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The interfacial tension between immiscible liquids is studied as a function of a model linear surfactant length and concentration using coarse grained, dissipative particle dynamics numerical simulations. The adsorption isotherms obtained…

We present a tensor constitutive model for predicting stress and flow-induced structure formation in dilute wormlike micellar solutions. The micellar solution is treated as a dilute suspension of rigid Brownian rods whose length varies…

流体动力学 · 物理学 2017-11-27 Sarit Dutta , Michael D. Graham

Ionic liquids are promising candidates for electrolytes in energy-storage systems. We demonstrate that mixing two ionic liquids allows to precisely tune their physical properties, like the dc conductivity. Moreover, these mixtures enable…

软凝聚态物质 · 物理学 2018-02-27 E. Thoms , P. Sippel , D. Reuter , M. Weiß , A. Loidl , S. Krohns

In a recent numerical study, we have shown that the unsteady motion past a sphere translating steadily in a wormlike micellar solution is caused due to the breakage of long micelles downstream of the sphere once the Weissenberg number…

流体动力学 · 物理学 2022-08-10 Chandi Sasmal

Recent molecular simulation and integral equation results alkali-halide ion pair potentials-of-mean-force in water are discussed. Dielectric model calculations are implemented to check that these models produce that characteristic structure…

chem-ph · 物理学 2008-02-03 Lawrence R. Pratt , Gerhard Hummer , Angel E. Garcia

We derive a self-consistent hydrodynamic theory of coupled binary-fluid-surfactant systems from the underlying microscopic physics using Rayleigh's variational principle. At the microscopic level, surfactant molecules are modelled as…

软凝聚态物质 · 物理学 2026-02-25 Alexandra J. Hardy , Samuel Cameron , Steven McDonald , Abdallah Daddi-Moussa-Ider , Elsen Tjhung

We have investigated thermodynamic and dynamic properties as well as the dielectric constant of water-metha\-nol model mixtures in the entire range of composition by using constant pressure molecular dynamics simulations at ambient…

软凝聚态物质 · 物理学 2015-12-25 E. Galicia-Andrés , H. Dominguez , L. Pusztai , O. Pizio

Isothermal-isobaric molecular dynamics simulations are used to examine the microscopic structure and other properties of a model solution consisting of NaCl salt dissolved in water-methanol mixture. The SPC/E water model and the united atom…

软凝聚态物质 · 物理学 2018-06-27 M. Cruz Sanchez , J. Gujt , S. Sokolowski , O. Pizio

Using statistical field theory supplemented with molecular dynamics simulations, we consider premelting on the surface of ice as a generic consequence of broken hydrogen bonds at the boundary between the condensed and gaseous phases. A…

统计力学 · 物理学 2015-06-22 David T. Limmer , David Chandler

An elastic-visco-plastic thermomechanical model for the simulation of cold forming and subsequent sintering of ceramic powders is introduced and based on micromechanical modelling of the compaction process of granulates. Micromechanics…

计算工程、金融与科学 · 计算机科学 2019-07-19 D. Kempen , A. Piccolroaz , D. Bigoni

Ion complexes hold the key for various energy transfer and communication systems in nature and industries. Achieving controllable mechanical and electrical properties in these complex systems is highly desirable but remains challenging. In…

材料科学 · 物理学 2024-12-18 Jihua Chen , Alejandro Espera , Jan Michael Y. Carrillo , Rigoberto Advincula

We study the structural changes occurring in the isotropic phase of the C$_{12}$=EO$_6$/H$_2$O lyotropic mixture (up to 35% surfactant weight concentration) upon increasing the concentration and temperature, from small individual micelles…

软凝聚态物质 · 物理学 2015-04-09 Doru Constantin , Éric Freyssingeas , Jean-François Palierne , Patrick Oswald

Velocity profiles in a wormlike micelle solution (CTAB in D2O) are recorded using ultrasound every 2 s after a step-like shear rate into the shear-banding regime. The stress relaxation occurs over more than six hours and corresponds to the…

软凝聚态物质 · 物理学 2007-05-23 L. Becu , S. Manneville , A. Colin

We study the effect of the molecular architecture of amphiphilic star polymers on the shape of aggregates they form in water. Both solute and solvent are considered at a coarse-grained level by means of dissipative particle dynamics…

软凝聚态物质 · 物理学 2017-03-31 O. Y. Kalyuzhnyi , J. M. Ilnytskyi , C. von Ferber

Ionic microgels are soft colloidal particles, composed of crosslinked polymer networks, that ionize and swell when dispersed in a good solvent. Swelling of these permeable, compressible particles involves a balance of electrostatic,…

软凝聚态物质 · 物理学 2020-01-29 Alan R. Denton , Mohammed O. Alziyadi

The phase behaviour of amphiphilic multiblock copolymers with a large number of blocks in semidilute solutions is studied by lattice Monte Carlo simulations. The influence on the resulting structures of the concentration, the solvent…

软凝聚态物质 · 物理学 2016-08-18 Virginie Hugouvieux , Monique A. V. Axelos , Max Kolb

Using molecular dynamics simulations and methods of importance sampling, we study the thermodynamics and dynamics of sodium chloride in the aqueous premelting layer formed spontaneously at the interface between ice and its vapor. We uncover…

统计力学 · 物理学 2020-12-21 Samuel P. Niblett , David T. Limmer

Experimental and modeling/simulation studies of phase equilibrium and growth morphologies of novel polymer-dispersed liquid crystal (PDLC) mixtures of PS (polystyrene) and liquid crystals that exhibit a direct isotropic/smectic-A (lamellar)…

软凝聚态物质 · 物理学 2015-05-13 Ezequiel R. Soule , Nasser Mohieddin Abukhdeir , Alejandro D. Rey

Chloride molten salts are increasingly used in pyroprocessing techniques for the separation of lanthanides. Understanding thermodynamic properties of these salts is essential to predict their critical characteristics and optimize the…

Thermodynamic multi-component solution solidification approach to liquid-to-glass transition is proposed and actual mechanisms underlying vitrification, other than viscous slowdown, are identified. Due to polydisperse aggregation in liquid…

材料科学 · 物理学 2022-09-14 Vladimir Belostotsky