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The correlation between the fast cage dynamics and structural relaxation is investigated in a model polymer system. It is shown that the cage vibration amplitude, as expressed by the Debye-Waller factor, and the relaxation time…

流体动力学 · 物理学 2009-09-01 A. Ottochian , C. De Michele , D. Leporini

We have studied the conformational and scaling behaviors of a flexible dendrimer immersed in athermal or good solvents. A self-consistent field theory combined with a pre-averaged excluded volume potential representing the two-body…

软凝聚态物质 · 物理学 2018-08-30 Meng Shi , Yingzi Yang , Feng Qiu

It is commonly accepted that in concentrated solutions or melts high-molecular weight polymers display random-walk conformational properties without long-range correlations between subsequent bonds. This absence of memory means, for…

软凝聚态物质 · 物理学 2009-11-11 J. P. Wittmer , P. Beckrich , F. Crevel , C. C. Huang , A. Cavallo , T. Kreer , H. Meyer

The scaling of the bond-bond correlation function $C(s)$ along linear polymer chains is investigated with respect to the curvilinear distance, $s$, along the flexible chain and the monomer density, $\rho$, via Monte Carlo and molecular…

软凝聚态物质 · 物理学 2009-11-10 J. P. Wittmer , H. Meyer , J. Baschnagel , A. Johner , S. Obukhov , L. Mattioni , M. Mueller , A. N. Semenov

Dynamic density functionals (DDFs) are popular tools for studying the dynamical evolution of inhomogeneous polymer systems. Here, we present a systematic evaluation of a set of diffusive DDF theories by comparing their predictions with data…

软凝聚态物质 · 物理学 2018-02-07 Shuanhu Qi , Friederike Schmid

We study effects of fluctuations on the mesoscopic length-scale on systems with mesoscopic inhomogeneities. Equations for the correlation function and for the average volume fraction are derived in the self-consistent Gaussian…

软凝聚态物质 · 物理学 2016-05-25 A. Ciach , W. T. Gozdz

We consider the properties of a self-avoiding polymer chain, adsorbed on a solid attractive substrate which is attached with one end to a pulling force. The conformational properties of such chain and its phase behavior are treated within a…

软凝聚态物质 · 物理学 2009-04-01 S. Bhattacharya , V. G. Rostiashvili , A. Milchev , T. A. Vilgis

We investigate interfacial properties between two highly incompatible polymers of different stiffness. The extensive Monte Carlo simulations of the binary polymer melt yield detailed interfacial profiles and the interfacial tension via an…

统计力学 · 物理学 2009-10-30 Marcus Mueller , Andreas Werner

In this paper we investigate the form factors of paths for a class of non Gaussian processes. These processes are characterized in terms of the Mittag-Leffler function. In particular, we obtain a closed analytic form for the form factors,…

概率论 · 数学 2020-08-11 José Luís da Silva , Ludwig Streit

As an important physical quantity to understand the internal structure of polymer chains, the structure factor is being studied both in theory and experiment. Theoretically, the structure factor of Gaussian chains have been solved…

软凝聚态物质 · 物理学 2021-04-21 Jie Huang , Xinghua Zhang , Gang Huang , Shiben Li

In this paper we study the shape characteristics of a polymer chain in a good solvent using a mesoscopic level of modelling. The dissipative particle dynamics simulations are performed in the $3D$ space at a range of chain lengths $N$. The…

软凝聚态物质 · 物理学 2016-11-24 Ostap Kalyuzhnyi , Jaroslav Ilnytskyi , Yurij Holovatch , Christian von Ferber

Self-avoiding polymers in strictly two-dimensional ($d=2$) melts are investigated by means of molecular dynamics simulation of a standard bead-spring model with chain lengths ranging up to N=2048. % The chains adopt compact configurations…

软凝聚态物质 · 物理学 2015-05-18 H. Meyer , J. P. Wittmer , T. Kreer , A. Johner , J. Baschnagel

We use Monte Carlo simulations to study polymer melts consisting of fully flexible and moderately stiff chains in the bond fluctuation model at a volume fraction $0.5$. In order to reduce the local density fluctuations, we test a…

软凝聚态物质 · 物理学 2015-06-24 Hsiao-Ping Hsu

A novel method to determine the density and temperature of a system based on quantum Fermionic fluctuations is generalized to the limit where the reached temperature T is large compared to the Fermi energy {\epsilon}f . Quadrupole and…

核理论 · 物理学 2015-06-03 Hua Zheng , Aldo Bonasera

Multispeckle x-ray photon correlation spectroscopy was employed to characterize the slow dynamics of a colloidal suspension formed by highly-charged, nanometer-sized disks. At scattering wave vectors $q$ corresponding to interparticle…

We propose the quantitative mean-field theory of mechanical unfolding of a globule formed by long flexible homopolymer chain collapsed in poor solvent and subjected to extensional deformation. We demonstrate that depending on the degree of…

软凝聚态物质 · 物理学 2012-05-15 Alexey A. Polotsky , Mohamed Daoud , Oleg Borisov , Tatiana M. Birshtein

We describe method to discuss thermodynamics of a defected semi-flexible homo-polymer chain in the two and three dimensions using fully directed self-avoiding walk lattice model. The defects are located along a line and these defects are…

软凝聚态物质 · 物理学 2020-11-23 Pramod Kumar Mishra

A simple quantum mechanical model consisting of a discrete level resonantly coupled to a continuum of finite width, where the coupling can be varied from perturbative to strong (Fano-Anderson model), is considered. The particle is initially…

量子物理 · 物理学 2019-02-19 E. Kogan

The diffraction of fast atoms at crystal surfaces is ideal for a detailed investigation of the surface electronic density. However, instead of sharp diffraction spots, most experiments show elongated streaks characteristic of inelastic…

原子物理 · 物理学 2017-08-02 Philippe Roncin , Maxime Debiossac

Conformational properties of polymer melts confined between two hard structureless walls are investigated by Monte Carlo simulation of the bond-fluctuation model. Parallel and perpendicular components of chain extension, bond-bond…

软凝聚态物质 · 物理学 2009-11-10 A. Cavallo , M. Müller , J. P. Wittmer , A. Johner , K. Binder