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Recent theory and experiments have shown how the buildup of a high-concentration polymer layer at a one-dimensional solvent-air interface can lead to an evaporation rate that scales with time as $t^{-1/2}$ and that is insensitive to the…

软凝聚态物质 · 物理学 2025-02-21 Max Huisman , Wilson C. K. Poon , Patrick B. Warren , Simon Titmuss , Davide Marenduzzo

The conformational and dynamical properties of active polymers in solution are determined by the nature of the activity, and the behavior of polymers with self-propelled, active Brownian particle-type monomers differs qualitatively from…

软凝聚态物质 · 物理学 2020-05-27 Aitor Martin-Gomez , Thomas Eisenstecken , Gerhard Gompper , Roland G. Winkler

The phoretic Brownian dynamics method is shown here to be an effective approach to simulate the properties of colloidal chemophoretic based systems. The method is then optimized to allow for the comparison with results from multiparticle…

软凝聚态物质 · 物理学 2024-06-17 Surabhi Jaiswal , Marisol Ripoll , Snigdha Thakur

The role of solvent quality in determining the universal material properties of dilute polymer solutions undergoing steady simple shear flow is examined. A bead-spring chain representation of the polymer molecule is used, and the influence…

软凝聚态物质 · 物理学 2020-07-03 K. Satheesh Kumar , J. Ravi Prakash

We consider the statics and dynamics of a flexible polymer confined between parallel plates both in the presence and absence of hydrodynamic interactions. The hydrodynamic interactions are described at the level of the fluctuating,…

软凝聚态物质 · 物理学 2012-11-01 Santtu T. T. Ollila , Colin Denniston , Mikko Karttunen , Tapio Ala-Nissila

Considering the example of interacting Brownian particles we present a linear response derivation of the boundary condition for the corresponding hydrodynamic description (the diffusion equation). This requires us to identify a non-analytic…

统计力学 · 物理学 2009-11-07 M. Fuchs , K. Kroy

We investigate the time evolution of a model system of interacting particles, moving in a $d$-dimensional torus. The microscopic dynamics are first order in time with velocities set equal to the negative gradient of a potential energy term…

统计力学 · 物理学 2018-02-12 Paolo Butta` , Joel L. Lebowitz

The present research is dedicated to provide deeper understanding of the impact of complex architecture of branched polymers on their behaviour in solvents. The folding dynamics of macromolecules and hydrodynamics of polymer fluids are…

软凝聚态物质 · 物理学 2020-12-09 K. Haydukivska , V. Blavatska , J. Paturej

When a liquid drop spreads on an adaptive substrate the latter changes its properties what may result in an intricate coupled dynamics of drop and substrate. Here we present a generic mesoscale hydrodynamic model for such processes that is…

流体动力学 · 物理学 2020-10-28 Uwe Thiele , Simon Hartmann

For various polymers with different topological structures we numerically evaluate the mean-square radius of gyration and the hydrodynamic radius systematically through simulation. We call polymers with nontrivial topology topological…

软凝聚态物质 · 物理学 2016-11-23 Erica Uehara , Tetsuo Deguchi

We discuss the hydrodynamic radius $R_H$ of polymer chains in good solvent, and show that the leading order correction to the asymptotic law $R_H \propto N^\nu$ ($N$ degree of polymerization, $\nu \approx 0.59$) is an ``analytic'' term of…

软凝聚态物质 · 物理学 2015-06-24 Burkhard Duenweg , Dirk Reith , Martin Steinhauser , Kurt Kremer

We performed a series of simulations for a linear polymer chain in a solvent using dissipative particle dynamics to check the scaling relations for the end-to-end distance, radius of gyration and hydrodynamic radius in three dimensions. The…

软凝聚态物质 · 物理学 2009-04-03 J. M. Ilnytskyi , Yu. Holovatch

The linear viscoelastic response of flexible polymer solutions in the dilute and semidilute unentangled regimes is investigated using Brownian dynamics simulations. The relaxation modulus and dynamic moduli are computed over a wide range of…

软凝聚态物质 · 物理学 2026-04-08 Amit Varakhedkar , P. Sunthar , J. Ravi Prakash

We demonstrate experimentally that the long-range hydrodynamic interactions in an incompressible quasi 2D isotropic fluid result in an anisotropic viscous drag acting on elongated particles. The anisotropy of the drag is increasing with…

流体动力学 · 物理学 2017-12-27 Christoph Klopp , Ralf Stannarius , Alexey Eremin

The dynamical scaling properties of selfavoiding polymerized membranes with internal dimension D embedded into d dimensions are studied including hydrodynamical interactions. It is shown that the theory is renormalizable to all orders in…

凝聚态物理 · 物理学 2009-10-30 Kay Joerg Wiese

We consider mixtures of two species of spherical colloidal particles that differ in their hydrodynamic radii, but are otherwise identical, in the presence of an external field. Since the particle-particle and particle-field interactions are…

软凝聚态物质 · 物理学 2018-09-26 André S. Nunes , Akshat Gupta , Nuno A. M. Araújo , Margarida M. Telo da Gama

In this study, we investigate the suitability of dissipative particle dynamics (DPD) simulations to predict the dynamics of polymer chains in dilute polymer solutions, where the chain is represented by a set of beads connected by almost…

软凝聚态物质 · 物理学 2019-07-31 Praphul Kumar , Harishyam , Indranil Saha Dalal

The static and dynamic properties of dendrimers in semidilute solutions of linear chains of comparable size are investigated using Brownian dynamics simulations. The radius of gyration and diffusivity of a wide variety of low generation…

软凝聚态物质 · 物理学 2024-06-19 Silpa Mariya , Jeremy J. Barr , P. Sunthar , J. Ravi Prakash

The dynamic structure factor of semiflexible polymers in solution is derived from the wormlike chain model. Special attention is paid to the rigid constraint of an inextensible contour and to the hydrodynamic interactions. For the cases of…

软凝聚态物质 · 物理学 2009-10-28 Klaus Kroy , Erwin Frey

Biological systems commonly combine intrinsically out-of-equilibrium active components with passive polymeric inclusions to produce unique material properties. To explore these composite systems, idealized models - such as polymers in…

软凝聚态物质 · 物理学 2025-03-27 Zahra K. Valei , Tyler N. Shendruk