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The stress versus strain curves in dense colloidal dispersions under start-up shear flow are investigated combining experiments on model core-shell microgels, computer simulations of hard disk mixtures, and mode coupling theory. In dense…

In the present work we compute the enhancement in the long time transport coefficients due to correlated motion of fluid particles at high density. The fully wave vecor dependent extended mode coupling model is studied with the inclusion of…

统计力学 · 物理学 2016-08-31 Sudha Srivastava , Shankar P. Das

Alder and Wainwright discovered the slow power decay $\sim t^{-d/2}$ ($d$:dimension) of the velocity autocorrelation function in moderately dense hard sphere fluids using the event-driven molecular dynamics simulations. In the…

统计力学 · 物理学 2008-05-05 Masaharu Isobe

We present a theory for the steady-state dynamics of a two-dimensional system of spherically symmetric active Brownian particles. The derivation of the theory consists of two steps. First, we integrate out the self-propulsions and obtain a…

软凝聚态物质 · 物理学 2019-05-01 Grzegorz Szamel

Using a combination of theory, experiment and simulation we investigate the nonlinear response of dense colloidal suspensions to large amplitude oscillatory shear flow. The time-dependent stress response is calculated using a recently…

软凝聚态物质 · 物理学 2015-05-20 J. M. Brader , M. Siebenbuerger , M. Ballauff , K. Reinheimer , M. Wilhelm , S. J. Frey , F. Weysser , M. Fuchs

The theoretical framework for higher-order correlation functions involving multiple times and multiple points in a classical, many-body system developed by Van Zon and Schofield [Phys. Rev. E 65, 011106 (2002)] is extended here to include…

统计力学 · 物理学 2007-05-23 Ramses van Zon , Jeremy Schofield

We analyze the behavior of supercooled fluids under shear both theoretically and numerically. Theoretically, we generalize the mode-coupling theory of supercooled fluids to systems under stationary shear flow. Our starting point is the set…

软凝聚态物质 · 物理学 2009-11-10 Kunimasa Miyazaki , David R. Reichman , Ryoichi Yamamoto

We have performed molecular dynamics simulations for a model two-dimensional soft-core mixture in a supercooled state. The mixture exhibits a slow structural relaxation in a quiescent state, however, the relaxation is much enhanced in…

软凝聚态物质 · 物理学 2009-11-10 Ryoichi Yamamoto , Kunimasa Miyazaki , David R. Reichman

The physics of active systems of self-propelled particles, in the regime of a dense liquid state, is an open puzzle of great current interest, both for statistical physics and because such systems appear in many biological contexts. We…

软凝聚态物质 · 物理学 2017-10-26 Saroj Kumar Nandi , Nir S. Gov

Velocity autocorrelation functions (VAF) of the fluids are studied on short- and long-time scales within a unified approach. This approach is based on an effective summation of the infinite continued fraction at a reasonable assumption…

统计力学 · 物理学 2019-01-25 V. V. Ignatyuk , I. M. Mryglod , T. Bryk

We discuss the general link between mode-coupling like equations (which serve as the basis of some recent theories of supercooled liquids) and the dynamical equations governing mean-field spin-glass models, or the dynamics of a particle in…

凝聚态物理 · 物理学 2015-06-25 Jean-Philippe Bouchaud , Leticia Cugliandolo , Jorge Kurchan , Marc Mézard

A mode-coupling theory for dense polymeric systems is developed which unifyingly incorporates the segmental cage effect relevant for structural slowing down and polymer chain conformational degrees of freedom. An ideal glass transition of…

软凝聚态物质 · 物理学 2009-11-07 S. -H. Chong , M. Fuchs

Mode coupling theory (MCT) appears to explain several, though not all, aspects of the glass transition in colloids (particularly when short-range attractions are present). Developments of MCT, from rational foundations in statistical…

软凝聚态物质 · 物理学 2007-05-23 M. E. Cates , C. B. Holmes , M. Fuchs , O. Henrich

The nonequilibrium dynamics of a binary Lennard-Jones mixture in a simple shear flow is investigated by means of molecular dynamics simulations. The range of temperature investigated covers both the liquid, supercooled and glassy states,…

软凝聚态物质 · 物理学 2009-11-07 Ludovic Berthier , Jean-Louis Barrat

This paper is concerned with the dynamics of a binary mixture of rod--like, repulsive colloidal particles driven out of equilibrium by means of a steady shear flow (Couette geometry). To this end we first derive, starting from a microscopic…

软凝聚态物质 · 物理学 2016-05-25 Rodrigo Lugo-Frias , Sabine H. L. Klapp

Dense suspensions of deformable particles can exhibit rich nonequilibrium dynamics arising from complex flow-structure coupling. Using a multi-phase field model, we show that steady shear drives an initially disordered, dense, soft…

软凝聚态物质 · 物理学 2026-02-10 Ioannis Hadjifrangiskou , Rahil N. Valani , Diogo E. P. Pinto

A simple model is proposed for the direct correlation function (DCF) for simple fluids consisting of a hard-core contribution, a simple parametrized core correction, and a mean-field tail. The model requires as input only the free energy of…

统计力学 · 物理学 2007-10-08 James F. Lutsko

The structure, thermodynamics and slow activated dynamics of the equilibrated metastable regime of glass-forming fluids remains a poorly understood problem of high theoretical and experimental interest. We apply a highly accurate…

软凝聚态物质 · 物理学 2024-08-21 Subhashish Chaki , Baicheng Mei , Kenneth S. Schweizer

For over 30 years, mode-coupling theory (MCT) has been the de facto theoretic description of dense fluids and the liquid-glass transition. MCT, however, is limited by its ad hoc construction and lacks a mechanism to institute corrections.…

软凝聚态物质 · 物理学 2015-08-12 David D. McCowan

The self-diffusion coefficient of a granular gas in the homogeneous cooling state is analyzed near the shearing instability. Using mode-coupling theory, it is shown that the coefficient diverges logarithmically as the instability is…

统计力学 · 物理学 2015-07-02 J. Javier Brey , Maria J. Ruiz-Montero