state approximation (QSSA) utilizes timescale separation to project models of biochemical networks…

分子网络 · 定量生物学 2015-06-19 Jae Kyoung Kim , Krešimir Josić , Matthew R. Bennett

The quasi-steady state assumption (QSSA) forms the basis for rigorous mathematical justification of the Michaelis-Menten formalism commonly used in modeling a broad range of intracellular phenomena. A critical supposition of QSSA-based…

定量方法 · 定量生物学 2011-03-08 Ed Reznik , Daniel Segre , William Erik Sherwood

The quasi-steady-state approximation (or stochastic averaging principle) is a useful tool in the study of multiscale stochastic systems, giving a practical method by which to reduce the number of degrees of freedom in a model. The method is…

化学物理 · 物理学 2015-06-18 Maria Bruna , S. Jonathan Chapman , Matthew J. Smith

The Quasi Steady-State (QSS) model of long-term dynamics relies on the idea of time-scale decomposition. Assuming that the fast variables are infinitely fast and are stable in the long-term, the QSS model replaces the differential equations…

系统与控制 · 计算机科学 2013-10-02 Xiaozhe Wang , Hsiao-Dong Chiang

For a theoretical understanding of the reactivity of complex chemical systems, relative energies of stationary points on potential energy hypersurfaces need to be calculated to high accuracy. Due to the large number of intermediates present…

化学物理 · 物理学 2018-10-30 Gregor N. Simm , Markus Reiher

Delay differential equations are used as a model when the effect of past states has to be taken into account. In this work we consider delay models of chemical reaction networks with mass action kinetics. We obtain a sufficient condition…

动力系统 · 数学 2020-06-05 Gheorghe Craciun , Maya Mincheva , Casian Pantea , Polly Y. Yu

We study, from a purely quantitative point of view, the quasi-steady-state assumption for the fundamental mathematical model of the general enzymatic reaction: we re-establish, on a rigorous basis, certain already known results and we…

动力系统 · 数学 2021-10-01 Vasiliki Bitsouni , Nikolaos Gialelis , Ioannis G. Stratis

The Quasi-Steady State Approximation (QSSA) can be an effective tool for reducing the size and stiffness of chemical mechanisms for implementation in computational reacting flow solvers. However, for many applications, stiffness remains,…

The methods of quantum chemistry and solid state theory to solve the many-body problem are reviewed. We start with the definitions of reduced density matrices, their properties (contraction sum rules, spectral resolutions, cumulant…

强关联电子 · 物理学 2007-05-23 P. Ziesche , F. Tasnadi

The paper has two goals: It presents basic ideas, notions, and methods for reduction of reaction kinetics models: quasi-steady-state, quasi-equilibrium, slow invariant manifolds, and limiting steps. It describes briefly the current state of…

化学物理 · 物理学 2022-05-17 A. N. Gorban
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