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The optical properties of weakly-doped two-dimensional materials are dominated by strong exciton and trion absorption and luminescence features. In this article we examine the influence of moir\'e patterns in semiconductor heterobilayers on…

介观与纳米尺度物理 · 物理学 2022-07-20 Yongxin Zeng , Allan H. MacDonald

Beyond-diffraction-limit optical absorption spectroscopy provides profound information on the graded band structures of composition-spread and stacked two-dimensional materials, in which direct/indirect bandgap, interlayer coupling,…

We investigated the nonlinear optical properties of CdSe/CdS nanoplatelets in the vicinity of heavy hole and light hole exciton resonances. The two color pump-probe technique was applied. The first intense pulse created non-equilibrium…

We perform the first-principles many-body GW and Bethe-Salpeter equation (BSE) calculations on the two-dimensional hexagonal boron nitride (2D-hBN) to explore the effects of opposite atoms on the electronic structure and linear one-photon…

材料科学 · 物理学 2023-01-04 You-Zhao Lan

Excitons, namely neutral excitations in a system of electrons arising from the electron-hole interaction, are often essential to explain optical measurements in materials. They are governed by the Bethe-Salpeter equation, which can be cast…

强关联电子 · 物理学 2024-10-29 M. A. García-Blázquez , J. J. Palacios

To translate electrical into optical signals one uses the modulation of either the refractive index or the absorbance of a material by an electric field. Contemporary electroabsorption modulators (EAMs) employ the quantum confined Stark…

In order to realize the significant potential of optical materials such as metal halides, computational techniques which give accurate optical properties are needed, which can work hand-in-hand with experiments to generate high efficiency…

材料科学 · 物理学 2021-03-04 Jamie M. Booth , Mike V. Klymenko , Jared H. Cole , Salvy P. Russo

Moir\'e materials offer a versatile platform for engineering excitons with unprecedented control, promising next-generation optoelectronic applications. While continuum models are widely used to study moir\'e excitons due to their…

材料科学 · 物理学 2025-10-08 Indrajit Maity , Johannes Lischner , Arash A. Mostofi , Ángel Rubio

Group-V monolayer materials exhibit intriguing electronic and optical properties, influenced by their unique crystal symmetries and structural phases. In this work, we study arsenic monolayers, investigating their electronic and optical…

材料科学 · 物理学 2026-04-28 Niloufar Dadkhah , Walter R. L. Lambrecht

We calculate, as a function of temperature and conduction band electron density, the optical absorption of a weakly n-doped, idealized semiconductor quantum well. In particular, we focus on the absorption band due to the formation of a…

强关联电子 · 物理学 2009-11-07 F. X. Bronold

With the examples of the C $K$-edge in graphite and the B $K$-edge in hexagonal BN, we demonstrate the impact of vibrational coupling and lattice distortions on the X-ray absorption near-edge structure (XANES) in 2D layered materials.…

The optical properties of two-dimensional transition metal dichalcogenide monolayers such as MoS$_2$ or WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. Screening effects due the presence of hexagonal-BN surrounding…

材料科学 · 物理学 2018-12-26 Iann C. Gerber , Xavier Marie

We present a tight-binding (TB) model and $\mathbf{k\cdot p}$ theory for electrons in monolayer and few-layer InSe. The model is constructed from a basis of all $s$ and $p$ valence orbitals on both indium and selenium atoms, with…

介观与纳米尺度物理 · 物理学 2017-01-05 S. J. Magorrian , V. Zólyomi , V. I. Fal'ko

We present ab initio absorption spectra of six three-dimensional semiconductors and insulators calculated using Gaussian-based periodic equation-of-motion coupled-cluster theory with single and double excitations (EOM-CCSD). The spectra are…

化学物理 · 物理学 2021-07-13 Xiao Wang , Timothy C. Berkelbach

Interband absorption and luminescence of quasi-two-dimensional, circularly symmetric, N_e electron quantum dots are studied at high magnetic fields, 8<B<60 T, and low temperatures, T<<2 K. In the N_e=0 and 1 dots, the initial and final…

介观与纳米尺度物理 · 物理学 2009-10-31 Augusto Gonzalez , Eduardo Menendez-Proupin

Electron irradiation of GaN nanowires in a scanning electron microscope strongly reduces their luminous efficiency as shown by cathodoluminescence imaging and spectroscopy. We demonstrate that this luminescence quenching originates from a…

介观与纳米尺度物理 · 物理学 2017-10-13 Jonas Lähnemann , Timur Flissikowski , Martin Wölz , Lutz Geelhaar , Holger T. Grahn , Oliver Brandt , Uwe Jahn

We present an electrostatic theory of band gap renormalization in atomically-thin semiconductors that captures the strong sensitivity to the surrounding dielectric environment. In particular, our theory aims to correct known band gaps, such…

材料科学 · 物理学 2018-01-24 Yeongsu Cho , Timothy C. Berkelbach

We develop a microscopic theory of a strong electromagnetic field interaction with gated bilayer graphene. Quantum kinetic equations for density matrix are obtained using a tight binding approach within second quantized Hamiltonian in an…

介观与纳米尺度物理 · 物理学 2017-05-24 A. A. Avetisyan , A. P. Djotyan , K. Moulopoulos

The electronic structure and optical response of electrically gated bilayer graphene are studied by first-principles approaches. We have obtained the induced band gap that is in good agreement with experiment when the applied electric field…

介观与纳米尺度物理 · 物理学 2015-03-13 Li Yang

The van der Waals layered semiconductor CrSBr, which exhibits A-type antiferromagnetism and a relatively high N\'{e}el temperature, has been successfully exfoliated into atomically thin sheets. In this study, we investigate the structural,…

材料科学 · 物理学 2025-02-07 Huicong Li , Yali Yang , Zhonghao Xia , Yateng Wang , Jiacheng Wei , Jiangang He , Rongming Wang