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We present the G$_0$W$_0$ band structure, core levels, and deformation potential of monolayer FeSe in the paramagnetic phase based on a starting mean field of the Kohn Sham density functional theory (DFT) with the PBE functional. We find…

材料科学 · 物理学 2020-06-09 Diana Y. Qiu , Sinisa Coh , Marvin L. Cohen , Steven G. Louie

The polarization-dependence of the exchange-correlation (XC) energy functional of periodic insulators within Kohn-Sham (KS) density-functional theory requires a ${\cal O} (1/q^2)$ divergence in the XC kernel for small vectors q. This…

材料科学 · 物理学 2009-10-30 Ph. Ghosez , X. Gonze , R. W. Godby

The quasiparticle band structures of 3d transition metals, ferromagnetic Fe, Ni and paramagnetic Cu, are calculated by the GW approximation. The width of occupied 3d valence band, which is overestimated in the LSDA, is in good agreement…

材料科学 · 物理学 2009-11-07 Atsushi Yamasaki , Takeo Fujiwara

We present a rigorous formulation of generalized Kohn-Sham density-functional theory. This provides a straightforward Kohn-Sham description of many-body systems based not only on particle-density but also on any other observable. We…

强关联电子 · 物理学 2008-02-03 M. Valiev , G. W. Fernando

In the exact Kohn-Sham density-functional theory (DFT), the total energy versus the number of electrons is a series of linear segments between integer points. However, commonly used approximate density functionals produce total energies…

材料科学 · 物理学 2013-04-03 Eli Kraisler , Leeor Kronik

The energy levels and optical transitions of tetrahedral core/shell InP/ZnSe quantum dots (QDs) are investigated by means of multi-band k$\cdot$p theory. Despite the $\overline{T}_d$ symmetry relaxing spherical selection rules, the…

介观与纳米尺度物理 · 物理学 2026-04-06 Josep Planelles , Juan I. Climente

The GW self-energy method has long been recognized as the gold standard for quasiparticle (QP) calculations of solids in spite of the fact that the neglect of vertex corrections and the use of a DFT starting point lacks rigorous…

材料科学 · 物理学 2017-12-06 Per S. Schmidt , Christopher E. Patrick , Kristian S. Thygesen

The electronic structure of the natural topological semimetal Co$_3$Sn$_2$S$_2$ crystals was studied using near-edge x-ray absorption spectroscopy (NEXAFS) and resonant photoelectron spectroscopy (ResPES). Although, the significant increase…

We have carried out a comprehensive investigation of the quasiparticle properties of a two-dimensional electron gas, interacting via the long-range Coulomb interaction, in the presence of bare mass anisotropy (i.e. with an elliptic…

介观与纳米尺度物理 · 物理学 2021-01-12 Seongjin Ahn , S. Das Sarma

Ab initio many-body perturbation theory within the $GW$ approximation is a Green's function formalism widely used in the calculation of quasiparticle excitation energies of solids. In what has become an increasingly standard approach,…

We present a general multi-component density functional theory in which electrons and nuclei are treated completely quantum mechanically, without the use of a Born-Oppenheimer approximation. The two fundamental quantities in terms of which…

材料科学 · 物理学 2007-05-23 Thomas Kreibich , Robert van Leeuwen , E. K. U. Gross

Using the Kohn-Sham (KS) inversion method of Hollins et al. [J. Phys.: Condens. Matter 29, 04LT01 (2017)], we invert densities from variational and diffusion quantum Monte Carlo (QMC) calculations to obtain benchmark QMC-KS potentials for a…

We present a microscopic theory of ground-state spectral function of bilayer quantum Hall systems that includes interactions between Hartree-Fock quasiparticles and quantum fluctuations of the order parameter field. The collective modes in…

介观与纳米尺度物理 · 物理学 2007-05-23 Yogesh N. Joglekar , Allan H. MacDonald

Multi-band Gutzwiller-correlated wave functions reconcile the contrasting concepts of itinerant band electrons versus electrons localized in partially filled atomic shells. The approximate evaluation of these variational ground states…

强关联电子 · 物理学 2007-05-23 Joerg Buenemann , Florian Gebhard , Werner Weber

We report unphysical irregularities and discontinuities in some key experimentally-measurable quantities computed within the GW approximation of many-body perturbation theory applied to molecular systems. In particular, we show that the…

化学物理 · 物理学 2019-05-06 Mickaël Véril , Pina Romaniello , J. A. Berger , Pierre-François Loos

The density-functional approach to quantum electrodynamics is extending traditional density-functional theory and opens the possibility to describe electron-photon interactions in terms of effective Kohn-Sham potentials. In this work, we…

量子物理 · 物理学 2016-02-17 Johannes Flick , Michael Ruggenthaler , Heiko Appel , Angel Rubio

The theoretical foundations of quantum mechanics and de Broglie--Bohm mechanics are analyzed and it is shown that both theories employ a formal approach to microphysics. By using a realistic approach it can be established that the internal…

量子物理 · 物理学 2015-06-26 W. A. Hofer

The properties of the Kohn-Sham (KS) exchange potential for open systems in thermodynamical equilibrium, where the number of particles is non-conserved, are analyzed with the Optimized Effective Potential (OEP) method of Density Functional…

其他凝聚态物理 · 物理学 2015-06-25 S. Rigamonti , C. R. Proetto , F. A. Reboredo

Here we present the details of a self-consistent procedure of the photoemission data analysis within the self-energy approach introduced in Ref.1 (cond-mat/0405696). We derive the relations of the quasiparticle self-energy with the…

强关联电子 · 物理学 2007-05-23 A. A. Kordyuk , S. V. Borisenko , A. Koitzsch , J. Fink , M. Knupfer , H. Berger

We present a microscopic theory of bipolar quantum well structures in the photovoltaic regime, based on the non-equilibrium Green's function formalism for a multi band tight binding Hamiltonian. The quantum kinetic equations for the single…

介观与纳米尺度物理 · 物理学 2012-06-14 U. Aeberhard , R. H. Morf