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相关论文: Nanothermodynamics:a generic approach to material …

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Nanothermodynamics extends standard thermodynamics to facilitate finite-size effects on the scale of nanometers. A key ingredient is Hill's subdivision potential that accommodates the non-extensive energy of independent small systems,…

统计力学 · 物理学 2015-04-21 Ralph V. Chamberlin

Nanothermodynamics is the thermodynamics of small systems, which are signifcantly affected by their surrounding environments. In nanothermodynamics, Hill introduced the concept of subdivision potential, which charaterizes the…

统计力学 · 物理学 2021-12-03 Yu Su , Zi-Fan Zhu , Hong Gong , Yao Wang , Rui-Xue Xu , YiJing Yan

The usual formulation of thermodynamics is based on the additivity of macroscopic systems. However, there are numerous examples of macroscopic systems that are not additive, due to the long-range character of the interaction among the…

统计力学 · 物理学 2022-06-22 Ivan Latella , Agustín Pérez-Madrid , Alessandro Campa , Lapo Casetti , Stefano Ruffo

We review first how properties of curved surfaces can be studied using Hill's thermodynamics, also called nano-thermodynamics. We proceed to show for the first time that Hill's analysis is equivalent to Gibbs for curved surfaces. This…

化学物理 · 物理学 2018-08-15 Dick Bedeaux , Signe Kjelstrup

The theory of small-system thermodynamics was originally developed to extend the laws of thermodynamics to length scales of nanometers. Here we review this "nanothermodynamics," and stress how it also applies to large systems that subdivide…

统计力学 · 物理学 2020-07-28 Ralph V. Chamberlin , Michael R. Clark , Vladimiro Mujica , George H. Wolf

Using a simple example of biological macromolecules which are partitioned between bulk solution and membrane, we investigate T.L. Hill's phenomenological nanothermodynamics for small systems. By introducing a {\em systems size dependent}…

生物物理 · 物理学 2012-04-24 Hong Qian

We consider the problem of constructing the size dependence for the thermal physical properties of nano-sized objects, taking specific heat as an example. The base methodology is Hill's nanothermodynamics. Having to abstain from use of the…

介观与纳米尺度物理 · 物理学 2015-01-12 Yury Tarasievich

A few decades after Hill's work on nano-thermodynamics, the development of a thermodynamic framework, to account consistently for the fluctuations of small systems due to their interactions with the surrounding environment, is still…

统计力学 · 物理学 2019-09-23 Salvatore Calabrese , Lamberto Rondoni , Amilcare Porporato

Recent progress in the synthesis and processing of nano-structured materials and systems calls for an improved understanding of thermal properties on small length scales. In this context, the question whether thermodynamics and, in…

材料科学 · 物理学 2007-05-23 M. Hartmann , G. Mahler , O. Hess

Thermodynamics makes definite predictions about the thermal behavior of macroscopic systems in and out of equilibrium. Statistical mechanics aims to derive this behavior from the dynamics and statistics of the atoms and molecules making up…

统计力学 · 物理学 2018-03-28 Sheldon Goldstein , David A. Huse , Joel L. Lebowitz , Pablo Sartori

Nanothermodynamics provides the theoretical foundation for understanding stable distributions of statistically independent subsystems inside larger systems. In this review it is emphasized that adapting ideas from nanothermodynamics to…

统计力学 · 物理学 2024-10-23 Ralph V. Chamberlin , Stuart M. Lindsay

In traditional thermodynamical and statistical-mechanical approaches one has (some) detailed knowledge of the principles governing the microdynamics of a system. However in many instances we may not have a Hamiltonian or good information…

统计力学 · 物理学 2007-05-23 David Ford

The use of statistical methods to model gravitational systems is crucial to physics practice, but the extent to which thermodynamics and statistical mechanics genuinely apply to these systems is a contentious issue. This paper provides new…

物理学史与哲学 · 物理学 2025-02-04 Lorenzo Lorenzetti

Classical thermodynamics is a theory based on coarse-graining, meaning that the thermodynamic variables arise from discarding information related to the microscopic features of the system at hand. In quantum mechanics, however, where one…

量子物理 · 物理学 2026-04-13 T. Pernambuco , L. C. Céleri

Thermodynamics is based on a coarse-grained approach, from which its fundamental variables emerge, effectively erasing the complicate details of the microscopic dynamics within a macroscopic system. The strength of Thermodynamics lies in…

量子物理 · 物理学 2025-04-17 Gabriel Fernandez Ferrari , Łukasz Rudnicki , Lucas Chibebe Céleri

Developing the non-equilibrium thermodynamics of friction is required for systematic design of low friction surfaces for a broad range of technological applications. Intuitively, the thermodynamic work done by a material sliding along a…

介观与纳米尺度物理 · 物理学 2019-11-07 Paola Carolina Torche , Tomas Polcar , Ondrej Hovorka

A generalized entropy arising in the context of superstatistics is obtained for an ideal gas. The curvature scalar associated to the thermodynamic space generated by this modified entropy is calculated using two formalisms of the geometric…

统计力学 · 物理学 2018-04-18 J. L. López , O. Obregón , J. Torres-Arenas

In a 2023 Nature Communication, Dong claims that a disjoining chemical potential should be used instead of "Hill's nanothermodynamics" because Hill's subdivision potential "remains elusive to relate...to any experimental observables." Here,…

统计力学 · 物理学 2024-01-05 Ralph V. Chamberlin

The origins of thermodynamics from the microscopic properties of matter have not been satisfactorily accounted for. This work presents a formulation that connects Lagrangian mechanics to thermodynamics. By using such a formulation and…

原子与分子团簇 · 物理学 2021-04-05 Eduardo Hernández-Huerta , Ruben Santamaria , Tomás Rocha Rinza

Recently a number of approaches has been developed to connect the microscopic dynamics of particle systems to the macroscopic properties of systems in nonequilibrium stationary states, via the theory of dynamical systems. This way a direct…

统计力学 · 物理学 2009-10-31 L. Rondoni , E. G. D. Cohen
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