化学振荡器通过相分离的时空组织
软凝聚态物质
2025-07-23 v1 斑图形成与孤子
生物物理
摘要
We study chemical oscillators in the presence of phase separation. By imposing timescale separation between slow reactions and fast diffusion, we define a dynamics at phase equilibrium for the relevant degrees of freedom. We demonstrate that phase separation affects reaction kinetics by localizing reactants within phases, allowing for control of oscillator frequency and amplitude. The analysis is validated with a spatial model. Finally, relaxing the timescale separation between reactions and diffusion leads to waves of phase equilibria at mesoscopic scales.
引用
@article{arxiv.2507.16030,
title = {Spatiotemporal organization of chemical oscillators via phase separation},
author = {Jonathan Bauermann and Giacomo Bartolucci and Artemy Kolchinsky},
journal= {arXiv preprint arXiv:2507.16030},
year = {2025}
}