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Polymer brushes normally swell in a good solvent and collapse in a poor solvent. An abnormal response of polymer brushes, so-called co-nonsolvency, is the phenomenon where the brush counter-intuitively collapses in a good solvent mixture.…

软凝聚态物质 · 物理学 2019-08-26 Gyehyun Park , YounJoon Jung

We introduce a new disorder regime for directed polymers in dimension $1+1$ that sits between the weak and strong disorder regimes. We call it the intermediate disorder regime. It is accessed by scaling the inverse temperature parameter…

概率论 · 数学 2014-03-28 Tom Alberts , Konstantin Khanin , Jeremy Quastel

Multiblock copolymer chains in implicit nonselective solvents are studied by Monte Carlo method which employs a parallel tempering algorithm. Chains consisting of 120 $A$ and 120 $B$ monomers, arranged in three distinct microarchitectures:…

软凝聚态物质 · 物理学 2014-10-20 Krzysztof Lewandowski , Michal Banaszak

The precise arrangement of different chemical moieties in a polymer determines its thermophysical properties. How the sequence of moieties impacts the properties of a polymer is an outstanding problem in polymer science. Herein, we address…

软凝聚态物质 · 物理学 2025-08-26 Sandeep Parma , R. Nagaranajan , Tarak K Patra

The possibilities to fractionate copolymers with respect to their chemical composition on a preparative scale by means of the establishment of liquid/liquid phase equilibria were studied for random copolymers of styrene and acrylonitrile…

材料科学 · 物理学 2009-11-10 Stefan Loske , Anja Schneider , Bernhard A. Wolf

In this paper we revisit the problem of a (non self-avoiding) polymer chain in a random medium which was previously investigated by Edwards and Muthukumar (EM). As noticed by Cates and Ball (CB) there is a discrepancy between the…

无序系统与神经网络 · 物理学 2009-10-31 Yadin Y. Goldschmidt

The formation of interface from an initial sharp interface in polydisperse A/B blends is studied using the external potential dynamic method. The present model is a nonlocal coupling model as we take into account the correlation between…

软凝聚态物质 · 物理学 2015-05-13 Shuanhu Qi , Xinghu Zhang , Dadong Yan

We analyse the nature of the confinement of an infinitely long (and finite) linear semiflexible homo-polymer chain confined in between two geometrical constraints (A&B) under good solvent condition in two dimensions. The constraints are…

软凝聚态物质 · 物理学 2017-10-16 Pramod Kumar Mishra

We present a theoretical argument to derive a scaling law between the mean translocation time $\tau$ and the chain length $N$ for driven polymer translocation. This scaling law explicitly takes into account the pore-polymer interactions,…

软凝聚态物质 · 物理学 2013-10-29 Timo Ikonen , Aniket Bhattacharya , Tapio Ala-Nissila , Wokyung Sung

The density crossover scaling of various thermodynamic properties of solutions and melts of self-avoiding and highly flexible polymer chains without chain intersections confined to strictly two dimensions is investigated by means of…

软凝聚态物质 · 物理学 2012-09-03 N. Schulmann , H. Meyer , P. Polińska , J. Baschnagel , J. P. Wittmer

It is commonly accepted that in concentrated solutions or melts high-molecular weight polymers display random-walk conformational properties without long-range correlations between subsequent bonds. This absence of memory means, for…

软凝聚态物质 · 物理学 2009-11-11 J. P. Wittmer , P. Beckrich , F. Crevel , C. C. Huang , A. Cavallo , T. Kreer , H. Meyer

We consider the rupture dynamics of a homopolymer chain pulled at one end at a constant loading rate r. Compared to single bond breaking, the existence of the chain introduces two new aspects into rupture dynamics: the non-Markovian aspect…

软凝聚态物质 · 物理学 2009-10-29 S. Fugmann , I. M. Sokolov

The production of sequence-specific copolymers using copolymer templates is fundamental to the synthesis of complex biological molecules and is a promising framework for the synthesis of synthetic chemical complexes. Unlike the…

软凝聚态物质 · 物理学 2022-02-16 Jordan Juritz , Jenny M Poulton , Thomas E Ouldridge

Heterogeneous distribution of passive and active domains in the chromosome plays a crucial role for its dynamic organization within the cell nucleus. Motivated by that here we investigate the steady-state conformation and dynamics of a…

软凝聚态物质 · 物理学 2024-09-27 Suman Majumder , Subhajit Paul

Using exact enumeration methods and Monte Carlo simulations we study the phase diagram relative to the conformational transitions of a two dimensional diblock copolymer. The polymer is made of two homogeneous strands of monomers of…

统计力学 · 物理学 2009-10-31 Marco Baiesi , Enrico Carlon , Enzo Orlandini , Attilio L. Stella

In three dimensions, or more generally, below the upper critical dimension, scaling laws for critical phenomena seem well understood, for both infinite and for finite systems. Above the upper critical dimension of four, finite-size scaling…

统计力学 · 物理学 2007-05-23 M. A. Sumour , D. Stauffer , M. M. Shabat , A. H. El-Astal

We investigate conformations and dynamics of a polymer considering its monomers to be active Brownian particles. This active polymer shows very intriguing physical behavior which is absent in an active Rouse chain. The chain initially…

软凝聚态物质 · 物理学 2020-04-13 Shalabh K. Anand , Sunil P. Singh

Advanced chain-growth computer simulation methodologies have been employed for a systematic statistical analysis of the critical behavior of a polymer adsorbing at a substrate. We use finitesize scaling techniques to investigate the…

软凝聚态物质 · 物理学 2017-05-09 J. A. Plascak , Paulo H. L. Martins , Michael Bachmann

We report molecular dynamics simulations of the segregation of two overlapping chains in cylindrical confinement. We find that the entropic repulsion between the chains can be sufficiently strong to cause segregation on a time scale that is…

软凝聚态物质 · 物理学 2011-11-09 Axel Arnold , Suckjoon Jun

Nonequilibrium molecular dynamics simulations are used to study the shear thinning behavior of immiscible symmetric polymer blends. The phase separated polymers are subjected to a simple shear flow imposed by moving a wall parallel to the…

软凝聚态物质 · 物理学 2009-11-07 Sandra Barsky , Mark O. Robbins