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As approaching the glass transition, particle motion in liquids becomes highly heterogeneous and regions with virtually no mobility coexist with liquid-like domains. This complex dynamics is believed to be responsible for different…

软凝聚态物质 · 物理学 2018-03-28 F. Puosi , N. Jakse , A. Pasturel

We numerically obtain the first quantitative demonstration that development of spatial correlations of mobility as temperature is lowered is responsible for the ``decoupling'' of transport properties of supercooled liquids. This result…

统计力学 · 物理学 2009-11-10 Ludovic Berthier

We develop a replicated liquid theory for structural glasses which exhibit spatial variation of physical quantities along one axis, say $z$-axis. The theory becomes exact with infinite transverse dimension $d-1 \to \infty$. It provides an…

软凝聚态物质 · 物理学 2025-11-14 Yukihiro Tomita , Hajime Yoshino

We present a calculation of a fourth-order, time-dependent density correlation function that measures higher-order spatiotemporall correlations of the density of a liquid. From molecular dynamics simulations of a glass-forming Lennard-Jones…

统计力学 · 物理学 2009-11-07 N. Lacevic , F. W. Starr , T. B. Schroder , V. N. Novikov , S. C. Glotzer

Using positional data from video-microscopy of a two-dimensional colloidal system and from simulations of hard discs we determine the wave-vector-dependent normal mode spring constants in the supercooled fluid and glassy state,…

软凝聚态物质 · 物理学 2012-10-26 Christian L. Klix , Florian Ebert , Fabian Weysser , Matthias Fuchs , Georg Maret , Peter Keim

Existence and growth of amorphous order in supercooled liquids approaching glass transition is a subject of intense research. Even after decades of work, there is still no clear consensus on the molecular mechanisms that lead to a rapid…

统计力学 · 物理学 2023-03-14 Rajsekhar Das , Saurish Chakrabarty , Smarajit Karmakar

We study theoretically the non-linear response properties of glass formers. We establish several general results which, together with the assumption of Time-Temperature Superposition, lead to a relation between the non-linear response and…

统计力学 · 物理学 2009-12-19 Marco Tarzia , Giulio Biroli , Jean-Philippe Bouchaud , Alexandre Lefèvre

We discuss the growth process of a crystalline phase out of a metastable over-compressed liquid that is brought into contact with a crystalline substrate. The process is modeled by means of molecular dynamics. The particles interact via the…

软凝聚态物质 · 物理学 2014-08-07 Francesco Turci , Tanja Schilling

Self- and cross-correlation dynamics of deeply supercooled liquids were recently identified using photon correlation spectroscopy and spin relaxometry on the one hand, and using dielectric investigations on the other. These results fueled a…

软凝聚态物质 · 物理学 2021-03-09 K. Moch , P. Münzner , R. Böhmer , C. Gainaru

Glasses are out-of-equilibrium systems aging under the crystallization threat. During ordinary glass formation, the atomic diffusion slows down rendering its experimental investigation impractically long, to the extent that a timescale…

无序系统与神经网络 · 物理学 2015-08-28 E. A. A. Pogna , C. Rodríguez-Tinoco , G. Cerullo , C. Ferrante , J. Rodríguez-Viejo , T. Scopigno

We study the distribution of overlaps of glassy minima, taking proper care of residual symmetries of the system. Ensembles of locally stable, low lying glassy states are efficiently generated by rapid cooling from the liquid phase which has…

软凝聚态物质 · 物理学 2009-10-31 K. K. Bhattacharya , K. Broderix , R. Kree , A. Zippelius

We study theoretically and numerically a family of multi-point dynamic susceptibilities that quantify the strength and characteristic lengthscales of dynamic heterogeneities in glass-forming materials. We use general theoretical arguments…

We discuss a novel approach, the point-to-set correlation functions, that allows to determine relevant static and dynamic length scales in glass-forming liquids. We find that static length scales increase monotonically when the temperature…

无序系统与神经网络 · 物理学 2013-07-04 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

I briefly review a recent series of papers putting forward a coarse-grained theoretical approach to the physics of supercooled liquids approaching their glass transition. After a suitable coarse-graining, the dynamics of the liquid is…

统计力学 · 物理学 2009-11-10 Ludovic Berthier

We analyze a simple dynamical model of glasses, based on the idea that each particle is trapped in a local potential well, which itself evolves due to hopping of neighbouring particles. The glass transition is signalled by the fact that the…

凝聚态物理 · 物理学 2009-10-28 Jean-Philippe Bouchaud , Alain Comtet , Cécile Monthus

Using molecular dynamics computer simulations we investigate how the glass transition and the properties of the resulting glass depend on the cooling rate with which the sample has been quenched. This is done by studying a two component…

凝聚态物理 · 物理学 2009-10-28 Katharina Vollmayr , Walter Kob , Kurt Binder

Based on experimental evidences we present a phenomenological description of the thermal glass transition as a dynamical phase transition. Different susceptibilities calculated on the basis of this description are in good qualitative…

无序系统与神经网络 · 物理学 2016-08-16 J. K. Krüger , J. Petersson , J. Baller , M. Henkel

The glass transition, extensively studied in dense fluids, polymers, or colloids, corresponds to a dramatic evolution of equilibrium transport coefficients upon a modest change of control parameter, like temperature or pressure. A similar…

统计力学 · 物理学 2013-05-06 Ludovic Berthier , Jorge Kurchan

We use event driven simulations to analyze glassy dynamics as a function of density and energy dissipation in a two-dimensional bidisperse granular fluid under stationary conditions. Clear signatures of a glass transition are identified,…

统计力学 · 物理学 2011-10-05 Iraj Gholami , Andrea Fiege , Annette Zippelius

In this note we revisit the Kovacs effect, concerning the way in which the volume of a glass-forming liquid, which has been driven out of equilibrium, changes with time while the system evolves towards a metastable state. The theoret- ical…

软凝聚态物质 · 物理学 2017-11-16 F. Aliotta , R. C. Ponterio , F. Saija , P. V. Giaquinta