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Recently, we have proposed a new dynamic line on the phase diagram in the supercritical region. Crossing this line corresponds to the radical changes of the fluid properties. Here, we focus on the dynamics of model Lennard-Jones and…

软凝聚态物质 · 物理学 2015-06-16 V. V. Brazhkin , Yu. D. Fomin , A. G. Lyapin , V. N. Ryzhov , E. N. Tsiok , Kostya Trachenko

We identify the pattern of microscopic dynamical relaxation for a two dimensional glass forming liquid. On short timescales, bursts of irreversible particle motion, called cage jumps, aggregate into clusters. On larger time scales, clusters…

软凝聚态物质 · 物理学 2010-10-04 R. Candelier , A. Widmer-Cooper , J. K. Kummerfeld , O. Dauchot , G. Biroli , P. Harrowell , D. R. Reichman

The interrelation of dynamic processes active on separated time-scales in glasses and viscous liquids is investigated using a model displaying two time-scale bifurcations both between fast and secondary relaxation and between secondary and…

无序系统与神经网络 · 物理学 2015-03-19 Andrea Crisanti , Luca Leuzzi , Matteo Paoluzzi

We consider the stationary state of a fluid comprised of inelastic hard spheres or disks under the influence of a random, momentum-conserving external force. Starting from the microscopic description of the dynamics, we derive a nonlinear…

统计力学 · 物理学 2013-02-25 W. T. Kranz , M. Sperl , A. Zippelius

The relationship between the microscopic arrangement of molecules in a supercooled liquid and its slow dynamics at low temperature near glass transition is studied by Molecular Dynamics (MD) simulations. A Lennard-Jones liquid with…

软凝聚态物质 · 物理学 2009-11-13 Sneha Elizabeth Abraham , Biman Bagchi

A kinetic Monte Carlo (KMC) method is used to study the structural properties and dynamics of a supercooled binary Lennard-Jones liquid around the glass transition temperature. This technique permits us to explore the potential energy…

软凝聚态物质 · 物理学 2015-06-24 Javier Hernandez-Rojas , David J. Wales

We use computer simulations to study the microscopic dynamics of an athermal assembly of soft particles near the fluid-to-solid, jamming transition. Borrowing tools developed to study dynamic heterogeneity near glass transitions, we…

材料科学 · 物理学 2010-06-24 Claus Heussinger , Ludovic Berthier , Jean-Louis Barrat

The overlap, or similarity, between liquid configurations is at the core of the mean-field description of the glass transition, and remains a useful concept when studying three-dimensional glass-forming liquids. In liquids, however, the…

统计力学 · 物理学 2021-01-05 Benjamin Guiselin , Gilles Tarjus , Ludovic Berthier

We present a quantitative study of strain correlations in quiescent supercooled liquids and glasses. Recent two-dimensional computer simulations and experiments indicate that even supercooled liquids exhibit long-lived, long-range strain…

We introduce a new and robust approach for characterizing spatially and temporally heterogeneous behavior within a system based on the evolution of dynamic fuctuations once averaged over different space lengths and time scales. We apply it…

无序系统与神经网络 · 物理学 2018-07-04 J. Ariel Rodriguez Fris , Eric R. Weeks , Francesco Sciortino , Gustavo A. Appignanesi

Recently a new approach to the determination of dynamic correlation lengths, {\xi}, for supercooled liquids, based on the properties of the slow (picosecond) vibrational dynamics, was carried out [L. Hong, V.N. Novikov, and A.P. Sokolov,…

软凝聚态物质 · 物理学 2015-05-30 D. Fragiadakis , R. Casalini , C. M. Roland

In supercooled liquids, at a temperature between the glass transition temperature Tg and the melting point Tm, thermodynamic properties remain continuous, while dynamic behavior exhibits anomalies. The origin of such thermodynamics-dynamic…

软凝聚态物质 · 物理学 2025-06-17 X. R. Tian , D. M. Zhang , B. Zhang , D. Y. Sun , X. G. Gong

Building on the recently derived inhomogeneous mode-coupling theory, we extend the generalised mode-coupling theory of supercooled liquids to inhomogeneous environments. This provides a first-principles-based, systematic and rigorous way of…

Granular simulations are used to probe the particle scale dynamics at short, intermediate, and long time scales for gravity driven, dense granular flows down an inclined plane. On approach to the angle of repose, where motion ceases, the…

软凝聚态物质 · 物理学 2009-11-11 L. E. Silbert

Understanding the mechanical properties of glasses remains elusive since the glass transition itself is not fully understood, even in well studied examples of glass formers in two dimensions. In this context we demonstrate here: (i) a…

We examine the phenomenon of dynamical heterogeneity in computer simulations of an equilibrium, glass-forming liquid. We describe several approaches to quantify the spatial correlation of single-particle motion, and show that spatial…

软凝聚态物质 · 物理学 2009-09-25 Sharon C. Glotzer , Claudio Donati

The dynamical behavior of a kind of models with hierarchically constrained dynamics is investigated. The models exhibit many properties resembling real structural glasses. In particular, we focus on the study of time-dependent temperature…

统计力学 · 物理学 2009-11-07 A. Prados , J. J. Brey

The dynamical glass transition is typically taken to be the temperature at which a glassy liquid is no longer able to equilibrate on experimental timescales. Consequently, the physical properties of these systems just above or below the…

软凝聚态物质 · 物理学 2017-03-08 Samuel S. Schoenholz , Ekin D. Cubuk , Efthimios Kaxiras , Andrea J. Liu

A relation between equilibrium, steady-state, and waiting-time dependent dynamical two-time correlation functions in dense glass-forming liquids subject to homogeneous steady shear flow is discussed. The systems under study show pronounced…

软凝聚态物质 · 物理学 2015-05-18 Matthias Krüger , Fabian Weysser , Thomas Voigtmann

Over times shorter than that required for relaxation of enthalpy, a liquid can exhibit striking heterogeneities. The picture of these heterogeneities is complex with transient patches of rigidity, irregular yet persistent, intersected by…

软凝聚态物质 · 物理学 2010-09-30 Peter Harrowell