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Active polymeric systems exhibit a rich spectrum of non-equilibrium phenomena arising from stochastic forces that explicitly break detailed balance. Despite the rapid growth of experimental and numerical studies, analytical progress remains…

软凝聚态物质 · 物理学 2026-03-09 Takahiro Sakaue , Enrico Carlon

A polymer model given in terms of beads, interacting through Hookean springs and hydrodynamic forces, is studied. Brownian dynamics description of this bead-spring polymer model is extended to multiple resolutions. Using this multiscale…

化学物理 · 物理学 2018-06-13 Edward Rolls , Radek Erban

We theoretically investigate the looping dynamics of a linear polymer immersed in a viscoelastic fluid. The dynamics of the chain is governed by a Rouse model with a fractional memory kernel recently proposed by Weber et al. (S. C. Weber,…

软凝聚态物质 · 物理学 2012-07-09 Rajarshi Chakrabarti

Molecular isomerization kinetics in liquid solvents are determined by a complex interplay between the friction acting on a rotating dihedral due to interactions with the solvent, internal dissipation effects (also known as internal…

化学物理 · 物理学 2023-09-15 Benjamin A. Dalton , Henrik Kiefer , Roland R. Netz

We study the equilibrium dynamics of a single polymer chain under good solvent condition. Special emphasis is laid on varying the drag force experienced by the chain while it moves. To this end we model the solvent in a mesoscopic manner by…

软凝聚态物质 · 物理学 2019-05-01 Suman Majumder , Henrik Christiansen , Wolfhard Janke

Using molecular dynamics simulations we examine the dynamics of a family of model polymers with varying chain length and torsional potential barriers. We focus on features of the dynamics of polymers that are seen experimentally but absent…

软凝聚态物质 · 物理学 2019-06-11 Daniel Fragiadakis , C. Michael Roland

Motivated by a recent paper by Barrett and S\"uli [J.W. Barrett & E. S\"uli: Existence of global weak solutions to compressible isentropic finitely extensible bead-spring chain models for dilute polymers, Math. Models Methods Appl. Sci., 26…

偏微分方程分析 · 数学 2016-01-07 Eduard Feireisl , Yong Lu , Endre Süli

The dynamics of a polymer ring enclosing a constant {\sl algebraic} area is studied. The constraint of a constant area is found to couple the dynamics of the two Cartesian components of the position vector of the polymer ring through the…

软凝聚态物质 · 物理学 2009-11-10 Arti Dua , Thomas A. Vilgis

Generalization of the Rouse model without any use of the postulates concerning the Gaussian distribution of the vector connecting the ends of segments is advanced. In the initial (in general, nonlinear) Langevin equations, self-averaging…

软凝聚态物质 · 物理学 2016-11-27 Nail Fatkullin

We show using Brownian dynamics simulations and theory how the shear relaxation modulus G(t) of dilute solutions of relatively stiff semiflexible polymers differs qualitatively from that of rigid rods. For chains shorter than their…

软凝聚态物质 · 物理学 2009-10-31 Matteo Pasquali , V. Shankar , David C. Morse

Slow dynamics in a fluid are studied in one of the most basic systems possible: polydisperse hard spheres. Monodisperse hard spheres cannot be studied as the slow down in dynamics as the density is increased is preempted by crystallisation.…

软凝聚态物质 · 物理学 2009-10-31 Richard P. Sear

Velocity relaxation of a spherically symmetric polymer, immersed in a viscous incompressible fluid, and after a sudden small impulse or a sudden twist from a state of rest, is studied on the basis of the linearized Navier-Stokes equations…

流体动力学 · 物理学 2015-06-17 B. U. Felderhof

We investigate the effect of hydrodynamic interactions on the non-equilibrium drift dynamics of an ideal flexible polymer pulled by a constant force applied at one end of the polymer using the perturbation theory and the renormalization…

统计力学 · 物理学 2009-11-13 Semjon Stepanow , Norio Kikuchi

Polymers exposed to shear flow exhibit a rich tumbling dynamics. While rigid rods rotate on Jeffery orbits, flexible polymers stretch and coil up during tumbling. Theoretical results show that in both of these asymptotic regimes the…

软凝聚态物质 · 物理学 2014-05-27 Philipp S. Lang , Benedikt Obermayer , Erwin Frey

The interplay of topological constraints, excluded volume interactions, persistence length and dynamical entanglement length in solutions and melts of linear chains and ring polymers is investigated by means of kinetic Monte Carlo…

统计力学 · 物理学 2009-10-31 M. Mueller , J. P. Wittmer , J. -L. Barrat

The conformational and dynamical properties of isolated semiflexible active polar ring polymers are investigated analytically. A ring is modeled as continuous Gaussian polymer exposed to tangential active forces. The analytical solution of…

软凝聚态物质 · 物理学 2022-06-22 Christian A. Philipps , Gerhard Gompper , Roland G. Winkler

The file is a Chapter from my review volume "Polymer Physics: Phenomenology of Polymeric Fluid Simulations". The chapter treats literature tests of the Rouse model, which is widely invoked as a description of polymer motion in melts. In…

软凝聚态物质 · 物理学 2024-08-27 George D. J. Phillies

The current theories on the mechanism for polymer drag-reduction (DR) are generally applicable for long-chain flexible polymers that form viscoelastic solutions. Rigid polymer solutions that generate DR seemingly lack prevalent viscoelastic…

流体动力学 · 物理学 2021-11-03 Lucas Warwaruk , Sina Ghaemi

By means of Brownian dynamics simulations we study the steady-state dynamic properties of a flexible active polymer in a poor solvent condition. Our results show that the effective diffusion constant of the polymer $D_{\rm eff}$ gets…

软凝聚态物质 · 物理学 2023-08-29 Suman Majumder , Subhajit Paul , Wolfhard Janke

Microorganisms thrive in complex environments and their behavior in fluids holds significant importance for various medical and industrial applications. By conducting Lattice Boltzmann simulations, the transport and rotational properties of…

软凝聚态物质 · 物理学 2025-03-25 Yuan Zhou , Kai Qi , Marco De Corato , Kevin Stratford , Ignacio Pagonabarraga