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相关论文: Exact curvilinear diffusion coefficients in the re…

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We give a lower bound on the diffusion coefficient of a polymer chain in an entanglement network with kinematic disorder, which is obtained from an exact calculation in a modified Rubinstein-Duke lattice gas model with periodic boundary…

软凝聚态物质 · 物理学 2009-11-07 Richard D. Willmann

We investigate the Rubinstein-Duke model for polymer reptation by means of density-matrix renormalization group techniques both in absence and presence of a driving field. In the former case the renewal time \tau and the diffusion…

统计力学 · 物理学 2009-11-07 Enrico Carlon , Andrzej Drzewinski , J. M. J. van Leeuwen

Diffusion of a polymer in a gel is studied within the framework of de Gennes' model for reptation. Our results for the scaling of the diffusion coefficient D and the longest relaxation time tau are markedly different from the most recently…

凝聚态物理 · 物理学 2009-10-31 G. T. Barkema , H. M. Krenzlin

We consider an arbitrarily charged polymer driven by a weak field through a gel according to the rules of the Rubinstein-Duke model. The probability distribution in the stationary state is related to that of the model in which only the head…

统计力学 · 物理学 2007-05-23 Andrzej Drzewinski , J. M. J. van Leeuwen

The repton model is a simple model of the "reptation" motion by which DNA diffuses through a gel during electrophoresis. In this paper we show that the model can be mapped onto a system consisting of two types of particles with hard-sphere…

软凝聚态物质 · 物理学 2009-10-30 M. E. J. Newman , G. T. Barkema

We analyze the Rubinstein-Duke model for polymer reptation by means of density matrix renormalization techniques. We find a crossover behavior for a series of quantities as function of the polymer length. The crossover length may become…

统计力学 · 物理学 2009-10-31 Enrico Carlon , Andrzej Drzewinski , J. M. J. van Leeuwen

Using a generalized Rubinstein-Duke model we prove rigorously that kinematic disorder leaves the prediction of standard reptation theory for the scaling of the diffusion constant in the limit for long polymer chains $D \propto L^{-2}$…

软凝聚态物质 · 物理学 2009-11-10 R. D. Willmann , G. M. Schütz , K. Jain

The competition between reptation and Rouse Dynamics is incorporated in the Rubinstein-Duke model for polymer motion by extending it with sideways motions, which cross barriers and create or annihilate hernias. Using the Density-Matrix…

统计力学 · 物理学 2009-11-13 Andrzej Drzewinski , J. M. J. van Leeuwen

We discuss the exact solution for the properties of the recently introduced ``necklace'' model for reptation. The solution gives the drift velocity, diffusion constant and renewal time for asymptotically long chains. Its properties are also…

统计力学 · 物理学 2009-11-11 Andrzej Drzewinski , J. M. J. van Leeuwen

We consider the magnetophoresis problem within the Rubinstein-Duke model, i.e. a reptating polymer pulled by a constant field applied to a single repton at the edge of a chain. Extensive density matrix renormalization calculations are…

统计力学 · 物理学 2009-11-10 A. Drzewinski , E. Carlon , J. M. J. van Leeuwen

Herein an alternative model to reptation to describe concentrated polymer dynamics is developed. The model assumes that the chains act as blobs that are able to diffuse past each other in a compressed state. Allowing that the local…

软凝聚态物质 · 物理学 2022-02-25 Dave E. Dunstan

A model for diffusion on a cubic lattice with a random distribution of traps is developed. The traps are redistributed at certain time intervals. Such models are useful for describing systems showing dynamic disorder, such as ion-conducting…

凝聚态物理 · 物理学 2009-10-31 S. Mandal , R. Dasgupta

Polymer dynamics at large fields in Rubinstein-Duke repton model is investigated theoretically. Simple diagrammatic approach and analogy with asymmetric simple exclusion models are used to analyze the reptation dynamics of polymers. It is…

统计力学 · 物理学 2009-11-10 Anatoly B. Kolomeisky , Andrzej Drzewinski

We compare the Rubinstein-Duke model for reptation to a model where the boundary dynamics is modified by calculating the viscosity of polymer melts. The question is investigated whether the viscosity is determined by details of the dynamics…

软凝聚态物质 · 物理学 2009-11-10 Matthias Paessens

Linear polymers are represented as chains of hopping reptons and their motion is described as a stochastic process on a lattice. This admittedly crude approximation still catches essential physics of polymer motion, i.e. the universal…

统计力学 · 物理学 2015-05-18 J. M. J. van Leeuwen , Andrzej Drzewinski

Stochastic reaction-diffusion processes may be presented in terms of integrable quantum chains and can be used to describe various biological and chemical systems. Exploiting the integrability of the models one finds in some cases good…

凝聚态物理 · 物理学 2007-05-23 Gunter M. Schütz

Kinetically-constrained models are lattice-gas models that are used for describing glassy systems. By construction, their equilibrium state is trivial and there are no equal-time correlations between the occupancy of different sites. We…

统计力学 · 物理学 2017-03-01 Eial Teomy , Yair Shokef

The reptation concept in polymer dynamics is studied for model chains with added stiffness. The main idea of a chain diffusing inside a tube can be transferred from fully flexible chains. However, the picture, which renormalizes the chain…

软凝聚态物质 · 物理学 2007-05-23 Roland Faller , Florian Mueller-Plathe

Understanding the complex viscoelastic properties of polymeric liquids remains a challenge in materials science and soft matter physics. Here, we present a simple and computationally efficient criterion for the topological constraints in…

软凝聚态物质 · 物理学 2007-05-23 P. Nikunen , I. Vattulainen , M. Karttunen

We analyze diffusion of small particles in a solid polymeric medium taking into account a short range particle-polymer interaction. The system is modeled by a particle diffusion on a ternary lattice where the sites occupied by polymer…

统计力学 · 物理学 2015-06-11 Federico Camboni , Andreas Koher , Igor M. Sokolov
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