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Nanostructured semiconductors emit light from electronic states known as excitons[1]. According to Hund's rules[2], the lowest energy exciton in organic materials should be a poorly emitting triplet state. Analogously, the lowest exciton…

Dark ground state exciton in semiconductor nanocrystals has been a subject of much interest due to its long lifetime attractive for applications requiring long-lived electronic or spin states. Significant effort has been made recently to…

Advances in opto-electronics require the development of materials with novel and engineered characteristics. A class of materials that has garnered tremendous interest is metal-halide perovskites, stimulated by meteoric increases in…

The ordering of optically bright and dark excitonic states in lead-halide perovskite nanocrystals has been a matter of some debate. It has been proposed that the unusually short radiative lifetimes in these materials is due to an optically…

化学物理 · 物理学 2023-06-28 Daniel Weinberg , Yoonjae Park , David T. Limmer , Eran Rabani

The trend towards ever smaller high-performance devices in modern technology requires novel materials with new functionalities. The recent emergence of atomically thin two-dimensional (2D) materials has opened up possibilities for the…

介观与纳米尺度物理 · 物理学 2019-06-05 Maja Feierabend , Zahra Khatibi , Gunnar Berghäuser , Ermin Malic

Semiconductor nanoplatelets (NPLs), with their large exciton binding energy, narrow photoluminescence (PL), and absence of dielectric screening for photons emitted normal to the NPL surface, could be expected to become the fastest…

Semiconductor nanocrystals could replace conventional bulk materials completely in displays and light-emitting diodes. Exciton transport dominates over charge carrier transport for materials with high exciton binding energies and long…

We report that dark excitons can have a large contribution to the emission intensity in carbon nanotubes due to an efficient exciton conversion from a dark state to a bright state. Time-resolved photoluminescence measurements are used to…

介观与纳米尺度物理 · 物理学 2019-12-11 A. Ishii , H. Machiya , Y. K. Kato

We study the band-edge exciton fine structure and in particular its bright-dark splitting in colloidal semiconductor nanocrystals by four different optical methods based on fluorescence line narrowing and time-resolved measurements at…

Light emission from higher-order correlated excitonic states has been recently reported in hBN-encapsulated monolayer WSe2 and WS2 upon optical excitation. These exciton complexes are found to be bound states of excitons residing in…

介观与纳米尺度物理 · 物理学 2019-04-19 Matthias Paur , Aday J. Molina-Mendoza , Rudolf Bratschitsch , Kenji Watanabe , Takashi Taniguchi , Thomas Mueller

Odd-angular momentum exciton states are dark to light in monolayers of transition-metal dichalcogenides and can be addressed only by two-photon probes. Besides, $2p$ excitons states are expected to show a fine splitting that arises from the…

介观与纳米尺度物理 · 物理学 2020-02-25 Luca Chirolli

Nanocrystals based on metal-halide perovskites offer a promising material platform for highly efficient lighting. Using transient optical spectroscopy, we study excitation recombination dynamics in manganese-doped CsPb(Cl,Br)3 perovskite…

It is strong Coulomb effects in carbon nanotubes that lead to formation of the so-called "bright" and "dark" (forbidden one-photon optical transition) exciton states, and dramatically decrease the efficiency of one-photon light emission via…

量子物理 · 物理学 2009-02-09 Nikolai G. Kalugin , Yuri V. Rostovtsev

Monolayer transition metal dichalcogenide (TMDC) crystals, as direct-gap materials with unusually strong light-matter interaction, have attracted much recent attention. In contrast to the initial understanding, the minima of the conduction…

This paper is written for the Special Issue in Honor of Emmanuel Rashba. We study the gas of indirect dipolar excitons created by an interband illumination of a pentalayer WSe$_2$/MoSe$_2$/WSe$_2$/MoSe$_2$/WSe$_2$. We show that two colinear…

介观与纳米尺度物理 · 物理学 2022-09-14 Yi Huang , B. I. Shklovskii

The Rashba spin-orbit coupling effect, primarily arising from structural-inversion asymmetry in periodic crystals, has garnered considerable attention due to its tunability and potential applications in spintronics. Its capability to…

Understanding the interplay between bright and dark exciton states is crucial for deciphering the luminescence properties of low-dimensional materials. The origin of the outstanding brightness of lead halide perovskites remains elusive.…

介观与纳米尺度物理 · 物理学 2024-04-16 Mohamed-Raouf Amara , Caixia Huo , Christophe Voisin , Qihua Xiong , Carole Diederichs

We consider a hybrid plasmon-exciton system comprised of a resonant molecular subsystem and three Au wires supporting a dipole mode which can be coupled to a dark mode in controllable fashion by variation of a symmetry parameter. The…

光学 · 物理学 2015-03-25 Maxim Sukharev , Paul N. Day , Ruth Pachter

We present an experimental demonstration of strong coupling between a surface plasmon propagating on a planar silver substrate, and the lowest excited state of CdSe nanocrystals. Variable-angle spectroscopic ellipsometry measurements…

材料科学 · 物理学 2009-12-16 D. E. Gómez , K. C. Vernon , T. J. Davis , T. L. Nguyen , P. Mulvaney

The spin-orbit -induced spin splitting of energy bands in low symmetry compounds (the Rashba Effect) has a long-standing relevance to spintronic applications and to the fundamental understanding of symmetry breaking in solids, yet the…

材料科学 · 物理学 2020-09-01 Carlos Mera Acosta , Elton Ogoshi , Adalberto Fazzio , Gustavo Dalpian , Alex Zunger
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