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We point out that large composite spin-orbital fluctuations in Mott insulators with $t_{2g}$ orbital degeneracy are a manifestation of quantum entanglement of spin and orbital variables. This results in a dynamical nature of the spin…

强关联电子 · 物理学 2007-05-23 Andrzej M. Oles , Peter Horsch , Louis Felix Feiner , Giniyat Khaliullin

Neutron spectroscopy was applied to study the magnetic interactions of orbitally degenerate Co$^{2+}$ on a host MgO rocksalt lattice where no long range spin or orbital order exists. The paramagnetic nature of the substituted monoxide…

A spin-orbital superexchange Hamiltonian in a Mott insulator with $t_{2g}$ orbital degeneracy is investigated. More specifically, we focus on a spin ferromagnetic state of the model and study a collective behavior of orbital angular…

强关联电子 · 物理学 2009-11-11 G. Khaliullin , S. Okamoto

We summarize some characteristic features of the frustrated magnetic interactions in spin-orbital models adequate for cubic transition metal oxides with orbital degeneracy. A generic tendency towards dimerization, found already in the…

强关联电子 · 物理学 2015-06-24 Andrzej M. Oles

Using generalizations of natural orbitals, spin-averaged natural orbitals, and two-particle charge correlators for solids, we investigate electronic structure of antiferromagnetic transition-metal oxides with a fully self-consistent,…

强关联电子 · 物理学 2024-02-07 Pavel Pokhilko , Dominika Zgid

We study the effective spin-orbital model derived for the d9 ions in a three-dimensional perovskite lattice, as in KCuF_3, where at each site the doubly degenerate eg orbitals contain a single hole. The model describes the superexchange…

强关联电子 · 物理学 2009-10-31 Andrzej M. Oles , Louis Felix Feiner , Jan Zaanen

Effect of rotationally-invariant Hund's rule coupling on a magnetism of multiorbital Hubbard models is studied within a dynamical mean field theory framework. Comparison of static magnetic susceptibilities and local densities of states of…

强关联电子 · 物理学 2012-10-03 A. E. Antipov , I. S. Krivenko , V. I. Anisimov , A. I. Lichtenstein , A. N. Rubtsov

We study a two-dimensional effective orbital superexchange model derived for strongly correlated e_g electrons coupled to t_{2g} core spins in layered manganites. One finds that the ferromagnetic and antiferromagnetic correlations closely…

强关联电子 · 物理学 2007-05-23 M. Daghofer , D. R. Neuber , A. M. Oles , W. von der Linden

Quantum magnets with spin $J=2$, which arise in spin-orbit coupled Mott insulators, can potentially display multipolar orders. We carry out an exact diagonalization study of a simple octahedral crystal field Hamiltonian for two electrons,…

强关联电子 · 物理学 2020-04-17 Sreekar Voleti , Dalini D. Maharaj , Bruce D. Gaulin , Graeme Luke , Arun Paramekanti

We present our theoretical results on an effective two-band double-exchange model on a pyrochlore lattice for understanding intricate phase competition in Mo pyrochlore oxides. The model includes the twofold degeneracy of $e_g'$ orbitals…

强关联电子 · 物理学 2015-05-28 Yukitoshi Motome , Nobuo Furukawa

In the present paper the ground state of a double orbitally degenerate model at weak intra-atomic interaction is studied using the Green functions method. Beside the diagonal matrix elements of electron-electron interactions the model…

强关联电子 · 物理学 2009-11-07 L. Didukh , Yu. Skorenkyy , V. Hankevych , O. Kramar

We study the effects of temperature and magnetic field on a two-orbital Hubbard model within dynamical mean field theory. We focus on the quarter filled system, which is a special point in the phase diagram due to orbital degeneracy. At…

强关联电子 · 物理学 2011-03-29 Robert Peters , Norio Kawakami , Thomas Pruschke

Theory of dilution effect in orbital ordered system is presented. The $e_g$ orbital model without spin degree of freedom and the spin-orbital coupled model in a three-dimensional simple-cubic lattice are analyzed by the Monte-Carlo…

强关联电子 · 物理学 2009-11-13 Takayoshi Tanaka , Sumio Ishihara

We investigate the collective behavior of orbital angular momentum in the spin ferromagnetic state of a Mott insulator with $t_{2g}$ orbital degeneracy. The frustrated nature of the interactions leads to an infinite degeneracy of classical…

强关联电子 · 物理学 2009-11-07 Giniyat Khaliullin , Satoshi Okamoto

We consider a model of strongly correlated $e_g$ electrons interacting by superexchange orbital interactions in the ferromagnetic phase of LaMnO$_3$. It is found that the classical orbital order with alternating occupied $e_g$ orbitals has…

强关联电子 · 物理学 2009-10-31 Jeroen van den Brink , Peter Horsch , Frank Mack , Andrzej M. Oles

Finite temperature orbital state in a ferromagnetic Mott insulator with triply-degenerate $t_{2g}$ orbital is investigated numerically. We employ the quantum Monte Carlo simulation with the loop algorithm. Indications for conventional…

强关联电子 · 物理学 2009-11-13 Takayoshi Tanaka , Sumio Ishihara

To understand effects of orbital degeneracy on magnetism, in particular effects of Hund's rule coupling, we study the two-orbital Hubbard model on a square lattice by a variational Monte Carlo method. As a variational wave function, we…

强关联电子 · 物理学 2009-01-29 Katsunori Kubo

We formulate the double exchange (DE) model for systems with $t_{2g}$ orbital degeneracy, relevant for hole-doped cubic vanadates. In the relevant regime of strong on-site Coulomb repulsion $U$ we solve the model using two distinct…

强关联电子 · 物理学 2007-06-13 Krzysztof Wohlfeld

The Kugel-Khomskii Hamiltonian for cubic titanates describes spin and orbital superexchange interactions between $d^1$ ions having three-fold degenerate $t_{2g}$ orbitals. Since orbitals do not couple along "inactive" axes, perpendicular to…

强关联电子 · 物理学 2009-11-10 A. B. Harris , Taner Yildirim , Amnon Aharony , Ora Entin-Wohlman , I. Ya. Korenblit

We investigate the Mott transitions in two-orbital Hubbard systems. Applying the dynamical mean field theory and the self-energy functional approach, we discuss the stability of itinerant quasi-particle states in each band. It is shown that…

强关联电子 · 物理学 2009-11-11 A. Koga , K. Inaba , N. Kawakami
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