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The transport of CO2 across the air-water interface is central to physical oceanography and carbon sequestration. A comprehensive understanding of this process requires high-resolution diagnostics of diffusion, absorption, and reaction…

流体动力学 · 物理学 2025-09-23 Dongfang Zhao , Yumin Shi , Shengkai Wang

X-ray four-wave mixing signals generated in the $k_1 + k_2 - k_3$ phase-matching direction are simulated for N1s transitions in para-nitroanline and two-ring hydrocarbons disubstituted with an amine and a nitroso groups. The two-dimensional…

原子物理 · 物理学 2008-11-20 Igor V. Schweigert , Shaul Mukamel

Fully energy-filtered X-ray photoelectron emission microscopy is used to analyze the spatial distribution of the silicon sub-oxide structure at the SiO2/Si interface as a function of underlying doping pattern. Using a spectroscopic…

材料科学 · 物理学 2012-11-21 F. de la Peña , N. Barrett , L. F. Zagonel , M. Walls , O. Renault

VOXES is a Von Hamos X-ray spectrometer developed at the INFN National Laboratories of Frascati for high-resolution laboratory X-ray spectroscopy in the 5--20~keV range. It uses curved mosaic crystals and motorized positioning stages to…

X-ray absorption spectroscopy (XAS) is a premier technique for materials characterization, providing key information about the local chemical environment of the absorber atom. In this work, we develop a database of sulfur K-edge XAS spectra…

Efficient electro-catalytic water-splitting technologies require suitable catalysts for the oxygen evolution reaction (OER). The development of novel catalysts could benefit from the achievement of a complete understanding of the reaction…

材料科学 · 物理学 2020-04-22 Francesco Nattino , Nicola Marzari

Optical coherence elastography (OCE) is a powerful non-invasive imaging technique for high-resolution assessment of tissue elasticity and viscoelasticity. Accurate characterization of viscoelastic properties requires estimating shear wave…

We present X-ray absorption spectroscopy and resonant inelastic X-ray scattering (RIXS) measurements on the iron L-edge of 0.5 mM aqueous ferricyanide. These measurements demonstrate the ability of high-throughput transition-edge-sensor…

We report a comprehensive resonant inelastic x-ray scattering (RIXS) study of various iridate materials focusing on core-level excitations and transitions between crystal-field split d-levels. The 2p core hole created at the Ir $L_3$…

强关联电子 · 物理学 2018-05-10 Young-June Kim , J. P. Clancy , H. Gretarsson , G. Cao , Yogesh Singh , Jungho Kim , M. H. Upton , D. Casa , T. Gog

Single-particle methods based on Kohn-Sham unoccupied states to describe near-edge X-ray absorption (XAS) spectra are routinely applied for the description of K-edge spectra, as there is no complication due to spin-orbit (SO) coupling. L-…

材料科学 · 物理学 2026-02-26 Esther A. B. Johnsen , Naoki Horiuchi , Toma Susi , Michael Walter

The Geostationary Operational Environmental Satellite (GOES) solar soft X-ray (SXR) irradiance in the 1-8{\AA} wavelength range is a long-standing measure of solar activity, used to define the classification of flare strengths. As a result,…

Recent developments of high-reputation-rate X-ray free electron lasers (XFELs) such as European XFEL and LSCS-II, combined with coincidence measurements at the COLTRIMS-Reaction Microscope, is now opening a door to realize a long-standing…

化学物理 · 物理学 2021-05-26 Fukiko Ota , Keisuke Hatada , D Sébilleau , Kiyoshi Ueda , Kaoru Yamazaki

Unknown changes in the crystalline order of regular TiO$_2$ result in the formation of black titania, which has garnered significant interest as a photocatalytic material due to the accompanying electronic changes. Herein, we determine the…

材料科学 · 物理学 2019-08-08 Brett Leedahl , Tristan de Boer , Xiaotao Yuan , Alexander Moewes

Lensless X-ray imaging provides element-specific nanoscale insights into thick samples beyond the reach of conventional light and electron microscopy. Coherent diffraction imaging (CDI) methods, such as ptychographic tomography, can recover…

We investigate laser-driven electron dynamics in solids on the atomic scale and in real space within Floquet formalism, and develop a method based on subcycle-resolved x-ray-optical wave mixing to reconstruct those dynamics. We analyze how…

光学 · 物理学 2020-12-21 Daria Popova-Gorelova , Robin Santra

As exposure to electromagnetic waves becomes increasingly widespread, it is important to quantify how incident fields couple into biological tissue and where absorbed energy is deposited. This work presents an analytical, physics based…

生物物理 · 物理学 2026-04-09 Hongyun Wang , Shannon E. Foley , Hong Zhou

We present in this paper mid-infrared (5-8~$\mu$m) spectroscopy toward the massive young binary W3~IRS~5, using the EXES spectrometer in high-resolution mode ($R\sim$50,000) from the NASA Stratospheric Observatory for Infrared Astronomy…

The time evolution of diffuse X-ray scattering intensities conditioned by the short-range order (SRO) in Ni-Mo solid solutions is investigated. As shown, the transition from a quenched (nonequilibrium) state to the equilibrium one is…

材料科学 · 物理学 2014-06-12 S. M. Bokoch , M. P. Kulish , V. A. Tatarenko , T. M. Radchenko

We have studied the electronic structure of epitaxially grown thin films of La$_{1-x}$Sr$_x$FeO$_3$ by {\it in-situ} photoemission spectroscopy (PES) and x-ray absorption spectroscopy (XAS) measurements. The Fe 2$p$ and valence-band PES…

Dynamical phase separation during a solid-solid phase transition poses a challenge for understanding the fundamental processes in correlated materials. Critical information underlying a phase transition, such as localized phase competition,…