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In a number of experimental situations, single polymer molecules can be suspended in a vacuum. Here collisions between such molecules are considered. The limit of high collision velocity is investigated numerically for a variety of…

软凝聚态物质 · 物理学 2015-05-19 J. M. Deutsch

My means of extensive Monte Carlo simulations the mean radius of gyration and the end-to-end distance are calculated for a single chain in a solvent over a broad range of volume fractions, pressures and temperatures. Our results indicate…

We analyze diffusion of small particles in a solid polymeric medium taking into account a short range particle-polymer interaction. The system is modeled by a particle diffusion on a ternary lattice where the sites occupied by polymer…

统计力学 · 物理学 2015-06-11 Federico Camboni , Andreas Koher , Igor M. Sokolov

The dynamics of polymer-nanoparticle (NP) mixtures, which involves multiple scales and system-specific variables, has posed a long-standing challenge on its theoretical description. In this paper, we construct a microscopic theory for…

软凝聚态物质 · 物理学 2021-06-15 Bokai Zhang , Jian Li , Juan-mei Hu , Lei Liu

We study the conformational properties of complex polymer macromolecules, consisting in general of $n$ subsequently connected chains (blocks) of different lengths and distinct chemical structure. Depending on the solvent conditions, the…

软凝聚态物质 · 物理学 2019-12-03 V. Blavatska , K. Haydukivska

We present an analytical and computational study characterizing the structural and dynamical properties of an active filament confined in cylindrical channels. We first outline the effects of the interplay between confinement and polar…

软凝聚态物质 · 物理学 2024-10-09 José Martín-Roca , Emanuele Locatelli , Valentino Bianco , Paolo Malgaretti , Chantal Valeriani

Stretched polymers with attractive interaction are studied in two and three dimensions. They are described by biased self-avoiding random walks with nearest neighbour attraction. The bias corresponds to opposite forces applied to the first…

统计力学 · 物理学 2009-11-07 Peter Grassberger , Hsiao-Ping Hsu

We consider three different continuum polymer models, that all depend on a tunable parameter r that determines the strength of the excluded-volume interactions. In the first model chains are obtained by concatenating hard spherocylinders of…

软凝聚态物质 · 物理学 2017-10-25 Giuseppe D'Adamo , Andrea Pelissetto

The correlations between the segments of a semidilute polymer solution are found to induce correlations in the positions of small particles added to the solution. Small means a diameter much less than the polymer's correlation length. In…

软凝聚态物质 · 物理学 2009-10-30 Richard P. Sear

Long linear polymers in a depinned interfaces environment have been studied for a long time, for instance in \cite{Caravenna2009depinning} when the temperature is constant. In this paper, we study an extension of this model by making the…

概率论 · 数学 2024-10-10 Angot Elric

We investigate the stretching response of a thick polymer model by means of extensive stochastic simulations. The computational results are synthesized in an analytic expression that characterizes how the force versus elongation curve…

软凝聚态物质 · 物理学 2009-11-11 Ngo Minh Toan , Davide Marenduzzo , Cristian Micheletti

Chain-like macromolecules (polymers) show characteristic adsorption properties due to their flexibility and internal degrees of freedom, when attracted to surfaces and interfaces. In this review we discuss concepts and features that are…

软凝聚态物质 · 物理学 2009-11-07 Roland Netz , David Andelman

A formula is derived for stiffness of a polymer chain in terms of the distribution function of end-to-end vectors. This relationship is applied to calculate the stiffness of Gaussian chains (neutral and carrying electric charges at the…

统计力学 · 物理学 2007-05-23 A. D. Drozdov

Synthetic polymers have a distribution of chain lengths which can be characterized by dispersity, D. Macroscopic properties of polymers are influenced by chain mobility in the melt and manipulating D can significantly impact these…

化学物理 · 物理学 2024-09-30 Taofeek Tejuosho , Sohil Kollipara , Sumant Patankar , Janani Sampath

We consider a model for the distribution of a long homopolymer with a zero-range potential at the origin in $\mathbb{R}^3$. The distribution can be obtained as a limit of Gibbs distributions corresponding to properly normalized potentials…

概率论 · 数学 2009-06-17 M. Cranston , L. Koralov , S. Molchanov , B. Vainberg

In a variety of situations, isolated polymer molecules are found in a vacuum and here we examine their properties. Angular momentum conservation is shown to significantly alter the average size of a chain and its conservation is only broken…

软凝聚态物质 · 物理学 2009-11-13 J. M. Deutsch

Chain-like macromolecules in solution, whether biological or synthetic, transform from an extended conformation to a compact one when temperature or other system parameters change. This collapse transition is relevant in various phenomena,…

软凝聚态物质 · 物理学 2026-05-18 Yanyan Zhu , Haim Diamant , David Andelman

Polymers are widely used in industry and in our daily life because of their diverse functionality, light weight, low cost and excellent chemical stability. However, on some applications such as heat exchangers and electronic packaging, the…

材料科学 · 物理学 2018-05-16 Congliang Huang , Xin Qian , Ronggui Yang

We study the behavior of a flexible polymer chain in the presence of a low-molecular weight solvent in the vicinity of a liquid-gas critical point within the framework of a self-consistent field theory. The total free energy of the dilute…

统计力学 · 物理学 2015-07-29 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , M. G. Kiselev

We explore the critical behaviour of two and three dimensional lattice models of polymers in dilute solution where the monomers carry a magnetic moment which interacts ferromagnetically with near-neighbour monomers. Specifically, the model…

统计力学 · 物理学 2021-08-25 Damien Paul Foster , Debjyoti Majumdar