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We revisit the problem of unphysical charge density delocalization/fractionalization induced by the self-interaction error of common approximate Kohn-Sham Density Functional Theory functionals on simulation of small to medium-size proteins…

化学物理 · 物理学 2024-07-30 Samuel A. Slattery , Jaden C. Yon , Edward F. Valeev

It is known for quite some time that approximate density functional (ADF) theories fail disastrously when describing the dis-sociative symmetric radical cations R2+. Considering this dissociation limit, previous work has shown that…

材料科学 · 物理学 2016-09-28 Ester Livshits , Roi Baer

An implementation of the Hartree-Fock (HF) method capable of robust convergence for well-behaved arbitrary central potentials is presented. The Hartree-Fock equations are converted to a generalized eigenvalue problem by employing a B-spline…

原子物理 · 物理学 2021-08-13 D. T. Waide , D. G. Green , G. F. Gribakin

We present a density matrix approach for computing global solutions of restricted open-shell Hartree-Fock theory, based on semidefinite programming (SDP), that gives upper and lower bounds on the Hartree-Fock energy of quantum systems.…

化学物理 · 物理学 2014-04-22 Srikant Veeraraghavan , David A. Mazziotti

We derive and implement symmetry-projected Hartree-Fock-Bogoliubov (HFB) equations and apply them to the molecular electronic structure problem. All symmetries (particle number, spin, spatial, and complex conjugation) are deliberately…

It has recently been shown that configuration state functions (CSF) with local orbitals can provide a compact reference state for low-spin open-shell electronic structures, such as antiferromagnetic states. However, optimizing a low-spin…

化学物理 · 物理学 2025-08-05 Hugh G. A. Burton

We present a group theoretical study of the symmetry-broken unrestricted Hartree-Fock orbitals and electron densities in the case of a two-dimensional N-electron single quantum dot (with and without an external magnetic field). The breaking…

介观与纳米尺度物理 · 物理学 2009-11-10 Constantine Yannouleas , Uzi Landman

Symmetry properties of densities and mean fields appearing in the nuclear Density Functional Theory with pairing are studied. We consider energy functionals that depend only on local densities and their derivatives. The most important…

核理论 · 物理学 2010-04-06 S. G. Rohozinski , J. Dobaczewski , W. Nazarewicz

The Hartree-Fock approximation for bosons employs variational wave functions that are a combination of permanents. These are bosonic counterpart of the fermionic Slater determinants, but with the significant distinction that the…

量子气体 · 物理学 2025-03-03 B. R. Que , J. M. Zhang , H. F. Song , Y. Liu

This contribution reviews the present status of the Skyrme-Hartree-Fock (SHF) approach as one of the leading self-consistent mean-field models in the physics of atomic nuclei. It starts with a brief summary of the formalism and strategy for…

核理论 · 物理学 2016-01-26 P. -G. Reinhard

Self-consistency based Kohn-Sham density functional theory (KS-DFT) electronic structure calculations with Gaussian basis sets are reported for a set of 17 protein-like molecules with geometries obtained from the protein data bank. It is…

化学物理 · 物理学 2012-01-10 Elias Rudberg

Persistence diagrams, combining geometry and topology for an effective shape description used in pattern recognition, have already proven to be an effective tool for shape representation with respect to a certainfiltering function.…

代数拓扑 · 数学 2018-12-26 Alessia Angeli , Massimo Ferri , Ivan Tomba

The Hartree-Fock equation admits homogeneous states that model infinitely many particles at equilibrium. We prove their asymptotic stability in large dimensions, under assumptions on the linearised operator. Perturbations are moreover…

偏微分方程分析 · 数学 2025-02-26 Charles Collot , Elena Danesi , Anne-Sophie de Suzzoni , Cyril Malézé

Numerical difficulties associated with computing matrix elements of operators between Hartree-Fock-Bogoliubov (HFB) wavefunctions have plagued the development of HFB-based many-body theories for decades. The problem arises from divisions by…

化学物理 · 物理学 2023-06-09 Guo P. Chen , Gustavo E. Scuseria

The Hartree-Fock equation is a fundamental equation in many-electron problems. It is of practical importance in quantum chemistry to find solutions to the Hartree-Fock equation. The self-consistent field (SCF) method is a standard numerical…

偏微分方程分析 · 数学 2023-11-17 Sohei Ashida

Some general features of the spectrum of the Hartree-Fock-Bogoliubov equations are examined. Special attention is paid to the asymptotic behavior of the single quasiparticle wave functions (s.qp.w.fs.), matter density distribution and…

核理论 · 物理学 2007-05-23 Aurel Bulgac

The Holographic Naturalness (HN) is a new paradigm towards an explanation of the Cosmological Constant (CC) and the Higgs Hierarchy (HH) in the Universe. Motivated by the Holographic Principle, and inspired by the (A)dS/CFT correspondence,…

高能物理 - 理论 · 物理学 2021-02-03 Andrea Addazi

We explore certain properties of the Hartree-Fock approximation to the ground state of the two-dimensional Hubbard model, emphasizing the fact that in the Hartree approach there is an enormous multiplicity of self-consistent solutions which…

强关联电子 · 物理学 2022-06-15 Kazue Matsuyama , Jeff Greensite

We show that the Hartree-Fock (HF) results cannot be reproduced within the framework of Kohn-Sham (KS) theory because the single-particle densities of finite systems obtained within the HF calculations are not $v$-representable, i.e., do…

其他凝聚态物理 · 物理学 2009-11-10 M. Ya. Amusia , A. Z. Msezane , V. R. Shaginyan , D. Sokolovski

A resonant level strongly coupled to a local phonon under nonequilibrium conditions is investigated. The nonequilibrium Hartree-Fock approximation is shown to correspond to approximating the steady state density matrix by delta functions at…

介观与纳米尺度物理 · 物理学 2009-11-10 A. Mitra , I. Aleiner , A. J. Millis