相关论文: When Blinking Helps: Suppressed Biexciton Emission…
Halide perovskite materials raised tremendous interest in recent years since their cheap fabrication, superior performance in both solar cell and light emitting diode (LED). Due to the existence of layered quantum well structure, quasi…
Lead-halide perovskite quantum dots (PQDs) are established quantum emitters with potential for entangled photon-pair generation via multiexciton cascades. However, the energetics and dynamics of many-body excitations remain poorly…
Chemically prepared colloidal semiconductor quantum dots have long been proposed as scalable and color-tunable single emitters in quantum optics, but they have typically suffered from prohibitively incoherent emission. We now demonstrate…
Development of quantum light sources and search for quantum systems capable of supporting collective many-body states are crucial for further progress of modern quantum technologies. Metal halide perovskite quantum dots (QDs) have emerged…
Photoluminescence (PL) intermittency is a ubiquitous phenomenon detrimentally reducing the temporal emission intensity stability of single colloidal quantum dots (CQDs) and the emission quantum yield of their ensembles. Despite efforts for…
Electron transfer to an individual quantum dot promotes the formation of charged excitons with enhanced recombination pathways and reduced lifetimes. Excitons with only one or two extra charges have been observed and exploited for very…
Strong coupling between lead halide perovskite materials and optical resonators enables both the polaritonic control of the photophysical properties of these emerging semiconductors and the observation of novel fundamental physical…
Lead halide perovskites have catalyzed the rise of main-group metal halide materials as promising candidates for next-generation optoelectronics, including solar cells, light-emitting diodes, lasers, sensors, and photocatalysts. Among…
Lead halide perovskite quantum dots (QDs), the latest generation of colloidal QD family, exhibit outstanding optical properties which are now exploited as both classical and quantum light sources. Most of their rather exceptional properties…
Nanostructured semiconductors emit light from electronic states known as excitons[1]. According to Hund's rules[2], the lowest energy exciton in organic materials should be a poorly emitting triplet state. Analogously, the lowest exciton…
Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown…
Photo-luminescence intermittency (blinking) in semiconductor nanocrystals (NCs), a phenomenon ubiquitous to single-emitters, is generally considered to be temporally random intensity fluctuations between bright (On) and dark (Off) states.…
Incoherent pumping in quantum dots (QDs) can create a biexciton state through two paths: via the formation of bright or dark exciton states. The latter, dark-pumping, path is shown to enhance the probability of two-photon simultaneous…
The coherent interaction of electromagnetic fields with solid-state two-level systems can yield deterministic quantum light sources for photonic quantum technologies. To date, the performance of semiconductor single-photon sources based on…
Advances in opto-electronics require the development of materials with novel and engineered characteristics. A class of materials that has garnered tremendous interest is metal-halide perovskites, stimulated by meteoric increases in…
Giant shell CdSe/CdS quantum dots are bright and flexible emitters, with near-unity quantum yield and suppressed blinking, but their single photon purity is reduced by efficient multiexcitonic emission. We report the observation, at the…
Layered halide perovskites exhibit remarkable optoelectronic properties and technological promise, driven by strongly bound excitons. The interplay of spin-orbit and exchange coupling creates a rich excitonic landscape, determining their…
Dark ground state exciton in semiconductor nanocrystals has been a subject of much interest due to its long lifetime attractive for applications requiring long-lived electronic or spin states. Significant effort has been made recently to…
Understanding the fine structure of excitons is crucial for optoelectronic and quantum photonic applications of lead halide perovskites. It is demonstrated that polarization-sensitive photon echo spectroscopy in magnetic field provides a…
The MAPbI$_3$ halide perovskite single crystals are studied at 5 K temperature using the photoluminescence excitation spectroscopy. Two non-interacting types of states are determined: bound excitons and defect-related states. Excitation of…