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Self-interaction is a fundamental flaw of practical Kohn-Sham Density Functional Theory (KS DFT) approximations responsible for numerous qualitative and even catastrophic shortcomings. Whereas self-interaction is easy to characterize in…

化学物理 · 物理学 2024-07-16 Samuel A. Slattery , Edward F. Valeev

The energy positions of frontier orbitals in organic electronic materials are often studied experimentally by (inverse) photoemission spectroscopy and theoretically within density functional theory. However, standard exchange-correlation…

We report calculations of the electronic structure of CaB$_6$ using the weighted density approximation (WDA) to density functional theory. We find a semiconducting band structure with a sizable gap, in contrast to local density…

强关联电子 · 物理学 2009-11-10 Z. Wu , D. J. Singh , R. E. Cohen

By introducing a set of auxiliary equations representing a many-body system, we have derived an extension of the Kohn-Sham scheme for the density functional theory. These equations consist of a Kohn-Sham-type equation determining…

材料科学 · 物理学 2009-11-07 Koichi Kusakabe

The eigenstates of interacting electrons in the fractional quantum Hall phase typically form fairly well defined bands in the energy space. We show that the composite fermion theory gives insight into the origin of these bands and provides…

凝聚态物理 · 物理学 2009-10-22 G. Dev , J. K. Jain

Quasiparticle interference (QPI) provides a wealth of information relating to the electronic structure of a material. However, it is often assumed that this information is constrained to two-dimensional electronic states. Here, we show that…

超导电性 · 物理学 2019-11-27 Luke C. Rhodes , Matthew D. Watson , Timur K. Kim , Matthias Eschrig

Koopmans-compliant functionals emerge naturally from extending the constraint of piecewise linearity of the total energy as a function of the number of electrons to each fractional orbital occupation. When applied to approximate…

材料科学 · 物理学 2015-06-19 Giovanni Borghi , Andrea Ferretti , Ngoc Linh Nguyen , Ismaila Dabo , Nicola Marzari

Recent experiments on two-dimensional (2D) electron systems have found a sharp increase in the effective mass of electrons with decreasing electron density. In an effort to understand this behavior we employ the many-body theory to…

介观与纳米尺度物理 · 物理学 2009-11-10 R. Asgari , B. Davoudi , B. Tanatar

One approximation is made to describe a M+1 electron many-body wavefunction by a M electron many-body wavefunction and a single electron wavefunction. Under this approximation, we have derived the Coulomb energy which relates the exciton…

材料科学 · 物理学 2007-05-23 Lin-Wang Wang

We calculate the self-energy of one-dimensional electron band with the three-dimensional long range Coulomb interaction within the random phase approximation, paying particular attention to the contribution coming from the electron…

凝聚态物理 · 物理学 2007-05-23 Z. Agic , P. Zupanovic , A. Bjelis

The present study has been carried out to understand the effect of electronic correlations on the recently found fermions in CoSi. For which the spectral functions of bulk and (001) surface of CoSi have been investigated by using DFT+DMFT…

强关联电子 · 物理学 2021-04-28 Paromita Dutta , Sudhir K. Pandey

Quasiparticle interference (QPI) of the electronic states has been widely applied in scanning tunneling microscopy (STM) to analyze the electronic band structure of materials. Single-defect induced QPI reveals defect-dependent interaction…

材料科学 · 物理学 2020-07-08 Wenhao Zhang , Kunliang Bu , Fangzhou Ai , Zongxiu Wu , Ying Fei , Yuan Zheng , Jianhua Du , Minghu Fang , Yi Yin

We compute the electronic band structure and optical properties of boron arsenide using the relativistic quasiparticle self-consistent $GW$ approach, including electron-hole interactions through solution of the Bethe-Salpeter equation. We…

材料科学 · 物理学 2019-06-07 John Buckeridge , David O. Scanlon

We present a combined theoretical and experimental study of the electronic structure of stoichiometric Bi$_4$Te$_3$, a natural superlattice of alternating Bi$_2$Te$_3$ quintuple layers and Bi bilayers. In contrast to the related…

The spectral weight ${\rm A({\bf p},\omega)}$ of the two dimensional ${\rm t-J}$ and Hubbard models has been calculated using exact diagonalization and quantum Monte Carlo techniques, at several densities ${\rm 1.0 \leq \langle n \rangle…

凝聚态物理 · 物理学 2009-10-22 A. Moreo , S. Haas , A. Sandvik , E. Dagotto

A remarkable consequence of the Hohenberg-Kohn theorem of density functional theory is the existence of an injective map between the electronic density and any observable of the many electron problem in an external potential. In this work,…

无序系统与神经网络 · 物理学 2021-08-16 Javier Robledo Moreno , Johannes Flick , Antoine Georges

The quasiparticle bands of diamond, a prototype covalent insulator, are herein studied by means of wave-function electronic-structure theory, with emphasis on the nature of the correlation hole around a bare particle. Short-range…

The development of high-performance electron sources requires theoretical frameworks that accurately link the microscopic electronic properties of cathode materials to their macroscopic photoemission observables. Here, we present a…

材料科学 · 物理学 2026-02-16 Richard Schier , Chen Wang , Jonas Dube , Julius Kühn , Alice Galdi , Thorsten Kamps , Caterina Cocchi

Electronic structure of layered van der Waals ferromagnet CrI$_{3}$ is studied with self consistent diagrammatic approaches beyond GW approximation. Considerable improvement in the calculated band gap as compared to the non-self-consistent…

材料科学 · 物理学 2021-09-01 Andrey L. Kutepov

Photo-emission spectroscopy directly probes individual electronic states, ranging from single excitations to high-energy satellites, which simultaneously represent multiple quasiparticles (QPs) and encode information about electronic…